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Photoluminesce (PL) spectroscopy offers excellent methods for mapping the PL decay on the nanosecond time scale. However, capturing maps of emission dynamics on the microsecond time scale can be highly time-consuming. We present a new…

Optics · Physics 2021-02-24 Jiri Junek , Karel Zidek

RAndom Temporal Signals (RATS) method has proven to be a useful and versatile method for measuring photoluminescence (PL) dynamics and fluorescence lifetime imaging (FLIM). Here, we present two fundamental development steps in the method.…

Optics · Physics 2023-02-15 Jiri Junek , Karel Zidek

Speckled illumination enhances widefield fluorescence microscopy by enabling optical sectioning and super resolution. In random illumination microscopy, sequences of speckled illumination patterns are used to excite fluorescent samples and…

Time-resolved photoluminescence is a validated method for tracking the photoexcited carrier dynamics in luminescent materials. This technique probes the photoluminescence decays upon a periodic excitation by short laser pulses. Herein, we…

Ultra-high intensity femtosecond lasers at focus are now routinely used for relativistic motion of charged particles with peak intensities over 10^18W/cm^2. Such high-field experiments are very sensitive to the value of the peak intensity.…

Optics · Physics 2020-05-25 Thomas Oksenhendler

We investigate valley exciton dynamics in MoSe2 monolayers in polarization- and time-resolved photoluminescence (PL) spectroscopy at 4K. Following circularly polarized laser excitation, we record a low circular polarization degree of the PL…

Materials Science · Physics 2015-03-19 G. Wang , E. Palleau , T. Amand , S. Tongay , X. Marie , B. Urbaszek

Ultrafast lasers ($< 500$ fs) have enabled laser-matter interactions at intensities exceeding $10^{18} \rm{Wcm}^{-2}$ with only millijoules of laser energy. However, as pulse durations become shorter, larger spectral bandwidths are…

We show that, in optical pump-probe experiments on bulk samples, the statistical distribution of the intensity of ultrashort light pulses after the interaction with a nonequilibrium complex material can be used to measure the time-dependent…

Strongly Correlated Electrons · Physics 2017-11-08 Francesco Randi , Martina Esposito , Francesca Giusti , Fulvio Parmigiani , Oleg Misochko , Daniele Fausti , Martin Eckstein

Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…

Photoluminescence (PL) is a fundamental light-matter interaction in which absorbed photons are re-emitted, playing a key role in science and engineering. It is commonly modeled by introducing a non-zero chemical potential into Planck's law…

Optics · Physics 2026-04-22 Tomer Bar Lev , Carmel Rotschild

In this paper we describe the technical implementation of pump-probe cathodoluminescence microscopy (PP-CL), a novel technique for studying ultrafast dynamics in materials using combined excitation of electron and laser pulses. The PP-CL…

Instrumentation and Detectors · Physics 2021-12-07 Magdalena Solà-Garcia , Kelly W. Mauser , Nika van Nielen , Toon Coenen , Sophie Meuret , Albert Polman

The measurement of weak temporal phase for picosecond and nanosecond laser pulses is important but quite difficult. We propose a simple iterative algorithm, which is based on a temporally movable phase modulation process, to retrieve the…

Optics · Physics 2016-07-06 Zhi Qiao , Yudong Yao , Xiaochao Wang , Yuanyuan Jing , Wei Fan , Zunqi Lin

Accurate spatio-temporal and spatio-spectral metrology is critical to the characterization and use of ultra-short, high-power lasers. The emergence of few cycle pulses, with bandwidths of tens or hundreds of nanometers, poses a significant…

We study the evolution of photoluminescence (PL) from homogeneous and inhomogeneous ensembles of a few coupled QDs. We discuss the relation between signals from a given QD ensemble under strong and weak excitation (full inversion and linear…

Mesoscale and Nanoscale Physics · Physics 2015-03-10 Wildan Abdussalam , Paweł Machnikowski

A phase retrieval technique using a spatial light modulator (SLM) and a phase diffuser for a fast reconstruction of smooth wave fronts is demonstrated experimentally. Diffuse illumination of a smooth test object with the aid of a phase…

Optics · Physics 2015-06-11 Mostafa Agour , Percival F. Almoro , Claas Falldorf

Time Resolved Correlation (TRC) is a recently introduced light scattering technique that allows to detect and quantify dynamic heterogeneities. The technique is based on the analysis of the temporal evolution of the speckle pattern…

Soft Condensed Matter · Physics 2007-05-23 Agnes Duri , Hugo Bissig , Veronique Trappe , Luca Cipelletti

Transverse deflecting structures (TDS) are widely used in accelerator physics to measure the longitudinal density of particle bunches. When used in combination with a dispersive section, the whole longitudinal phase space density can be…

Specific heat and linear thermal expansivity are fundamental thermal dynamics and have been proven as interesting relaxing quantities to investigate in glass transition and glassy state. However, their possibility has much less been…

Soft Condensed Matter · Physics 2021-09-06 Pengfei Zhang , Marco Gandolfi , Francesco Banfi , Christ Glorieux , Liwang Liu

While transient photoluminescence measurements are a very popular tool to monitor the charge-carrier dynamics in the field of halide perovskite photovoltaics, interpretation of data obtained on multilayer samples is highly challenging due…

Materials Science · Physics 2021-02-18 Lisa Krückemeier , Benedikt Krogmeier , Zhifa Liu , Uwe Rau , Thomas Kirchartz

We experimentally demonstrate spectral broadening and shaping of exponentially-decaying nanosecond pulses via nonlinear mixing with a phase-modulated pump in a periodically-poled lithium niobate (PPLN) waveguide. A strong, 1550~nm pulse is…

Optics · Physics 2015-06-22 Imad Agha , Serkan Ates , Luca Sapienza , Kartik Srinivasan
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