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CrI3 is a layered ferromagnetic insulator that has recently attracted enormous interest as it was the first example of a stand-alone monolayer ferromagnet, paving the way towards the study of two-dimensional magnetic materials and their use…

The recent discovery of ferromagnetism in 2D van der Waals (vdw) crystals has generated widespread interest, owing to their potential for fundamental and applied research. Advancing the understanding and applications of vdw magnets requires…

Integrating monolayers derived from 2D van der Waals (vdW) magnetic materials into next-generation technological applications remains a significant challenge due to their structural and magnetic instability issues. Template-assisted…

Materials Science · Physics 2025-10-08 Ihsan Caha , Aqrab ul Ahmad , Francis Leonard Deepak

Two-dimensional (2D) layered magnetic materials are generating a great amount of interest for the next generation of electronic devices thanks to their remarkable properties associated to spin dynamics. The recently discovered layered…

Since the celebrated discovery of graphene, the family of two-dimensional (2D) materials has grown to encompass a broad range of electronic properties. Recent additions include spin-valley coupled semiconductors, Ising superconductors that…

The magnetic properties in two-dimensional van der Waals materials depend sensitively on structure. CrI3, as an example, has been recently demonstrated to exhibit distinct magnetic properties depending on the layer thickness and stacking…

Two dimensional (2D) van der Waals (vdW) materials have demonstrated fascinating optical, electrical and thickness-dependent characteristics. These have been explored by numerous authors but reports on magnetic properties and spintronic…

The synthesis of two-dimensional van der Waals magnets has paved the way for both technological applications and fundamental research on magnetism confined to ultra-small length scales. Edge magnetic moments in ferromagnets are expected to…

The crystallographic, magnetic, and transport properties of the van der Waals bonded, layered compound CrTe3 have been investigated on single crystal and polycrystalline materials. The crystal structure contains layers made up of lozenge…

Strongly Correlated Electrons · Physics 2017-04-19 Michael A. McGuire , V. Ovidiu Garlea , Santosh KC , Valentino R. Cooper , Jiaqiang Yan , Huibo Cao , Brian C. Sales

The recent experimental discovery of intrinsic ferromagnetism in single-layer CrI3 opens a new avenue to low-dimensional spintronics. However, the low Curie temperature Tc=45 K is still a large obstacle to its realistic device application.…

Materials Science · Physics 2019-06-26 Hongxing Li , Yuan-Kai Xu , Kang Lai , Wei-Bing Zhang

Graphene-based heterostructures are a promising material system for designing the topologically nontrivial Chern insulating devices. Recently, a two-dimensional (2D) monolayer ferromagnetic insulator CrI$_{3}$ was successfully synthesized…

Materials Science · Physics 2018-02-07 Jiayong Zhang , Bao Zhao , Tong Zhou , Yang Xue , Chunlan Ma , Zhongqin Yang

To broaden the scope of van der Waals 2D magnets, we report the synthesis and magnetism of covalent 2D magnetic Cr$_2$Te$_3$ with a thickness down to one-unit-cell. The 2D Cr$_2$Te$_3$ crystals exhibit robust ferromagnetism with a Curie…

The mechanical properties of magnetic materials are instrumental for the development of the magnetoelastic theory and the optimization of strain-modulated magnetic devices. In particular, two-dimensional (2D) magnets hold promise to enlarge…

Among the recently widely studied van der Waals layered magnets CrX3 (X=Cl, Br, I), CrCl3 monolayer (ML) is particularly puzzling as it is solely shown by experiments to have an in-plane magnetic easy axis and, furthermore, all of previous…

Materials Science · Physics 2020-01-08 Feng Xue , Yusheng Hou , Zhe Wang , Ruqian Wu

Van der Waals (vdW) ferromagnets are an important class of materials for spintronics applications. The recent discovery of atomically vdW magnets CrI$_3$ and Cr$_2$Ge$_2$Te$_6$ has triggered a renaissance in the area of two-dimensional (2D)…

Strongly Correlated Electrons · Physics 2021-10-22 Yu Liu , Zhixiang Hu , Eli Stavitski , Klaus Attenkofer , C. Petrovic

The van der Waals magnets CrX$_3$ (X = I, Br, and Cl) exhibit highly tunable magnetic properties and are promising candidates for developing novel two-dimensional (2D) magnetic devices such as magnetic tunnel junctions and spin tunneling…

Mesoscale and Nanoscale Physics · Physics 2022-12-06 Jia Wang , Zahra Ahmadi , David Lujan , Jeongheon Choe , Takashi Taniguchi , Kenji Watanabe , Xiaoqin Li , Jeffrey E. Shield , Xia Hong

The recent discovery of magnetism in atomically thin layers of van der Waals (vdW) crystals has created new opportunities for exploring magnetic phenomena in the two-dimensional (2D) limit. In most 2D magnets studied to date the c-axis is…

Recently intrinsic ferromagnetism in two-dimensional(2D) van der Waals materials was discovered [1, 2, 3]. A monolayer of Chromiun triiodide(CrI3) is ferromagnetic while a bilayer structure was reported to be anti-ferro magnetic, moreover…

Materials Science · Physics 2018-11-30 E. Suarez Morell , Andrea León , R. Hiroki Miwa , P. Vargas

Two-dimensional (2D) magnetic materials offer unprecedented opportunities for fundamental physics and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2Ge2Te6, this emerging field has expanded to…

Magnetic layered van der Waals crystals are an emerging class of materials giving access to new physical phenomena, as illustrated by the recent observation of 2D ferromagnetism in Cr2Ge2Te6 and CrI3. Of particular interest in…

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