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We calculate the microwave spectra of ultracold KRb alkali metal dimers, including hyperfine interactions and in the presence of electric and magnetic fields. We show that microwave transitions may be used to transfer molecules between…

Chemical Physics · Physics 2015-05-13 J. Aldegunde , Hong Ran , Jeremy M. Hutson

We explore the external electric field control of a species of ultralong-range molecules that emerge from the interaction of a ground state polar molecule with a Rydberg atom. The external field mixes the Rydberg electronic states and…

Atomic Physics · Physics 2012-06-01 M. Mayle , S. T. Rittenhouse , P. Schmelcher , H. R. Sadeghpour

The vast majority of QED results are obtained in relatively weak fields and so in the framework of perturbation theory. However, forthcoming laser facilities providing extremely high fields can be used to enter not-yet-studied regimes.…

Plasma Physics · Physics 2019-07-01 C. Baumann , E. N. Nerush , A. Pukhov , I. Yu. Kostyukov

Utilizing single-photon photoassociation, we have achieved ultracold rubidium molecules with a high number density that provides a new efficient approach toward molecular quantum degeneracy. A new detection mechanism for ultracold molecule…

Atomic Physics · Physics 2015-06-12 Jun-Ren Chen , Cheng-Yang Kao , Hung-Bin Chen , Yi-Wei Liu

We model numerically the ultrarelativistic dynamics of a dense plasma microtarget in a focus of several intersecting femtosecond laser pulses of multi-petawatt power each. The aim is to examine perspective future experimental approaches to…

Plasma Physics · Physics 2025-04-03 T. Liseykina , E. Peganov , S. Popruzhenko

A new perspective on how to manipulate molecules by means of very strong laser pulses is emerging with insights from the so-called light-induced potentials, which are the adiabatic potential energy surfaces of molecules severely distorted…

Chemical Physics · Physics 2016-03-03 Bo Y. Chang , Ignacio R. Sola , Seokmin Shin

A method is proposed to manipulate the annihilation dynamics of a dense gas of positronium atoms employing superradiance and subradiance regimes of the cooperative spontaneous emission of the system. The annihilation dynamics is controlled…

Quantum Physics · Physics 2012-06-18 Ni Cui , Mihai Macovei , Karen Z. Hatsagortsyan , Christoph H. Keitel

We probe resonant dipolar interactions between ultracold $^{40}$K$^{87}$Rb molecules and Rydberg $^{87}$Rb atoms in an optically trapped ensemble. Through state-selective ionization detection of the KRb molecules, we observe resonant energy…

Atomic Physics · Physics 2025-04-10 Lingbang Zhu , Jeshurun Luke , Roy Shaham , Yi-Xiang Liu , Kang-Kuen Ni

The formation of ultracold metastable RbCs molecules is observed in a double species magneto-optical trap through photoassociation below the ^85Rb(5S_1/2)+^133Cs(6P_3/2) dissociation limit followed by spontaneous emission. The molecules are…

Atomic Physics · Physics 2015-06-03 N. Bouloufa-Maafa , M. Aymar , O. Dulieu , C. Gabbanini

The lifetimes and decay channels of ultralong-range Rydberg molecules created in a dense BEC are examined by monitoring the time evolution of the Rydberg population using field ionization. Studies of molecules with values of principal…

Ultracold hybrid ion-atom traps offer the possibility of microscopic manipulation of quantum coherences in the gas using the ion as a probe. However, inelastic processes, particularly charge transfer can be a significant process of ion loss…

Atomic Physics · Physics 2015-06-19 B. M. McLaughlin , H. D. L. Lamb , I. C. Lane , J. F. McCann

We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…

Atomic Physics · Physics 2015-10-28 Woojun Lee , Hyosub Kim , Kyungtae Kim , Jaewook Ahn

Gaining control over chemical reactions on the quantum level is a central goal of the modern field of cold and ultracold chemistry. Here, we demonstrate a novel method to coherently steer reaction flux of a three-body recombination process…

Exploring inelastic and reactive collisions on the quantum level is a main goal of the developing field of ultracold chemistry. We present first experimental studies of inelastic collisions of metastable ultracold triplet molecules in the…

We associate Sr atom pairs on sites of a Mott insulator optically and coherently into weakly-bound ground-state molecules, achieving an efficiency above 80\%. This efficiency is 2.5 times higher than in our previous work [S. Stellmer, B.…

Quantum Gases · Physics 2017-07-25 Alessio Ciamei , Alex Bayerle , Chun-Chia Chen , Benjamin Pasquiou , Florian Schreck

Suggestion of modifications of finite-dimensional QED models are proposed for interpreting chemical reactions in terms of artificial atoms and molecules on quantum dots placed in optical cavities. Moving both photons and atoms is possible…

Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

Quantum Physics · Physics 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

Approaching energy coupling in laser-irradiated metals, we point out the role of electron-electron collision as an efficient control factor for ultrafast optical absorption. The high degree of laser-induced electron-ion nonequilibrium…

Chemical reactions at ultracold temperature provide an ideal platform to study chemical reactivity at the fundamental level, and to understand how chemical reactions are governed by quantum mechanics. Recent years have witnessed the…

Quantum Gases · Physics 2019-09-25 Jun Rui , Huan Yang , Lan Liu , De-Chao Zhang , Ya-Xiong Liu , Jue Nan , Bo Zhao , Jian-Wei Pan

Coherent superpositions and entanglement are hallmarks of quantum mechanics, but they are fragile and can easily be perturbed by their environment. Selected isolated physical systems can maintain coherence and generate entanglement using…

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