Related papers: Quantum-Enhanced continuous-wave stimulated Raman …
Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…
Raman sensing and Raman microscopy are amongst the most specific optical technologies to identify the chemical compounds of unknown samples, and to enable label-free biomedical imaging with molecular contrast. However, the high cost and…
We study the fundamental limits of noise spectroscopy using estimation theory, Faraday rotation probing of an atomic spin system, and squeezed light. We find a simple and general expression for the Fisher information, which quantifies the…
Cavity optomechanical (COM) sensors, enhanced by quantum squeezing or entanglement, have become powerful tools for measuring ultra-weak forces with high precision and sensitivity. However, these sensors usually rely on linear COM couplings,…
The vibrational and electronic properties of 2-dimensinal (2D) materials can be efficiently tuned by external strain due to their good stretchability. Resonant Raman spectroscopy is a versatile tool to study the physics of phonons,…
We develop a system for measurements of power spectra of transmitted light intensity fluctuations, in which the extraneous noise, including shot noise, is reduced. In essence, we just apply light, measure the power of the transmitted light…
Time-resolved spontaneous Raman spectroscopy serves as a probe for incoherent quasiparticle and collective excitation dynamics, and allows to distinguish symmetry changes across a photoinduced phase transition through the inelastic light…
Raman spectroscopy of crystalline/molecular systems is well backed with quantum chemical calculations and group theory, making it a unique characterization tool. For the "intermediate" case of nanoscale systems, however, the use of Raman…
We propose a novel protocol for quantum illumination: a quantum-enhanced noise radar. A two-mode squeezed state, which exhibits continuous-variable entanglement between so-called signal and idler beams, is used as input to the radar system.…
Label-free optical microscopy through absorption or scattering spectroscopy provides fundamental insights across biology and materials science, yet its sensitivity remains fundamentally limited by photon shot noise. While recent…
We create squeezed light by exploiting the quantum nature of the mechanical interaction between laser light and a membrane mechanical resonator embedded in an optical cavity. The radiation pressure shot noise (fluctuating optical force from…
Laser light with squeezed quantum uncertainty is a powerful tool for interferometric sensing. A routine application can be found in gravitational wave observatories. A significant quantum advantage is only achievable if a large fraction of…
Absorption spectroscopy is routinely used to characterise chemical and biological samples. For the state-of-the-art in absorption spectroscopy, precision is theoretically limited by shot-noise due to the fundamental Poisson-distribution of…
We present experimental demonstration of a recently predicted path interference phenomenon [Nanophotonics 7, 1687 (2018)]. A SERS process becomes resonant when both incident and the converted frequencies match with two plasmon resonances --…
We report the observation of all-optically tunable Raman fluorescence from a single quantum dot. The Raman photons are produced in an optically-driven Lambda-system defined by subjecting the single electron charged quantum dot to a magnetic…
Raman spectroscopy reveals chemically specific information and provides label-free insight into the molecular world. However, the signals are intrinsically weak and call for enhancement techniques. Here, we demonstrate Purcell enhancement…
Quantum sensors promise revolutionary advances in medical imaging, energy production, mass detection, geodesy, foundational physics research, and a host of other fields. In many sensors, the signal takes the form of a changing qubit…
Stimulated Raman scattering (SRS) in ultra-high-Q surface-tension-induced spherical and chip-based toroid microcavities is considered both theoretically and experimentally. These microcavities are fabricated from silica, exhibit small mode…
Squeezing of light's quantum noise requires temporal rearranging of photons. This again corresponds to creation of quantum correlations between individual photons. Squeezed light is a non-classical manifestation of light with great…
We study the quantum noise in the harmonic mode of a singly resonant frequency doubler simultaneously driven in both modes. This simple extension of the frequency doubler greatly improves its performance as a bright squeezed light source.…