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The theory of the electron relaxation in metals excited by an ultrashort optical pump is developed on the basis of the solution of the linearized kinetic equation. The kinetic equation includes both the electron-electron and the…

Strongly Correlated Electrons · Physics 2014-03-06 V. V. Baranov , V. V. Kabanov

We study the electron and phonon thermalization in simple metals excited by a laser pulse. The thermalization is investigated numerically by solving the Boltzmann transport equation taking into account all the relevant scattering mechanism:…

Materials Science · Physics 2018-02-28 Shota Ono

We propose a kinetic model of transient nonequilibrium phenomena in metals exposed to ultrashort laser pulses when heated electrons affect the lattice through direct electron-phonon interaction. This model describes the destruction of a…

Statistical Mechanics · Physics 2009-10-31 L. A. Falkovsky , E. G. Mishchenko

Electron and phonon transient temperatures are analyzed in the case of nondegenerate semiconductors. An analytical solution is obtained for rectangular laser pulse absorption. It is shown that thermal diffusion is the main energy relaxation…

Electron-electron thermalization and electron-phonon relaxation processes in laser-excited solids are often assumed to occur on different timescales. This is true for the majority of the conduction band electrons in a metal. However,…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Sebastian T. Weber , Baerbel Rethfeld

The rate of energy transfer between electrons and phonons is investigated by a first principles framework for electron temperatures up to $T_e=50000$ K while considering the lattice at ground state. Two typical but differently complex…

Other Condensed Matter · Physics 2022-03-08 Jia Zhang , Rui Qin , Wenjun Zhu , Jan Vorberger

The equilibration of electronic carriers in metals after excitation by an ultra-short laser pulse provides an important class of non-equilibrium phenomena in metals and allows measuring the effective electron-phonon coupling parameter.…

Materials Science · Physics 2022-10-06 Peter Kratzer , Laurenz Rettig , Irina Yu. Sklyadneva , Evgueni V. Chulkov , Uwe Bovensiepen

The out-of-equilibrium dynamics of electrons and phonons upon laser excitation are often described by the two-temperature model, which assumes that both subsystems are separately in thermal equilibrium. However, recent experiments show that…

Materials Science · Physics 2021-01-04 Ulrike Ritzmann , Peter M. Oppeneer , Pablo Maldonado

We investigate the momentum-resolved dynamics of conduction electrons in noble metals following ultrashort optical excitation with linearly polarized light. Using a momentum-resolved Boltzmann equation approach for electron-phonon…

Mesoscale and Nanoscale Physics · Physics 2025-04-29 Jonas Grumm , Andreas Knorr

Ultrafast electron dynamics of solids after an absorption of femtosecond laser pulse is governed by electron-electron, electron-phonon, phonon-electron, and phonon-phonon collisions. It is of importance to construct a framework for…

Materials Science · Physics 2019-01-16 Shota Ono

We compute the transient dynamics of phonons in contact with high energy "hot" charge carriers in 12 polar and non-polar semiconductors, using a first-principles Boltzmann transport framework. For most materials, we find that the decay in…

Mesoscale and Nanoscale Physics · Physics 2017-10-03 Sridhar Sadasivam , Maria K. Y. Chan , Pierre Darancet

A semiempirical theory for the excitation and subsequent relaxation of nonthermal electrons is described. The theory, which is applicable to ultrafast-laser excited metals, is based on the Boltzmann transport equation for the carrier…

Materials Science · Physics 2023-07-12 D. M. Riffe , Richard B. Wilson

The non-equilibrium dynamics of electrons is of a great experimental and theoretical value providing important microscopic parameters of the Coulomb and electron-phonon interactions in metals and other cold plasmas. Because of the…

Superconductivity · Physics 2008-11-19 V. V. Kabanov , A. S. Alexandrov

The electrons and phonons in metal films after ultra-short pulse laser heating are in highly non-equilibrium states not only between the electron sub-system and the phonon sub-system but also within the electron sub-system. An…

Materials Science · Physics 2014-08-05 Jun Zhou , Nianbei Li , Ronggui Yang

Using the Boltzmann equation for electrons in metals, we show that the optical phonons soften and have a dispersion due to screening in agreement with the results reported recently [M. Reizer, Phys. Rev. B {\bf 61}, 40 (2000)]. Additional…

Materials Science · Physics 2009-11-07 L. A. Falkovsky

A simple bulk model of electron-phonon coupling in metals has been surprisingly successful in explaining experiments on metal films that actually involve surface- or other low-dimensional phonons. However, by an exact application of this…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 S. -X. Qu , A. N. Cleland , M. R. Geller

We study the electron-phonon relaxation in the model of a granular metal film, where the grains are formed by regularly arranged potential barriers of arbitrary transparency. The relaxation rate of Debye acoustic phonons is calculated,…

Mesoscale and Nanoscale Physics · Physics 2023-11-15 Nikolai A. Stepanov , Mikhail A. Skvortsov

The Two Temperature model of M I Kaganov, I M Lifshitz and L V Tanatarov (Sov. Phys. JETP 4, 173 (1957)) about relaxation between electrons and bulk phonons is extended to the case of surface phonons. The state of electrons and phonons is…

Statistical Mechanics · Physics 2009-11-11 Navinder Singh

A model calculation is given for the energy relaxation of a non-equilibrium distribution of hot electrons prepared in a metallic sample that has been subjected to homogeneous photo-excitation by a femtosecond laser pulse. The model assumes…

Statistical Mechanics · Physics 2009-11-11 Navinder Singh

Ultrafast laser excitation of a metal causes correlated, highly nonequilibrium dynamics of electronic and ionic degrees of freedom, which are however only poorly captured by the widely-used two-temperature model. Here we develop an…

Materials Science · Physics 2017-12-06 Pablo Maldonado , Karel Carva , Martina Flammer , Peter M. Oppeneer
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