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The circular dichroism (CD) of photoelectrons generated by near-infrared (NIR) laser pulses using multiphoton ionization of excited He$^+$ ions in the 3p(m=+1) state. The ions were prepared by circularly polarized extreme ultraviolet (XUV)…

We investigate few-photon ionization of lithium atoms prepared in the polarized 2$p$($m_\ell=\!+1$) state when subjected to femtosecond light pulses with left- or right-handed circular polarization at wavelengths between 665 nm and 920 nm.…

The photoionization of chiral molecules prepared in a coherent superposition of excited states can give access to the underlying chiral coherent dynamics in a procedure known as photoexcitation induced photoelectron circular dichroism…

Atomic and Molecular Clusters · Physics 2018-08-29 Alex G Harvey , Zdeněk Mašín , Olga Smirnova

Magnetic Circular Dichroism (MCD) is a standard technique for the study of magnetic properties of materials in synchrotron beamlines. We present here a new scattering geometry in the Transmission Electron Microscope through which MCD can be…

Many chirality-sensitive light-matter interactions are governed by chiral electron dynamics. Therefore, the development of advanced technologies harnessing chiral phenomena would critically benefit from measuring and controlling chiral…

Photoelectron diffraction (PED) is a powerful and essential experimental technique for resolving the structure of surfaces with sub-angstrom resolution. In the high energy regime, researchers in angle-resolved photoemission spectroscopy…

The calculations presented here reveal that an electron probe carrying orbital angular momentum is just a particular case of a wider class of electron beams that can be used to measure electron magnetic circular dichroism (EMCD) with atomic…

Materials Science · Physics 2015-06-22 Jan Rusz , Juan-Carlos Idrobo , Somnath Bhowmick

Chiral molecules show differences in their chemical and optical properties due to different spatial arrangements of the atoms in the two enantiomers. A common way to optically differentiate them is to detect the disparity in the absorption…

Altermagnets are a new class of magnetic materials that are promising for spintronics technology. Here it is shown that in altermagnets, the circular dichroism (CD) in resonant photoelectron diffraction (RPED) contains a time-reversal odd…

Materials Science · Physics 2025-09-26 Peter Krüger

A comprehensive study of high-accuracy photoionization cross sections is carried out using the relativistic Breit-Pauli R-matrix (BPRM) method for (hnu + Fe XVII --> Fe XVIII + e). Owing to its importance in high-temperature plasmas the…

Solar and Stellar Astrophysics · Physics 2015-05-27 Sultana N. Nahar , Anil K. Pradhan , Guo-Xin Chen , Werner Eissner

The non-linear response of dielectrics to intense, ultrashort electric fields has been a sustained topic of interest for decades with one of its most important applications being femtosecond laser micro/nano-machining. More recently,…

The angle-resolved inner-shell photoionization of R-trifluoromethyloxirane, C3H3F3O, is studied experimentally and theoretically. Thereby, we investigate the photoelectron circular dichroism (PECD) for nearly-symmetric O 1s and F 1s…

DNA and proteins are chiral: their three-dimensional structure cannot be superimposed with its mirror image. Circular dichroism spectroscopy is widely used to characterize chiral compounds, but data interpretation is difficult in the case…

Biomolecules · Quantitative Biology 2020-09-09 Steven Daly , Frederic Rosu , Valerie Gabelica

Shadow X-ray Magnetic Circular Dichroism Photo-Emission Electron Microscopy (XMCD-PEEM) is a recent technique, in which the photon intensity in the shadow of an object lying on a surface, may be used to gather information about the…

Time-resolved x-ray magnetic circular dichroism (XMCD) enables a unique spectroscopic view on complex spin and charge dynamics in multi-elemental magnetic materials. So far, its application in the soft-x-ray range has been limited to…

Chiroptical effects using circularly polarized light produce signals that change sign when switching either molecular handedness (enantiosensitivity) or the light helicity (circular dichroism). Here, we break this…

Recently it was demonstrated (Schattschneider et al., Nature 441 (2006), 486), that an analogue of the X-ray magnetic circular dichroism (XMCD) experiment can be performed with the transmission electron microscope (TEM). The new phenomenon…

Materials Science · Physics 2009-09-29 Jan Rusz , Stefano Rubino , Peter Schattschneider

PEPSI is the bench-mounted, two-arm, fibre-fed and stabilized Potsdam Echelle Polarimetric and Spectroscopic Instrument for the 2x8.4 m Large Binocular Telescope (LBT). Three spectral resolutions of either 43 000, 120 000 or 270 000 can…

Resonance-enhanced multiphoton ionization (REMPI) is a widely used technique for studying molecular photoionization and producing molecular cations for spectroscopy and dynamics studies. Here, we present a model for describing…

Chemical Physics · Physics 2016-08-24 Matthias Germann , Stefan Willitsch

Circular dichroism (CD) is absorption difference of right-hand and left-hand circularly polarized light by components. CD spectroscopy technique is an important tool for detecting molecular chirality, but the molecular circular dichroism…