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Despite its reasonable accuracy for ground-state properties of semiconductors and insulators, second-order Moller-Plesset perturbation theory (MP2) significantly underestimates band gaps. Here, we evaluate the band gap predictions of…

Materials Science · Physics 2021-09-15 Malte F. Lange , Timothy C. Berkelbach

Despite decades of practice, finite-size errors in many widely used electronic structure theories for periodic systems remain poorly understood. For periodic systems using a general Monkhorst-Pack grid, there has been no comprehensive and…

Computational Physics · Physics 2023-11-16 Xin Xing , Xiaoxu Li , Lin Lin

We revisit the extraction of $\alpha_s(M_\tau^2)$ from the QCDperturbative corrections to the hadronic $\tau$ branching ratio, using an improved fixed-order perturbation theory based on the explicit summation of all renormalization-group…

High Energy Physics - Phenomenology · Physics 2012-05-22 Gauhar Abbas , B. Ananthanarayan , Irinel Caprini

We study the adiabatic connection that has as weak-coupling expansion the M{\o}ller-Plesset perturbation series, generalizing to the open-shell case previous closed-shell results for the large-coupling limit. We first focus on the hydrogen…

Chemical Physics · Physics 2024-04-01 Kimberly J. Daas , Eveline Klute , Michael Seidl , Paola Gori-Giorgi

We propose estimators for dynamic second order response theory in coarse grained variables for driven out-of-equilibrium subsystems. The error is controlled through the the notion of subsystem spectral gap for the convergence of coarse…

Probability · Mathematics 2024-11-19 Fenna Müller , Max von Renesse

The adaptive perturbation method decomposes a Hamiltonian by the diagonal elements and non-diagonal elements of the Fock state. The diagonal elements of the Fock state are solvable but can contain the information about coupling constants.…

High Energy Physics - Theory · Physics 2020-12-25 Chen-Te Ma

The original formulation (Phys. Rev. Lett. 119, 063002, 2017) of the natural orbital functional - second-order M{\o}ller-Plesset (NOF-MP2) method is based on the MP2 that uses the canonical Hartree-Fock molecular orbitals. The current work…

Chemical Physics · Physics 2018-08-22 Mario Piris

The adiabatic approximation in quantum mechanics is considered in the case where the self-adjoint hamiltonian $H_0(t)$, satisfying the usual spectral gap assumption in this context, is perturbed by a term of the form $\epsilon H_1(t)$. Here…

funct-an · Mathematics 2008-02-03 Alain Joye

We performed all-electron ab initio self-consistent field Hartree-Fock linear combination of atomic orbital, in which electronic correlation using density functional were included to perform electronic calculations in MgB2 new…

Materials Science · Physics 2007-05-23 Armando Reyes-Serrato , Donald H. Galvan

The Atom-Calibrated Basis-set Extrapolation (ACBE) method is introduced as a robust approach for extrapolating MP2 correlation energies from small basis sets. Unlike conventional extrapolation techniques, ACBE incorporates system- and…

Chemical Physics · Physics 2025-04-07 E. Fabiano , F. Della Sala

We confront predictions of inflationary scenarios with the WMAP data, in combination with complementary small-scale CMB measurements and large-scale structure data. The WMAP detection of a large-angle anti-correlation in the…

In adiabatic quantum computing finding the dependence of the gap of the Hamiltonian as a function of the parameter varied during the adiabatic sweep is crucial in order to optimize the speed of the computation. Inspired by this challenge,…

Quantum Physics · Physics 2023-06-14 Naeimeh Mohseni , Carlos Navarrete-Benlloch , Tim Byrnes , Florian Marquardt

${\cal H}^2$-matrix constitutes a general mathematical framework for efficient computation of both partial-differential-equation and integral-equation-based operators. Existing linear-complexity ${\cal H}^2$ matrix-matrix product (MMP)…

Numerical Analysis · Mathematics 2019-08-15 Miaomiao Ma , Dan Jiao

We adapt a variational procedure to calculate ground state properties of the Holstein model in the adiabatic limit. At strong coupling, this adaption leads to rapid convergence of results. The intermediate coupling regime is further handled…

Strongly Correlated Electrons · Physics 2010-03-10 Zhou Li , D. Baillie , C. Blois , F. Marsiglio

The maximum a posteriori (MAP) configuration of binary variable models with submodular graph-structured energy functions can be found efficiently and exactly by graph cuts. Max-product belief propagation (MP) has been shown to be suboptimal…

Machine Learning · Computer Science 2012-02-19 Daniel Tarlow , Inmar E. Givoni , Richard S. Zemel , Brendan J. Frey

Considering the worst-case scenario, junction tree algorithm remains the most general solution for exact MAP inference with polynomial run-time guarantees. Unfortunately, its main tractability assumption requires the treewidth of a…

Discrete Mathematics · Computer Science 2022-02-10 Alexander Bauer , Shinichi Nakajima

Graphs are a highly expressive data structure, but it is often difficult for humans to find patterns from a complex graph. Hence, generating human-interpretable sequences from graphs have gained interest, called graph2seq learning. It is…

Machine Learning · Computer Science 2022-01-31 Takeshi D. Itoh , Takatomi Kubo , Kazushi Ikeda

An adiabatic-connection fluctuation-dissipation theorem approach based on a range separation of electron-electron interactions is proposed. It involves a rigorous combination of short-range density functional and long-range random phase…

Materials Science · Physics 2009-03-03 Julien Toulouse , Iann C. Gerber , Georg Jansen , Andreas Savin , János G. Ángyán

We investigate the adiabatic approximation to the exact-exchange kernel for calculating correlation energies within the adiabatic-connection fluctuation-dissipation framework of time-dependent density functional theory. A numerical study is…

Chemical Physics · Physics 2023-05-12 Maria Hellgren , Lucas Baguet

The Homotopy Analysis Method (HAM) is a widely used analytical approach for solving nonlinear problems, yet its theoretical foundation lacks rigorous justification, and its intrinsic correlation with perturbation theory remains ambiguous,…

General Mathematics · Mathematics 2026-04-16 Hang Xu