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Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…
The nonlinear properties of a metamaterial sample composed of double-layer metallic patterns and voltage controllable diodes are experimentally investigated. Second harmonics and spectrum modulations are clearly observed in a wide band of…
Integrating 2D materials onto on-chip photonic devices holds significant potential for nonlinear frequency conversion across various applications. The lack of inversion symmetry in monolayers of transition metal dichalcogenides (TMDs),…
We experimentally study the optical second harmonic generation (SHG) from deep subwavelength gold-silver heterodimer and silver-silver and gold-gold homodimers. Our results show that the SHG from the heterodimer is about an order of…
Modulation of metasurfaces in time gives rise to several exotic space-time scattering phenomena by violating the reciprocity and generation of higher-order frequency harmonics. We introduce a new design paradigm for time-modulated…
We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…
Directional harmonic generation is an important property characterizing the ability of nonlinear optical antennas to diffuse the signal in well-defined region of space. Herein, we show how sub-wavelength facets of an organic molecular…
We present a theoretical study of second-harmonic generation from a singular metasurface. The singular metasurfaces strongly interact with the incident light, where the large field enhancement forms an intense surface polarization that…
Optical second-harmonic generation (SHG) is studied for the confined geometry of a circular cylindrical waveguide or optical fiber. A model situation of high symmetry is considered where the material with nonlinear susceptibility is…
We demonstrate a nonlinear plasmonic metasurface that exhibits strongly asymmetric second-harmonic generation: nonlinear scattering is efficient upon excitation in one direction and it is substantially suppressed when the excitation…
Plasmonic nanocavities have proven to be a powerful optical platform for confining light at a length scale much smaller than the diffraction limit. Enhanced electromagnetic fields within the cavity mode volume enable multiple significant…
Plasmonic dimer antennas create strong field enhancement by squeezing light into a nanoscale gap. These optical hotspots are highly attractive for boosting nonlinear processes, such as harmonic generation, photoelectron emission, and…
A simple and flexible technique for achieving quasi-phase-matching in integrated photonic waveguides without periodic poling is proposed and experimentally demonstrated, referred to as mode-shape-modulation (MSM). It employs a periodic…
A quantum optical model for the high-order harmonic generation is presented, in which both the exciting field and the high harmonic modes are quantized, while the target material appears via parameters only. As a consequence, the model is…
We theoretically predict efficient optical second-harmonic generation (SHG) from a few hundred nanometer thick slab consisting of a quadratic nonlinear anisotropic medium whose linear principal permittivities are, at the fundamental…
High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…
In this work, we investigate the generation of second harmonic light by gold nanorods and demonstrate that the collected nonlinear intensity depends upon a phase interplay between different modes available in the nanostructure. By recording…
Second harmonic generation (SHG) microscopy is a valuable tool for optical microscopy. SHG microscopy is normally performed as a point scanning imaging method, which lacks phase information and is limited in spatial resolution by the…
Nonlinear frequency conversion plays a crucial role in advancing the functionality of next-generation optical systems. Portable metrology references and quantum networks will demand highly efficient second-order nonlinear devices, and the…
Silicon-based nonlinear metasurfaces were implemented only with third-order nonlinearity due to the crystal centrosymmetry and the efficiencies are considerably low, which hinders their practical applications with low-power lasers. Here, we…