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Unconventional emissions from exciton and trion in monolayer WS2 are studied by photoexcitation. Excited by 532nm laser beam, the carrier species in the monolayer WS2 are affected by the excess electrons escaping from photoionization of…

Mesoscale and Nanoscale Physics · Physics 2016-08-08 Ke Wei , Yu Liu , Hang Yang , Xiangai Cheng , Tian Jiang

We report a rare atom-like interaction between excitons in monolayer WS2, measured using ultrafast absorption spectroscopy. At increasing excitation density, the exciton resonance energy exhibits a pronounced redshift followed by an…

The potential for low-threshold optical nonlinearity has received significant attention in the fields of photonics and conceptual optical neuron networks. Excitons in two-dimensional (2D) semiconductors are particularly promising in this…

We have observed a large spin splitting between "spin" $+1$ and $-1$ heavy-hole excitons, having unbalanced populations, in undoped GaAs/AlAs quantum wells in the absence of any external magnetic field. Time-resolved photoluminescence…

Condensed Matter · Physics 2016-08-31 L. Vina , L. Munoz , E. Perez , J. Fernandez-Rossier , C. Tejedor , K. Ploog

Monolayer transition metal dichalcogenides (TMDs) with strong spin-orbit coupling combined with broken inversion symmetry, leading to a coupling of spin and valley degrees of freedom, make these materials highly interesting for potential…

Mesoscale and Nanoscale Physics · Physics 2020-09-23 Liang Xilong , Qin Chengbing , Gao Yan , Han Shuangping , Zhang Guofeng , Chen Ruiyun , Hu Jianyong , Xiao Liantuan , Jia Suotang

We develop a theory to calculate exciton binding energies of both two- and three-dimensional spin polarized exciton gases within a mean field approach. Our method allows the analysis of recent experiments showing the importance of the…

Condensed Matter · Physics 2019-08-15 J. Fernández-Rossier , C. Tejedor , L. Muñoz , L. Viña

We use femtosecond pump-probe spectroscopy to study the coherent interaction of excited exciton states in WSe2 and MoSe2 monolayers via the optical Stark effect. For co-circularly polarized pump and probe, we measure a blueshift which…

Mesoscale and Nanoscale Physics · Physics 2025-06-09 Max Wegerhoff , Moritz Scharfstädt , Stefan Linden , Andrea Bergschneider

Coupling between exciton states across the Brillouin zone in monolayer transition metal dichalcogenides can lead to ultrafast valley depolarization. Using time- and angle-resolved photoemission, we present momentum- and energy-resolved…

Excitons, Coulomb bound electron-hole pairs, are composite bosons and their interactions in traditional semiconductors lead to condensation and light amplification. The much stronger Coulomb interaction in transition metal dichalcogenides…

Mesoscale and Nanoscale Physics · Physics 2017-04-05 M. Manca , M. M. Glazov , C. Robert , F. Cadiz , T. Taniguchi , K. Watanabe , E. Courtade , T. Amand , P. Renucci , X. Marie , G. Wang , B. Urbaszek

In heterostructures consisting of different transition-metal dichalcogenide monolayers, a staggered band alignment can occur, leading to rapid charge separation of optically generated electron-hole pairs into opposite monolayers. These…

We report circularly-polarized optical reflection spectroscopy of monolayer WS$_2$ and MoS$_2$ at low temperatures (4~K) and in high magnetic fields to 65~T. Both the A and the B exciton transitions exhibit a clear and very similar Zeeman…

Mesoscale and Nanoscale Physics · Physics 2016-02-11 Andreas V. Stier , Kathleen M. McCreary , Berend T. Jonker , Junichiro Kono , Scott A. Crooker

We study the neutral exciton energy spectrum fine structure and its spin dephasing in transition metal dichalcogenides such as MoS$_2$. The interaction of the mechanical exciton with its macroscopic longitudinal electric field is taken into…

Mesoscale and Nanoscale Physics · Physics 2014-05-15 M. M. Glazov , T. Amand , X. Marie , D. Lagarde , L. Bouet , B. Urbaszek

We investigate the two-pulse photon echo response of excitons in the mixed lead halide perovskite crystal \sample in dependence on the excitation intensity and polarization of the incident laser pulses. Using spectrally narrow picosecond…

Coulomb bound electron-hole pairs, excitons, govern the optical properties of semi-conducting transition metal dichalcogenides like MoS$_2$ and WSe$_2$. We study optical transitions at the K-point for 2H homobilayer MoS$_2$ in Density…

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

We report magneto-optical spectroscopy of gated monolayer MoS$_2$ in high magnetic fields up to 28T and obtain new insights on the many-body interaction of neutral and charged excitons with the resident charges of distinct spin and valley…

The valley degree of freedom is a sought-after quantum number in monolayer transition-metal dichalcogenides. Similar to optical spin orientation in semiconductors, the helicity of absorbed photons can be relayed to the valley (pseudospin)…

Mesoscale and Nanoscale Physics · Physics 2020-04-01 Min Yang , Cedric Robert , Zhengguang Lu , Dinh Van Tuan , Dmitry Smirnov , Xavier Marie , Hanan Dery

Understanding exciton thermalization is critical for optimizing optoelectronic and photocatalytic processes in many materials. However, it is hard to access the dynamics of such processes experimentally, especially on systems such as…

We investigate the magnetic-field-induced splitting of biexcitons in monolayer WS$_2$ using polarization-resolved photoluminescence spectroscopy in out-of-plane magnetic fields up to 30 T. The observed $g$ factor of the biexciton amounts to…

We have experimentally studied the pump-probe Kerr rotation dynamics in WSe$_2$ monolayers. This yields a direct measurement of the exciton valley depolarization time $\tau_v$. At T=4K, we find $\tau_v\approx 6$ps, a fast relaxation time…

Mesoscale and Nanoscale Physics · Physics 2014-10-10 C. R. Zhu , K. Zhang , M. Glazov , B. Urbaszek , T. Amand , Z. W. Ji , B. L. Liu , X. Marie
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