Related papers: Optomechanical Collective Effects in Surface-Enhan…
The surface-enhanced Raman scattering (SERS) signal from an AgFON plasmonic substrate, recoated with benzenethiol, was observed to increase by about 100% upon heating for 3.5 min at 100C and 1.5 min at 125C. The signal intensity was found…
Stimulated Raman scattering (SRS) in plasma in the degenerate regime is studied theoretically and numerically. Different from normal SRS with the non-degenerate eigen electrostatic mode excited, the degenerate SRS is developed at plasma…
Based on our previous study [S. Wang $\textit{et al}$. J. Chem. Phys. $\textbf{153}$, 184102 (2020)], we generalize the theory of molecular emission power spectra (EPS) from one molecule to multichromophoric systems in the framework of…
We study the spontaneous emission from a regular lateral array or a randomly distributed ensemble of quantum dots under strong excitation (full inversion) conditions. We focus on the similarities and differences between the cases of random…
The random lasing (RL) emission of dyed vesicular polymeric films in diffusive regime of light propagation was investigated under helium temperature. It represents itself the coupling effect of stimulated emission and stimulated Raman…
We propose and demonstrate a novel technique that combines Raman scattering and optical cycling in molecules with diagonal Franck-Condon factors. This resonance Raman optical cycling manipulates molecules to behave like efficient…
Superradiance, the enhanced collective emission of energy from a coherent ensemble of quantum systems, has been typically studied in atomic ensembles. In this work we study theoretically the enhanced emission of energy from coherent…
In the context of the quantum-mechanical description of single-molecule surface-enhanced Raman scattering, intensity-field correlation measurements of photons emitted from a plasmonic cavity are explored, theoretically, using the technique…
We show that spontaneous Raman scattering of incident radiation can be observed in cavity-QED systems without external enhancement or coupling to any vibrational degree of freedom. Raman scattering processes can be evidenced as resonances…
The inelastic scatterings of matter systems, such as Raman scattering, contain rich information on mechanical vibrations like as resonant frequencies, which lead to various applications, for example, a sensor for specific molecules.…
Quantum entanglement offers an incredible resource for enhancing the sensing and spectroscopic probes. Here we develop a microscopic theory for the stimulated Raman scattering (SRS) using entangled photons. We demonstrate that the…
Molecular optomechanics stems from the description of Raman scattering in the presence of an optical resonator using a cavity optomechanics formalism. We extend the molecular optomechanics formalism to the case of hybrid…
The Sudden Approximation (SA) for scattering of atoms from surfaces is generalized to allow for double collision events and scattering from time-dependent quantum liquid surfaces. The resulting new schemes retain the simplicity of the…
Currently the extent of nanoplastic in the environment can only be estimated by extrapolation from the plastic waste that can be detected. To be able to quantify the whole extent of the problem, detection methods have to be developed that…
As a highly sensitive vibrational imaging method, stimulated Raman scattering (SRS) microscopy is finding various applications, while its theoretical treatment seems still under development. Here we present a theoretical estimation of…
Herein we report experimental evidence of directional SERS from molecules situated inside a single nanowire-nanoparticle junction cavity. The emission was confined to a narrow range of wavevectors perpendicular to the axis of the cavity. In…
Interaction between light and molecular vibrations leads to hybrid light-matter states called vibrational polaritons. Even though many intriguing phenomena have been predicted for single-molecule vibrational strong coupling (VSC), several…
We study coherent backscattering of a monochromatic laser by a dilute gas of cold two-level atoms in the weakly nonlinear regime. The nonlinear response of the atoms results in a modification of both the average field propagation (nonlinear…
We present a numerical study of the spatial coherence of light that is radiated from a dilute ensemble of atoms. The spatial coherence is established as a result of the collective (cooperative) coupling of the atoms to the light, and is…
We study the stationary photon output and statistics of small lasers. Our closed-form expressions clarify the contribution of collective effects due to the interaction between quantum emitters. We generalize laser rate equations and explain…