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Embedding a WS$_2$ monolayer in flakes of hexagonal boron nitride allowed us to resolve and study the photoluminescence response due to both singlet and triplet states of negatively charged excitons (trions) in this atomically thin…

Mesoscale and Nanoscale Physics · Physics 2018-06-08 D. Vaclavkova , J. Wyzula , K. Nogajewski , M. Bartos , A. O. Slobodeniuk , C. Faugeras , M. Potemski , M. R. Molas

There has been a massive growth in the study of transition metal dichalcogenides (TMDs) over the past decade, based upon their interesting and unusual electronic, optical and mechanical properties, such as tuneable and strain-dependent…

Applied Physics · Physics 2020-11-02 Fang Wang , Suhao Li , Mark A. Bissett , Ian A. Kinloch , Zheling Li , Robert J. Young

The ultrafast formation of strongly bound excitons in two-dimensional semiconductors provide a rich platform for studying fundamental physics as well as developing novel optoelectronic technologies. While extensive research has explored the…

Tuning the electronic properties of a material by subjecting it to strain constitutes an important strategy to enhance the performance of semiconducting electronic devices. Using local strain, confinement potentials for excitons can be…

Monolayers of transition metal dichalcogenides (TMDs) have recently emerged as a promising optoelectronic platform. To leverage their full potential, however, it is important to understand and engineer the properties of the different…

One of the fascinating properties of the new families of two-dimensional crystals is their high stretchability and the possibility to use external strain to manipulate, in a controlled manner, their optical and electronic properties. Strain…

Mesoscale and Nanoscale Physics · Physics 2015-07-24 Rafael Roldán , Andres Castellanos-Gomez , Emmanuele Cappelluti , Francisco Guinea

As device miniaturization approaches the atomic limit, it becomes highly desirable to exploit novel paradigms for tailoring electronic structures and carrier dynamics in materials. Elastic strain can in principle be applied to achieve…

Materials Science · Physics 2013-07-10 Xuewen Fu , Cong Su , Qiang Fu , Xinli Zhu , Rui Zhu , Chuanpu Liu , Jun Xu , Ji Feng , Ju Li , Dapeng Yu

Strain provides an effective means to tune the electrical properties while retaining the native chemical composition of the material. Unlike three-dimensional solids, two-dimensional materials withstand higher levels of elastic strain…

Mesoscale and Nanoscale Physics · Physics 2020-04-14 Ashby Phillip John , Arya Thenapparambil , Madhu Thalakulam

Charged excitons, or X$^{\pm}$-trions, in monolayer transition metal dichalcogenides have binding energies of several tens of meV. Together with the neutral exciton X$^0$ they dominate the emission spectrum at low and elevated temperatures.…

In monolayer transition metal dichalcogenides, quantum emitters are associated with localized strain that can be deterministically applied to create designer nano-arrays of single photon sources. Despite an overwhelming empirical…

Strain engineering has arisen as a powerful technique to tune the electronic and optical properties of two-dimensional semiconductors like molybdenum disulfide (MoS2). Although several theoretical works predicted that biaxial strain would…

Applied Physics · Physics 2021-05-11 Felix Carrascoso , Riccardo Frisenda , Andres Castellanos-Gomez

Monolayers of transition metal dichalcogenides (TMDs) have a remarkable excitonic landscape with deeply bound bright and dark exciton states. Their properties are strongly affected by lattice distortions that can be created in a controlled…

Atomically thin two-dimensional semiconducting transition metal dichalcogenides (TMDs) can withstand large levels of strain before their irreversible damage occurs. This unique property offers a promising route for control of the optical…

Strain engineering has emerged as a powerful tool to modify the optical and electronic properties of two-dimensional crystals. Here we perform a systematic study of strained semiconducting transition metal dichalcogenides. The effect of…

Materials Science · Physics 2015-11-24 Habib Rostami , Rafael Roldán , Emmanuele Cappelluti , Reza Asgari , Francisco Guinea

Two dimensional (2D) van der Waals (vdW) magnetic semiconductors are a new class of quantum materials for studying the emergent physics of excitons and spins in the 2D limit. Twist engineering provides a powerful tool to manipulate the…

We revisit low-temperature optical spectra of transition-metal dichalcogenide monolayers and point to a possible crystallization of electrons (or holes) at low to moderate charge densities. To calculate the excitonic spectra under such…

Mesoscale and Nanoscale Physics · Physics 2023-08-16 Dinh Van Tuan , Hanan Dery

Herein, we present an experimental demonstration of the robust exciton-trion polaritons (ETPs) by measuring and simulating the resonance reflectance spectra of various configurational WS2 monolayers with different dielectric screenings.…

Semiconducting Transition Metal Dichalcogenides (TMDs) have significant nonlinear optical effects. In this work we have used second-harmonic generation (SHG) and the four-wave mixing (FWM) spectroscopy in resonance with the excitons in…

Exciton-phonon interactions in transition metal dichalcogenides (TMD) are strong and lead to phenomena such as coherent phonon generation. When stacked and twisted, their properties can be tuned by the twisting angle. In experiments with…

Materials Science · Physics 2026-05-01 Rafael R. Del Grande , David A. Strubbe

Electrical control of individual spins and photons in solids is key for quantum technologies, but scaling down to small, static systems remains challenging. Here, we demonstrate nanoscale electrical tuning of neutral and charged excitons in…

Mesoscale and Nanoscale Physics · Physics 2023-11-01 Jawaher Almutlaq , Jiangtao Wang , Linsen Li , Chao Li , Tong Dang , Vladimir Bulović , Jing Kong , Dirk Englund