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A Monte-carlo (MC) simulation procedure has been developed where the pair bond energies are allowed to take into account the various coordination numbers of surface atoms and the presence of adsorbates. The pair bond energies are calculated…

Materials Science · Physics 2009-10-31 Mahesh Menon , Badal C. Khanra

Engineered nanoparticles made from noble metals, rare-earth oxides or semiconductors are emerging as the central constituents of future nanotech developments. In this review, a survey of the complexing strategies between nanoparticles and…

Materials Science · Physics 2011-08-25 J. -P. Chapel , J. -F. Berret

Experimental results are presented on anomalous behavior of absorption currents in PVDF during the stepwise increase of the voltage applied through a corona. These results, supplemented with the dynamics of the time constant of the electret…

Materials Science · Physics 2009-02-27 A. F. Butenko

Titration of methacrylic acid / ethyl-acrylate copolymers is studied experimentally and theoretically. At low salt concentrations, this polyacid exhibits a plateau in the titration curve below the neutralization point. The plateau has been…

Soft Condensed Matter · Physics 2007-05-23 I. Borukhov , D. Andelman , R. Borrega , M. Cloitre , L. Leibler , H. Orland

First-principles calculations using density functional theory based on norm-conserving pseudopotentials have been performed to investigate the Cs adsorption on the Si(001) surface for 0.5 and 1 ML coverages. We found that the saturation…

Strongly Correlated Electrons · Physics 2007-05-23 R. Shaltaf , E. Mete , S. Ellialtioglu

The behaviour of rod-coil diblock copolymers close to a surface is discussed by using extended scaling methods. The copolymers are immersed in selective solvent such that the rods are likely to aggregate to gain energy. The rods are assumed…

Soft Condensed Matter · Physics 2009-11-11 C. Nowak , T. A. Vilgis

In this paper we perform molecular dynamics simulations of a spherical polyelectrolyte brush and counterions in a salt-free medium. The dielectric discontinuity on the grafted nanoparticle surface is taken into account by the method of…

Soft Condensed Matter · Physics 2018-01-12 Vinicius B. Tergolina , Alexandre P. dos Santos

During the last 3 years, our group has investigated extensively the complexation mechanism between neutral-polyelectrolyte block copolymers with oppositely charged species. These species are surfactant micelles, multivalent counterions and…

Soft Condensed Matter · Physics 2007-05-23 J. -F. Berret , P. Herve , M. Morvan , K. Yokota , M. Destarac , J. Oberdisse , I. Grillo , R. Schweins

A theory is presented which quantitatively accounts for the cooperative adsorption of cationic surfactants to anionic polyelectrolytes. For high salt concentration we find that the critical adsorption concentration (CAC) is a bilinear…

Soft Condensed Matter · Physics 2009-11-13 Paulo S. Kuhn , Yan Levin , Marcia C. Barbosa , Ana Paula Ravazzolo

In detailed microcanonical analyses of densities of states obtained by extensive multicanonical Monte Carlo computer simulations, we investigate the caloric properties of conformational transitions adsorbing polymers experience near…

Statistical Mechanics · Physics 2019-03-27 Monika Möddel , Wolfhard Janke , Michael Bachmann

The theory on the magnetic field energy absorption by metal nanoparticles of a nonspherical shape irradiated with ultrashort laser pulses of different duration is developed. The effect of both the particle surface and the particle shape on…

Mesoscale and Nanoscale Physics · Physics 2019-10-03 N. I. Grigorchuk

We have performed multicanonical chain-growth simulations of a polymer interacting with an adsorbing surface. The polymer, which is not explicitly anchored at the surface, experiences a hierarchy of phase transitions between conformations…

Statistical Mechanics · Physics 2009-11-11 Michael Bachmann , Wolfhard Janke

We present an ab initio study of the structural and electronic properties of styrene molecules adsorbed on the dimerized Si(100) surface at different coverages, ranging from the single-molecule to the full monolayer. The adsorption…

Soft Condensed Matter · Physics 2009-11-11 A. Calzolari , A. Ruini , M. J. Caldas , E. Molinari

We use a coarse-grained molecular dynamics model to study the electrophoretic behaviour of flexible polyelectrolyte chains. We first characterize the static properties of the model with respect to the chain length, the polyelectrolyte…

Soft Condensed Matter · Physics 2008-12-16 Kai Grass , Christian Holm

Metal nanoparticles are receiving increased scientific attention owing to their unique physical and chemical properties that make them suitable for a wide range of applications in diverse fields, such as electrochemistry, biochemistry, and…

Chemical Physics · Physics 2020-10-09 Bendix Petersen , Rafael Roa , Joachim Dzubiella , Matej Kanduc

Polyelectrolyte complexation plays an important role in materials science and biology. The internal structure of the resultant polyelectrolyte complex (PEC) phase dictates properties such as physical state, response to external stimuli, and…

A theoretical model of vapor-liquid phase transition in a system of charged hard cores of different diameters is suggested (with the parameters of the transition obtained in a number of studies using the Monte Carlo method). The model is…

Plasma Physics · Physics 2007-05-23 A. L. Khomkin , I. A. Mulenko

A spherical quantum dot (QD) heterosystem CdS/SiO$_2$ has been studied. Each QD has a hydrogen-like impurity in its center. Besides that, it has been accounted that a polarization trap for electron exists at the interfaces due to the…

Mesoscale and Nanoscale Physics · Physics 2017-12-15 V. I. Boichuk , R. Ya. Leshko , D. S. Karpyn

Enantioselective interactions of chiral molecules include distinct absorptions to opposite-handed circularly polarized light, known as chiral absorption. Traditionally, chiral absorption has been primarily attributed to electric dipole and…

Optics · Physics 2024-06-03 Hanwei Wang , Yang Zhao

We investigate a model nanopore sensor that is able to detect analyte ions that are present in the electrolyte solution in very small concentrations. The nanopore selectively binds the analyte ions with which the local concentrations of the…

Applied Physics · Physics 2018-12-31 Eszter Mádai , Mónika Valiskó , Dezső Boda