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We study the phase behaviour of cholesteric liquid crystal shells with different geometries. We compare the cases of tangential and no anchoring at the surface, focussing on the former case, which leads to a competition between the…

Soft Condensed Matter · Physics 2023-03-01 Giuseppe Negro , Livio Nicola Carenza , Giuseppe Gonnella , Davide Marenduzzo , Enzo Orlandini

We study how dispersions of colloidal particles in a cholesteric liquid crystal behave under a time-dependent electric field. By controlling the amplitude and shape of the applied field wave, we show that the system can be reproducibly…

Soft Condensed Matter · Physics 2015-05-05 Giuseppe D'Adamo , D. Marenduzzo , C. Micheletti , E. Orlandini

We demonstrate a novel route of spatially organizing the colloid arrangements on the polymer-grafted substrate by use of self-consistent field and density functional theories. We find that grafting of polymers onto a substrate can…

Soft Condensed Matter · Physics 2007-05-23 Kang Chen , Yu-qiang Ma

Hypothesis: Colloidal molecules with anisotropic shapes and interactions are powerful model systems for deciphering the behavior of real molecules and building units for creating materials with designed properties. While many strategies for…

Soft Condensed Matter · Physics 2022-07-19 Yogesh Shelke , Susana Marín-Aguilar , Fabrizio Camerin , Marjolein Dijkstra , Daniela J. Kraft

Active elastomeric liquid crystal particles with initial cylindrical shapes are obtained by means of soft lithography and polymerization in a strong magnetic field. Gold nanocrystals infiltrated into these particles mediate energy transfer…

The geometric shape, symmetry, and topology of colloidal particles often allow for controlling colloidal phase behavior and physical properties of these soft matter systems. In liquid crystalline dispersions, colloidal particles with low…

Soft Condensed Matter · Physics 2024-10-14 Ye Yuan , Ivan I. Smalyukh

Complex colloidal cluster morphologies are desirable for the fabrication of advanced materials, such as photonic crystals and meta-materials, and can be formed through evaporation-driven packing. By coupling lattice Boltzmann and discrete…

Soft Condensed Matter · Physics 2026-05-07 Junyu Yang , Abhinav Naga , Xitong Zhang , Halim Kusumaatmaja

We study colloidal particles in a nematic-liquid-crystal-filled microfluidic channel and show how elastic interactions between the particle and the channel wall lead to different particle dynamics compared with conventional microfluidics.…

Soft Condensed Matter · Physics 2017-07-31 Sourav Mondal , Apala Majumdar , Ian M. Griffiths

We study the rheological properties of colloidal microphases in two dimensions simulating a model of colloidal particles with competing interactions. Due to the competition between short-range attraction and long-range repulsion, as a…

Soft Condensed Matter · Physics 2009-11-13 A. Imperio , L. Reatto , S. Zapperi

We perform numerical simulations to study self-assembly of nanoparticles mediated by an elastic planar surface. We show how the nontrivial elastic response to deformations of these surfaces leads to anisotropic interactions between the…

Soft Condensed Matter · Physics 2012-01-04 Andela Šarić , Angelo Cacciuto

Predicting the macroscopic chiral behaviour of cholesteric liquid crystals from the microscopic chirality of the particles is highly non-trivial, even when the chiral interactions are purely entropic in nature. Here we introduce a novel…

Soft Condensed Matter · Physics 2016-04-27 Simone Dussi , Marjolein Dijkstra

We simulate colloids (radius $R \sim 1\mu$m) trapped at the interface between a cholesteric liquid crystal and an immiscible oil, at which the helical order (pitch p) in the bulk conflicts with the orientation induced at the interface,…

Soft Condensed Matter · Physics 2013-11-11 J. S. Lintuvuori , A. C. Pawsey , K. Stratford , M. E. Cates , P. S. Clegg , D. Marenduzzo

We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with a uniform far-field alignment in a liquid crystal host. Displacing energetically…

The design of complex materials and the formation of specific patterns often arise from the properties of the individual building blocks. In this respect, colloidal systems offer a unique opportunity because nowadays they can be synthesized…

Soft Condensed Matter · Physics 2022-03-01 Fabrizio Camerin , Emanuela Zaccarelli

We present a novel, self-consistent and robust theoretical model to investigate elastic interactions between topological defects in liquid crystal shells. Accounting for the non-concentric nature of the shell in a simple manner, we are able…

Soft Condensed Matter · Physics 2016-12-14 Alexandre Darmon , Olivier Dauchot , Teresa Lopez-Leon , Michael Benzaquen

The physical mechanism of elasticity of liquid surfaces coated with colloidal particles is proposed. It is suggested that particles are separated by water clearings and the capillary interaction between them is negligible. The case is…

Soft Condensed Matter · Physics 2015-03-12 Edward Bormashenko , Gene Whyman , Oleg Gendelman

Using laser tweezers and fluorescence confocal polarizing microscopy, we study colloidal interactions of solid microspheres in the nematic bulk caused by elastic distortions around the particles with strong tangential surface anchoring. The…

Soft Condensed Matter · Physics 2009-11-11 I. I. Smalyukh , O. D. Lavrentovich , A. N. Kuzmin , A. V. Kachynski , P. N. Prasad

Identifying and removing microplastics (MPs) from the environment is a global challenge. This study explores how the colloidal fraction of common MPs behave at aqueous interfaces of liquid crystal (LC) films. We observed polyethylene (PE)…

Soft Condensed Matter · Physics 2022-10-06 Fiona Mukherjee , Anye Shi , Xin Wang , Fengqi You , Nicholas L. Abbott

Cholesteric liquid crystals (CLCs) have a characteristic length scale given by the pitch of the twisted stacking of their constituent rod-like molecules. Under homeotropic anchoring conditions where the molecules prefer to orient…

Soft Condensed Matter · Physics 2020-05-13 Maxim O. Lavrentovich , Lisa Tran

When a drop containing colloidal particles evaporates on a surface, a circular stain made of these particles is often observed due to an internal flow toward the contact line. To hinder this effect, several approaches have been proposed…

Soft Condensed Matter · Physics 2016-01-06 François Boulogne , François Ingremeau , Julien Dervaux , Laurent Limat , Howard A. Stone