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We describe a fully broadband approach for electron spin resonance (ESR) experiments where it is possible to not only tune the magnetic field but also the frequency continuously over wide ranges. Here a metallic coplanar transmission line…

We present non-conventional electron spin resonance (ESR) experiments using microfabricated superconducting waveguides. We show that a very broad frequency range, from 0.5 to 40 GHz, becomes accessible with a high frequency accuracy of less…

Mesoscale and Nanoscale Physics · Physics 2014-01-13 C. Clauss , D. Bothner , D. Koelle , R. Kleiner , L. Bogani , M. Scheffler , M. Dressel

We report the development of the frequency-modulation (FM) method for measuring electron spin resonance (ESR) absorption in the 210-420 GHz frequency range. We demonstrate that using a high-frequency ESR spectrometer without resonating…

Strongly Correlated Electrons · Physics 2010-07-14 Balint Nafradi , Richard Gaal , Titusz Feher , Laszlo Forro

We report the development of a continuous-wave and pulsed X-band electron spin resonance (ESR) spectrometer for the study of spins on ordered surfaces down to cryogenic temperatures. The spectrometer operates in ultra-high vacuum and…

We describe instrumentation for a high-frequency electron paramagnetic resonance (EPR) and pulsed electron-electron double resonance (PELDOR) spectroscopy. The instrumentation is operated in the frequency range of 107$-$120 GHz and…

Instrumentation and Detectors · Physics 2015-06-19 Franklin H. Cho , Viktor Stepanov , Susumu Takahashi

In this work, we demonstrate the use of frequency-tunable superconducting NbTiN coplanar waveguide microresonators for multi-frequency pulsed electron spin resonance (ESR) experiments. By applying a bias current to the center pin, the…

Quantum Physics · Physics 2017-07-19 A. T. Asfaw , A. J. Sigillito , A. M. Tyryshkin , T. Schenkel , S. A. Lyon

We present a new experimental approach to investigate the magnetic properties of the anisotropic heavy-fermion system YbRh$_2$Si$_2$ as a function of crystallographic orientation. Angle-dependent electron spin resonance (ESR) measurements…

In this work, we study the development of a coplanar waveguide (CPW) resonator and its use in an electron spin resonance (ESR) spectrometer. The CPW resonator is designed to operate in S-band. It has a short circuit configuration which…

Applied Physics · Physics 2020-12-16 Subhadip Roy , Anuvab Nandi , Pronoy Das , Chiranjib Mitra

The design and performance of an electron spin resonance spectrometer operating at 3 and 9 GHz microwave frequencies combined with a 9 T superconducting magnet is described. The probehead contains a compact two-loop, one gap resonator and…

Other Condensed Matter · Physics 2009-11-10 Ferenc Simon , Ferenc Muranyi

We report pulsed electron-spin resonance (ESR) measurements on an ensemble of Bismuth donors in Silicon cooled at 10mK in a dilution refrigerator. Using a Josephson parametric microwave amplifier combined with high-quality factor…

We present three designs for planar superconducting microwave resonators for electron spin resonance (ESR) experiments. We implement finite element simulations to calculate the resonance frequency and quality factors as well as the…

Mesoscale and Nanoscale Physics · Physics 2019-08-21 Stefan Weichselbaumer , Petio Natzkin , Christoph W. Zollitsch , Mathias Weiler , Rudolf Gross , Hans Huebl

The quest to enhance the sensitivity of electron spin resonance (ESR) is an ongoing challenge. One potential strategy involves increasing the frequency, for instance, moving from Q-band (approximately 35 GHz) to W-band (approximately 94…

Chemical Physics · Physics 2024-11-22 Moamen Jbara , Oleg Zgadzai , Wolfgang Harneit , Aharon Blank

We report on electron spin resonance (ESR) measurements of phosphorus donors localized in a 200 square micron area below the inductive wire of a lumped element superconducting resonator. By combining quantum limited parametric amplification…

Mesoscale and Nanoscale Physics · Physics 2017-02-10 C. Eichler , A. J. Sigillito , S. A. Lyon , J. R. Petta

We present a comprehensive exploration of loop-gap resonators (LGRs) for electron spin resonance (ESR) studies, enabling investigations into the hybridization of solid-state magnetic materials with microwave polariton modes. The…

Strongly Correlated Electrons · Physics 2024-02-02 Aulden K. Jones , Martin Mourigal , Andrew M. Mounce , Michael P. Lilly

We report electron spin resonance spectroscopy measurements performed at millikelvin temperatures in a custom-built spectrometer comprising a superconducting micro-resonator at $7$ GHz and a Josephson parametric amplifier. Owing to the…

We describe a quasi-optical multifrequency ESR spectrometer operating in the 75-225 GHz range and optimized at 210 GHz for general use in condensed matter physics, chemistry and biology. The quasi-optical bridge detects the change of mm…

Materials Science · Physics 2012-10-23 Kalman L Nagy , Dario Quintavalle , Titusz Feher , Andras Janossy

The spin dynamics of the ferromagnetic Kondo lattice CeRuPO is investigated by Electron Spin Resonance (ESR) at microwave frequencies of 1, 9.4, and 34~GHz. The measured resonance can be ascribed to a rarely observed bulk Ce3+ resonance in…

Strongly Correlated Electrons · Physics 2010-10-13 T. Förster , J. Sichelschmidt , C. Krellner , C. Geibel , F. Steglich

A systematic electron spin resonance (ESR) investigation of the low temperature regime for the (ET)2SF5CF2SO3 system was performed in the frequency range of ~200-700 GHz, using backward wave oscillator sources, and at fields up to 25 T.…

We establish a testbed system for the development of high-sensitivity Electron Spin Resonance (ESR) techniques for small samples at cryogenic temperatures. Our system consists of a Niobium Nitride thin-film planar superconducting…

The use of superconducting micro-resonators in combination with quantum-limited Josephson parametric amplifiers has in recent years lead to more than four orders of magnitude improvement in the sensitivity of pulsed Electron Spin Resonance…

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