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X-ray Free Electron Lasers (XFEL) are revolutionary photons sources, whose ultrashort, brilliant pulses are expected to allow single molecule diffraction experiments providing structural information on the atomic length scale. This ultimate…

Optics · Physics 2015-05-20 Andrea Fratalocchi , Giancarlo Ruocco

We propose and examine the use of biphoton pairs, such as those created in parametric down conversion or four-wave mixing, to enhance the precision and the resolution of measuring optical displacements by position-sensitive detection. We…

Quantum Physics · Physics 2016-05-04 Kevin Lyons , Shengshi Pang , Paul G. Kwiat , Andrew N. Jordan

Accurate spatio-temporal and spatio-spectral metrology is critical to the characterization and use of ultra-short, high-power lasers. The emergence of few cycle pulses, with bandwidths of tens or hundreds of nanometers, poses a significant…

Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that…

Quantum Physics · Physics 2021-08-25 Stefan Lerch , André Stefanov

Multiphoton interference is an essential phenomenon at the very heart not only of fundamental quantum optics and applications in quantum information processing and sensing but also of demonstrations of quantum computational supremacy in…

Quantum Physics · Physics 2023-12-25 Vincenzo Tamma , Simon Laibacher

Entangled photons have the remarkable ability to be more sensitive to signal and less sensitive to noise than classical light. Joint photons can sample an object collectively, resulting in faster phase accumulation and higher spatial…

Optics · Physics 2015-09-04 Chien-Hung Lu , Matthew Reichert , Xiaohang Sun , Jason W. Fleischer

Time-resolved measurements of materials provide a wealth of information on quasiparticle dynamics, and have been the focus of optical studies for decades. In this paper, we develop a theory for explicitly evaluating time-resolved resonant…

Strongly Correlated Electrons · Physics 2019-03-27 Yuan Chen , Yao Wang , Chunjing Jia , Brian Moritz , Andrij M. Shvaika , James K. Freericks , Thomas P. Devereaux

Spectral diffusion is a result of random spectral jumps of a narrow line as a result of a fluctuating environment. It is an important issue in spectroscopy, because the observed spectral broadening prevents access to the intrinsic line…

We first extend our recent experiments of correlation imaging through scattering media to the case of a thick medium, composed of two phase scatterers placed respectively in the image and the Fourier planes of the crystal. The spatial…

Quantum Physics · Physics 2020-05-05 Gnatiessoro Soro , Eric Lantz , Alexis Mosset , Fabrice Devaux

We have developed a simulation-based method of spectral analysis for pile-up affected data of X-ray CCDs without any loss of photon statistics. As effects of the photon pile-up appear as complicated nonlinear detector responses, we employ a…

Instrumentation and Methods for Astrophysics · Physics 2022-03-14 Tsubasa Tamba , Hirokazu Odaka , Aya Bamba , Hiroshi Murakami , Koji Mori , Kiyoshi Hayashida , Yukikatsu Terada , Tsunefumi Mizuno , Masayoshi Nobukawa

Recent technological advances allowed the coherent optical manipulation of high-energy electron wavepackets with attosecond precision. Here we theoretically investigate the collision of optically-modulated pulsed electron beams with atomic…

Atomic Physics · Physics 2021-04-21 Yuya Morimoto , Peter Hommelhoff , Lars Bojer Madsen

We experimentally demonstrate shaping of the two-photon wavefunction of entangled photon-pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the two-photon wavefunction exactly like a…

Quantum Physics · Physics 2011-12-06 Avi pe'er , Barak Dayan , Asher A. Friesem , Yaron Silberberg

A new experimental setup combining X-Ray Photon Correlation Spectroscopy (XPCS) in the hard x-ray regime and a high-pressure sample environment is developed to monitor the pressure dependence of the internal motion of complex systems down…

X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…

Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…

Optics · Physics 2017-01-24 Jonathan Tollerud , Jeffrey Davis

Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…

One of the problems often encountered in X-ray mirror manufacturing is setting proper manufacturing tolerances to guarantee an angular resolution - often expressed in terms of Point Spread Function (PSF) - as needed by the specific science…

Optics · Physics 2015-09-17 D. Spiga , L. Raimondi

We show that the combination of X-ray scattering with a nanofocused beam and X-ray cross correlation analysis is an efficient means for the full structural characterization of mesocrystalline nanoparticle assemblies with a single…

Speckle patterns manifesting from the interaction of coherent X-rays with matter offer a glimpse into the dynamics of nanoscale domains that underpin many emergent phenomena in quantum materials. While the dynamics of the average structure…