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Phase-mismatch in nonlinear optical processes can severely limit the propagation and conversion efficiency of light fields. Here, we present an efficient optimal-control strategy to mitigate the detrimental effects of phase-mismatch in an…

Quantum Physics · Physics 2025-09-17 Ning Jia , Hamid R. Hamedi , Jing Qian

The development of optical metamaterials has resulted in the demonstration of remarkable physical properties, including cloaking, optical magnetism, and negative refraction. The latter has attracted particular interest, mainly because of…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Hayk Harutyunyan , Ryan Beams , Lukas Novotny

Using a powerful homogenization technique, one- and two-dimensional graphene metasurfaces are homogenized both at the fundamental frequency (FF) and second harmonic (SH). In both cases, there is excellent agreement between the predictions…

Optics · Physics 2019-05-17 Qun Ren , J. W. You , N. C. Panoiu

Nonlinear metasurfaces offer new paradigm for boosting optical effect beyond limitations of conventional materials. In this work, we present an alternative way to produce pronounced third-harmonic generation (THG) based on nonlinear field…

A distant-neighbor quantum-mechanical method is used to study the nonlinear optical wave mixing in graphene nanoflakes (GNFs), including sum- and difference-frequency generation, as well as four-wave mixing. Our analysis shows that…

Optics · Physics 2022-03-11 Hanying Deng , Changming Huang , Yingji He , Fangwei Ye

It has recently been demonstrated that difference frequency mixing (DFM) can generate surface plasmons in graphene [1]. Here, we present detailed calculations comparing the contributions to this effect from substrate and from graphene…

We present the first experimental investigation of nonlinear optical properties of graphene flakes. We find that at near infrared frequencies a graphene monolayer exhibits a remarkably high third-order optical nonlinearity which is…

Materials Science · Physics 2011-01-13 E. Hendry , P. J. Hale , J. J. Moger , A. K. Savchenko , S. A. Mikhailov

Sub-wavelength graphene structures support localized plasmonic resonances in the terahertz and mid-infrared spectral regimes. The strong field confinement at the resonant frequency is predicted to significantly enhance the light-graphene…

A possibility to greatly enhance frequency-conversion efficiency of stimulated Raman scattering is shown by making use of extraordinary properties of three-wave mixing of ordinary and backward waves. Such processes are commonly attributed…

Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear…

Integrating graphene with plasmonic nanostructures results in multifunctional hybrid systems with enhanced performance for numerous applications. In this work, we take advantage of the remarkable mechanical properties of graphene to combine…

Graphene placed in a magnetic field possesses an extremely high mid/far-infrared optical nonlinearity originating from its unusual band structure and selection rules for the optical transitions near the Dirac point. Here we study the linear…

Mesoscale and Nanoscale Physics · Physics 2016-11-26 Xianghan Yao , Alexey Belyanin

Graphene has unique properties paving the way for groundbreaking future applications. Its large optical nonlinearity and ease of integration in devices notably makes it an ideal candidate to become a key component for all-optical switching…

Four-wave mixing (FWM) is an important nonlinear optical phenomenon that underlines many of the discoveries and device applications since the laser was invented. Examples include parametric amplification, mode-locked pulses and frequency…

Third harmonic generation of terahertz radiation is expected to occur in monolayer graphene due to the nonlinear relationship between the crystal momentum and the current density. In this work, we calculate the terahertz nonlinear response…

Applied Physics · Physics 2018-06-22 Parvin Navaeipour , Marc M. Dignam

Local electromagnetic field enhancement in resonant metamaterials is useful for efficient generation of nonlinear phenomena; however, the field enhancement is suppressed by losses of nonlinear elements in metamaterials. For overcoming this…

Optics · Physics 2018-11-15 Yasuhiro Tamayama , Takuya Yoshimura

The nonlinear optical response of materials to exciting light is enhanced by resonances between the incident laser frequencies and the energy levels of the excited material. Traditionally, in molecular nonlinear spectroscopy one tunes the…

Optics · Physics 2019-01-30 Yael Blechman , Euclides Almeida , Basudeb Sain , Yehiam Prior

Nonlinear optics, especially frequency mixing, underpins modern optical technology and scientific exploration in quantum optics, materials and life sciences, and optical communications. Since nonlinear effects are weak, efficient frequency…

We demonstrate enhanced four-wave mixing (FWM) in doped silica waveguides integrated with graphene oxide (GO) layers. Owing to strong mode overlap between the integrated waveguides and GO films that have a high Kerr nonlinearity and low…

Materials with massless Dirac fermions can possess exceptionally strong and widely tunable optical nonlinearities. Experiments on graphene monolayer have indeed found very large third-order nonlinear responses, but the reported variation of…