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Lanthanide-based single-ion magnetic molecules can have large magnetic hyperfine interactions as well as large magnetic anisotropy. Recent experimental studies reported tunability of these properties by changes of chemical environments or…

Materials Science · Physics 2019-10-29 Aleksander L. Wysocki , Kyungwha Park

The influence of hyperfine coupling to nuclear spins and of their quadrupolar splitting on the induced moment order in singlet ground state magnets is investigated. The latter are found among non-Kramers f electron compounds. Without…

Strongly Correlated Electrons · Physics 2025-12-19 Peter Thalmeier

We studied the effect of nuclear-quadrupole interactions on the field-free impulsive alignment of different asymmetric-top molecules. Our analysis is focused on the influence of the hyperfine- and rotational-energy-level structures. These…

Atomic Physics · Physics 2024-08-05 Linda V. Thesing , Andrey Yachmenev , Rosario González-Férez , Jochen Küpper

Molecular spin qubits with long spin coherence time as well as non-invasive operation methods on such qubits are in high demand. It was shown that both molecular electronic and nuclear spin levels can be used as qubits. In solid state…

Materials Science · Physics 2020-10-28 Robert L. Smith , Aleksander L. Wysocki , Kyungwha Park

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

Nuclear spins in $4f$ single-molecule magnets (SMMs) are promising qubits or qudits candidates for quantum information processing due to their relative isolation and reduced susceptibility to environmental disturbances, while hyperfine…

Nuclear spins of dopant atoms in semiconductors are promising candidates as quantum bits, due to the long lifetime of their quantum states. Conventionally, coherent control of nuclear spins is done using ac magnetic fields. Using the…

Mesoscale and Nanoscale Physics · Physics 2018-06-27 Péter Boross , Gábor Széchenyi , András Pályi

The study of highly charged electronic and muonic hydrogen-like ions, provides an intriguing way to probe the internal structure of their atomic nuclei. In this work, we use nuclear structure calculations to accurately calculate the…

Nuclear quadrupole interaction extends the limits imposed by hyperfine interaction on the spin coherence of the electron and nuclei in a quantum dot. The strain-induced nuclear quadrupole interaction suppresses the nuclear spin flip and…

Mesoscale and Nanoscale Physics · Physics 2008-04-01 R. I. Dzhioev , V. L. Korenev

The spin interaction of a hole confined in a quantum dot with the surrounding nuclei is described in terms of an effective magnetic field. We show that, in contrast to the Fermi contact hyperfine interaction for conduction electrons, the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 C. Testelin , F. Bernardot , B. Eble , M. Chamarro

Quantum tunneling dominates the low temperature magnetization dynamics in molecular magnets and presents features that are strongly system dependent. The current discussion is focused on the terbium(III) bis(phtalocyanine)…

Mesoscale and Nanoscale Physics · Physics 2020-04-21 Gheorghe Taran , Edgar Bonet , Wolfgang Wernsdorfer

We investigate the energy levels of heteronuclear alkali metal dimers in levels correlating with the lowest rotational level of the ground electronic state, which are important in efforts to produce ground-state ultracold molecules. We use…

Atomic Physics · Physics 2009-11-13 J. Aldegunde , Ben A. Rivington , Piotr S. Żuchowski , Jeremy M. Hutson

We study the mechanism of dynamical nuclear spin polarization by hyperfine interaction in spin-blocked double quantum dot system. We calculate the hyperfine transition rates and solve the master equations for the nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Changxue Deng , Xuedong Hu

We investigate the hyperfine energy levels and Zeeman splittings for homonuclear alkali-metal dimers in low-lying rotational and vibrational states, which are important for experiments designed to produce quantum gases of deeply bound…

Atomic Physics · Physics 2010-03-09 J. Aldegunde , Jeremy M. Hutson

We analyze the interference between tunneling paths that occurs for a spin system with special Hamiltonian both for dipole and quadrupole excitation. Using an instanton approach, we find that as the strength of the second-order transverse…

Other Condensed Matter · Physics 2015-06-11 Yousef Yousefi , Khikmat Kh. Muminov

Hyperfine interactions between electron and nuclear spins have been widely used in material science, organic chemistry, and structural biology as a sensitive probe to the local chemical environment through spatial identification of nuclear…

Mesoscale and Nanoscale Physics · Physics 2022-12-28 Jinkyung Kim , Kyungju Noh , Yi Chen , Fabio Donati , Andreas J. Heinrich , Christoph Wolf , Yujeong Bae

Optically driven electronic spins coupled in quantum dots to nuclear spins show a pre-pulse signal (revival amplitude) after having been trained by long periodic sequences of pulses. The size of this revival amplitude depends on the…

Mesoscale and Nanoscale Physics · Physics 2024-02-09 Alina Joch , Götz S. Uhrig

The nuclear spins of ionized donors in silicon have become an interesting quantum resource due to their very long coherence times. Their perfect isolation, however, comes at a price, since the absence of the donor electron makes the nuclear…

We investigate interactions between the proton spin, the deuteron spin, and the orbital angular momentum in the electronic ground state of the HD molecule. These interactions lead to hyperfine splittings of molecular energy levels. Our…

Chemical Physics · Physics 2020-07-29 Jacek Komasa , Mariusz Puchalski , Krzysztof Pachucki

Large scale ab initio calculations of the electric contribution (i.e. the electric field gradient) to the electric quadrupole hyperfine interaction constants $B$ for the $5p~^2P_{3/2}$ state in $^{109}$Cd$^+$ ion and the $5s5p~^3P_{1,2}$…

Atomic Physics · Physics 2022-10-05 Benquan Lu , Xiaotong Lu , Tao Wang , Hong Chang
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