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We have performed a density functional theory study of the possible layered geometries occurring after dehydrogenation of a self-assembled monolayer (SAM) of biphenyl-thiol molecules (BPTs) adsorbed on a Au(111), as it has been…

Mesoscale and Nanoscale Physics · Physics 2011-11-10 Pepa Cabrera-Sanfelix , Andrés Arnau , Daniel Sánchez-Portal

For the first time, we report the formation of pentagonal atomic chains during tensile deformation of ultra thin BCC Fe nanowires. Extensive molecular dynamics simulations have been performed on $<$100$>$/{110} BCC Fe nanowires with…

Mesoscale and Nanoscale Physics · Physics 2016-12-20 G. Sainath , B. K. Choudhary

We used DFT to study the energetics of the decomposition of alane, AlH3, on the Si(001) surface, as the acceptor complement to PH3. Alane forms a dative bond with the raised atoms of silicon surface dimers, via the Si atom lone pair. We…

Materials Science · Physics 2017-09-13 Richard L. Smith , David R. Bowler

We investigate the thermal conductivity of plumbene using molecular dynamics simulations, overcoming existing limitations by optimizing the parameters of Tersoff and Stillinger-Weber potentials via artificial neural networks. Our findings…

Materials Science · Physics 2023-11-20 Rafat Mohammadi , Behrad Karimi , John Kieffer , Daniel Hashemi

The intermetallic compound Zr3Al is severely deformed by the method of repeated cold rolling. By X-ray diffraction it is shown that this leads to amorphization. TEM investigations reveal that a homogeneously distributed debris of very small…

An ideal one-dimensional electronic system is formed along atomic chains on Au-decorated vicinal silicon surfaces but the nature of its low temperature phases has been puzzled for last two decades. Here, we unambiguously identify the low…

Materials Science · Physics 2022-05-09 Euihwan Do , Jae Whan Park , Oleksandr Stetsovych , Pavel Jelinek , Han Woong Yeom

A single-crystal sheet of graphene is synthesized on the low-symmetry substrate Ir(110) by thermal decomposition of C$_2$H$_4$ at 1500 K. Using scanning tunneling microscopy, low-energy electron diffraction, angle-resolved photoemission…

The controlled growth of organic layer on surface is still awaiting for an on-line reliable monitoring that would allow improvement of its quality. We show here that the self-assembly of the perylene monolayer deposited on Ag(110) at room…

Atomic Physics · Physics 2016-02-17 Nataliya Kalashnyk , Philippe Roncin

Accurate atomic coordinates of the room-temperature (root3xroot3)R30degree and low-temperature (3x3) phases of 1/3 ML Sn on Ge(111) have been established by grazing-incidence x-ray diffraction with synchrotron radiation. The Sn atoms are…

Materials Science · Physics 2009-10-31 O. Bunk , J. H. Zeysing , G. Falkenberg , R. L. Johnson , M. Nielsen , M. M. Nielsen , R. Feidenhans'l

Methylated polycyclic aromatic hydrocarbons (PAHs) have been hypothesised to be present in the interstellar medium (ISM) through their 3.4 and 6.9 $\mu$m absorption bands. To investigate the hydrogenation of these methylated PAHs, the…

Astrophysics of Galaxies · Physics 2026-02-11 A. T. Hopkinson , F. G. Doktor , J. Pitfield , M. Moll , J. D. Thrower , L. Hornekær

Extensive density-functional calculations are performed to understand atomic chemisorption on the TiC(111) and TiN(111) surfaces, in particular the calculated pyramid-shaped trends in the adsorption energies for second- and third-period…

Materials Science · Physics 2009-11-11 Carlo Ruberto , Aleksandra Vojvodic , Bengt I. Lundqvist

The potential of graphene for hydrogen storage, coupled with the established role of Platinum as a catalyst for the hydrogen evolution reaction and the spillover effect, makes Pt-functionalized graphene a promising candidate for…

Recent progress in the synthesis and processing of nano-structured materials and systems calls for an improved understanding of thermal properties on small length scales. In this context, the question whether thermodynamics and, in…

Materials Science · Physics 2007-05-23 M. Hartmann , G. Mahler , O. Hess

The structure of 1,3,5_triphenylbenzene C6H3(C6H5)3 at 473 K was investigated using the X-ray diffraction method. The measurements of scattered radiation intensity were performed in a wide range of wave vector. For the first time the…

Chemical Physics · Physics 2019-08-07 Henryk Drozdowski , Malgorzata Sliwinska-Bartkowiak

We report an extensive study of the properties of carbyne using first-principles calculations. We investigate carbyne's mechanical response to tension, bending, and torsion deformations. Under tension, carbyne is about twice as stiff as the…

Materials Science · Physics 2013-12-03 Mingjie Liu , Vasilii I. Artyukhov , Hoonkyung Lee , Fangbo Xu , Boris I. Yakobson

Using helium-3 atom scattering, we have studied the adsorption kinetics, the structure and the diffusional dynamics of atomic hydrogen on the surface of a graphene monolayer on Ni(111). Diffraction measurements reveal a 4$^\circ$ rotated…

Mesoscale and Nanoscale Physics · Physics 2022-12-15 Emanuel Bahn , Anton Tamtögl , John Ellis , William Allison , Peter Fouquet

Due to their ability to reversibly absorb/desorb hydrogen without hysteresis, Pd--Au nanoalloys have been proposed as materials for hydrogen sensing. For sensing, it is important that absorption/desorption isotherms are reproducible and…

Materials Science · Physics 2021-08-17 J. Magnus Rahm , Joakim Löfgren , Erik Fransson , Paul Erhart

The zig-zag Nitrogen (N) chain similar to the Ch-N structure has long been considered a potential high energy density structure. However, all previously predicted zig-zag N chain structures similar to Ch-N exhibit imaginary frequencies in…

Materials Science · Physics 2025-02-28 Chengfeng zhang , Guo Chen , Yanfeng Zhang , Jie Zhang , Xianlong Wang

The method for production of atomic chains by heating of graphene nanoribbons (GNRs) is proposed and studied by molecular dynamics simulations. The Brenner potential is revised to adequately describe formation of atomic chains, edges and…

Mesoscale and Nanoscale Physics · Physics 2018-10-09 Alexander S. Sinitsa , Irina V. Lebedeva , Andrey M. Popov , Andrey A. Knizhnik

We use a version of the density functional theory to study the changes in the height of the tethered layer of chains built of jointed spherical segments with the change of the length and surface density of chains. For the model in which the…

Soft Condensed Matter · Physics 2012-02-21 M. Borówko , A. Patrykiejew , O. Pizio , S. Sokołowski