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Two-dimensional CrI3 has attracted much attention as it is reported to be a ferromagnetic semiconductor with the Curie temperature around 45K. By performing first-principles calculations, we find that the magnetic ground state of CrI3 is…

Computational Physics · Physics 2019-01-09 Zewen Wu , Jin Yu , Shengjun Yuan

It has been predicted theoretically and indirectly confirmed experimentally that single-layer CrX$_3$ (X=Cl, Br, I) might be the prototypes of topological magnetic insulators (TMI). In this work, by using first-principles calculations…

Materials Science · Physics 2020-10-07 Y. O. Kvashnin , A. Bergman , A. I. Lichtenstein , M. I. Katsnelson

We performed the detailed microscopic analysis of the inter-layer magnetic couplings for bilayer CrI$_3$. As the first step toward understanding the recent experimental observations and utilizing them for device applications, we estimated…

Materials Science · Physics 2019-04-10 Seung Woo Jang , Min Yong Jeong , Hongkee Yoon , Siheon Ryee , Myung Joon Han

Layered Ising metamagnets are antiferromagnetic (AF) materials consisting of monolayer Ising ferromagnets coupled to each other via interlayer AF interactions. They exhibit rich magnetic phase diagrams, featuring tricritical and critical…

Mesoscale and Nanoscale Physics · Physics 2026-01-29 Feng Liu , Jiayong Xiao , Shengwei Jiang , Kin Fai Mak , Jie Shan

CrI3 is a layered ferromagnetic insulator that has recently attracted enormous interest as it was the first example of a stand-alone monolayer ferromagnet, paving the way towards the study of two-dimensional magnetic materials and their use…

Resulting from strong magnetic anisotropy two-dimensional ferromagnetism was recently shown to be stabilized in chromium triiodide, CrI$_3$, in the monolayer limit. While its properties remain largely unexplored, it provides a unique…

Integrating monolayers derived from 2D van der Waals (vdW) magnetic materials into next-generation technological applications remains a significant challenge due to their structural and magnetic instability issues. Template-assisted…

Materials Science · Physics 2025-10-08 Ihsan Caha , Aqrab ul Ahmad , Francis Leonard Deepak

Noncollinear spin textures in low-dimensional magnetic systems have been studied for decades because of their extraordinary properties and promising applications derived from the chirality and topological nature. However, material…

Mesoscale and Nanoscale Physics · Physics 2020-09-29 Xiaobo Lu , Ruixiang Fei , Linghan Zhu , Li Yang

We apply the density-functional theory to study various phases (including non-magnetic (NM), anti-ferromagnetic (AFM), and ferromagnetic (FM)) in monolayer magnetic chromium triiodide (CrI$_3$), a recently fabricated 2D magnetic material.…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Lucas Webster , Liangbo Liang , Jia-An Yan

Long-range magnetic orders in atomically thin ferromagnetic CrI3 give rise to new fascinating physics and application perspectives. The physical properties of two-dimensional (2D) ferromagnetism CrI3 are significantly influenced by…

Materials Science · Physics 2019-11-13 Kai Guo , Bowen Deng , Zhongtai Shi , Yue Li , Xin Wang , Lei Bi , Li Zhang , Haipeng Lu , Peiheng Zhou , Linbo Zhang , Yingchun Cheng , Bo Peng

The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman…

Two-dimensional (2D) ferromagnets with high Curie temperature have long been the pursuit for electronic and spintronic applications. CrI3 is a rising star of intrinsic 2D ferromagnets, however, it suffers from weak exchange coupling. Here…

Materials Science · Physics 2020-09-22 Yu Guo , Nanshu Liu , Yanyan Zhao , Xue Jiang , Si Zhou , Jijun Zhao

We have studied intrinsic defect complexes in In$_2$O$_3$ using ab initio random structure searching (AIRSS). Our first-principles density-functional-theory calculations predict the thermodynamic stability of several novel defect…

Materials Science · Physics 2016-09-16 Jamie M. Wynn , Richard J. Needs , Andrew J. Morris

Moir\'e magnetism featured by stacking engineered atomic registry and lattice interactions has recently emerged as an appealing quantum state of matter at the forefront condensed matter physics research. Nanoscale imaging of moir\'e magnets…

We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

After the discovery of magnetism in monolayer CrI3, the magnetic properties of different 2D materials from the chromium-trihalide family are intuitively assumed to be similar, yielding magnetic anisotropy from the spin-orbit coupling on…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 C. Bacaksiz , D. Šabani , R. M. Menezes , M. V. Milošević

The exploration of magnetism in two-dimensional layered materials has attracted extensive research interest. For the monoclinic phase CrI3 with interlayer antiferromagnetism, finding a static and robust way of realizing the intrinsic…

Materials Science · Physics 2022-11-30 Shiyang Sun , Xuyan Chen , Xuqi Li , Huihui Zhang , Haidan Sang , Shifei Qi , Zhenhua Qiao

We study the Raman spectrum of CrI$_3$, a material that exhibits magnetism in a single-layer. We employ first-principles calculations within density functional theory to determine the effects of polarization, strain, and incident angle on…

Materials Science · Physics 2018-08-08 Daniel T. Larson , Efthimios Kaxiras

Chromium triiodide is an intrinsically magnetic van der Waals material down to the single-layer limit. Here, we provide a first-principles description of finite-temperature magnetic and spectral properties of monolayer (ML) CrI$_3$ based on…

Strongly Correlated Electrons · Physics 2022-05-24 Yaroslav O. Kvashnin , Alexander N. Rudenko , Patrik Thunström , Malte Rösner , Mikhail I. Katsnelson

We present a detailed study on the microscopic origin of magnetism in suspended and dielectrically embedded CrI$_3$ monolayer. To this end, we down-fold two distinct minimal generalized Hubbard models with different orbital basis sets from…

Strongly Correlated Electrons · Physics 2021-10-06 D. Soriano , A. N. Rudenko , M. I. Katsnelson , M. Rösner