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Free electron beams such as those employed in electron microscopes have evolved into powerful tools to investigate photonic nanostructures with an unrivaled combination of spatial and spectral precision through the analysis of electron…

Quantum Physics · Physics 2021-04-22 F. Javier García de Abajo , Valerio Di Giulio

Probing optical excitations with nanometer resolution is important for understanding their dynamics and interactions down to the atomic scale. Electron microscopes currently offer the unparalleled ability of rendering spatially-resolved…

Quantum Physics · Physics 2020-07-16 Valerio Di Giulio , Mathieu Kociak , F. Javier García de Abajo

Elementary quasi-particles in a two dimensional electron system can be described as exciton-polarons since electron-exciton interactions ensures dressing of excitons by Fermi-sea electron-hole pair excitations. A relevant open question is…

Mesoscale and Nanoscale Physics · Physics 2018-02-07 Sylvain Ravets , Patrick Knüppel , Stefan Faelt , Martin Kroner , Werner Wegscheider , Atac Imamoglu

We show that the scattering interaction between a high energy electron and a photon can be strongly enhanced by different types of localized plasmons in a non-trivial way. The scattering interaction is predicted by an eigen-response theory,…

Optics · Physics 2014-01-21 Kin Hung Fung , Anil Kumar , Nicholas X. Fang

We theoretically investigate plasmon polaritons in cubic lattices of spherical metallic nanoparticles. The nanoparticles, each supporting triply-degenerate localized surface plasmons, couple through the Coulomb dipole-dipole interaction,…

Mesoscale and Nanoscale Physics · Physics 2018-03-12 Simon Lamowski , Charlie-Ray Mann , Felicitas Hellbach , Eros Mariani , Guillaume Weick , Fabian Pauly

Nonlinear optical processes in low dimensional materials are often weak or symmetry forbidden, limiting their use in nanoscale light sources and on chip frequency conversion. Here, we show that combining two weakly nonlinear systems,…

Plasmons --the collective oscillations of electrons in conducting materials-- play a pivotal role in nanophotonics because of their ability to couple electronic and photonic degrees of freedom. In particular, plasmons in graphene --the…

Materials Science · Physics 2018-05-08 Renwen Yu , F. Javier García de Abajo

Strong coupling of plasmonic excitations and dipolar emitters, such as organic molecules, have been studied extensively in the last years. The questions whether strong coupling can be achieved with a single molecule only and how this is…

Molecular polaritons have gained considerable attention due to their potential to control nanoscale molecular processes by harnessing electromagnetic coherence. Although recent experiments with liquid-phase vibrational polaritons have shown…

Plasmon-emitter interactions are of paramount importance in modern nanoplasmonics and are generally maximal at short emitter-surface separations. However, when the separation falls below 10-20 nm, the classical theory progressively…

Mesoscale and Nanoscale Physics · Physics 2020-01-20 P. A. D. Gonçalves , Thomas Christensen , Nicholas Rivera , Antti-Pekka Jauho , N. Asger Mortensen , Marin Soljačić

Exciton polaritons are hybrid particles of excitons (bound electron-hole pairs) and cavity photons, which are renowned for displaying Bose Einstein condensation and other coherent phenomena at elevated temperatures. However, their formation…

Mesoscale and Nanoscale Physics · Physics 2024-08-29 Kenneth Choo , Olivier Bleu , Jesper Levinsen , Meera M. Parish

We investigate the many-body states of exciton-polaritons that can be observed by pump-probe spectroscopy. Here, a weak-probe `spin-down' polariton is introduced into a coherent state of `spin-up' polaritons created by a strong pump. We…

Hyperbolic phonon polaritons (HPhPs) in hexagonal boron nitride (hBN) enable the direct manipulation of mid-infrared light at nanometer scales, many orders of magnitude below the free-space light wavelength. High resolution monochromated…

We simulate the near-field effects of strong coupling between molecular excitons and localized surface plasmons, supported by aluminum nanodisks. The simulations are done using a simple model of a two-level system, implemented in a…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Nadav Fain , Tal Ellenbogen , Tal Schwartz

Monolayers of transition metal dichalcogenides (TMDC) are direct-gap semiconductors with strong light-matter interactions featuring tightly bound excitons, while plasmonic crystals (PCs), consisting of metal nanoparticles that act as…

Mesoscale and Nanoscale Physics · Physics 2023-09-19 Lara Greten , Robert Salzwedel , Tobias Göde , David Greten , Stephanie Reich , Stephen Hughes , Malte Selig , Andreas Knorr

The electronic excitation of molecules triggers diverse phenomena such as luminescence and photovoltaic effects, which are the bases of various energy-converting devices. Understanding and control of the excitations at the single-molecule…

Chemical Physics · Physics 2017-07-12 Hiroshi Imada , Kuniyuki Miwa , Miyabi Imai-Imada , Shota Kawahara , Kensuke Kimura , Yousoo Kim

Multi-exciton correlations shape the photo-induced response of nanostructured materials, particularly when interactions are enhanced by light confinement. Here multidimensional coherent spectroscopy is used to quantify biexciton and…

Mesoscale and Nanoscale Physics · Physics 2025-07-11 Giuseppe Fumero , Jagannath Paul , Jared K. Wahlstrand , Alan D. Bristow

Formation of dressed light-matter states in optical structures, manifested as Rabi splitting of the eigen energies of a coupled system, is one of the key effects in quantum optics. In pursuing this regime with semiconductors, light is…

In this review we look at the concepts and state-of-the-art concerning the strong coupling of surface plasmon-polariton modes to states associated with quantum emitters such as excitons in J-aggregates, dye molecules and quantum dots. We…

Optics · Physics 2015-01-19 P. Törmä , W. L. Barnes

Understanding the radiative decay of exciton-polaritons is essential for achieving long-lived polaritons - a key prerequisite for enhancing nonlinear and quantum polaritonic effects. However, conventional wisdom - the coupled oscillator…

Optics · Physics 2025-09-01 Jiaxun Song , Li He , Bo Zhen
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