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In this paper, we present a unified computational method based on pseudospectral approximations for the design of optimal pulse sequences in open quantum systems. The proposed method transforms the problem of optimal pulse design, which is…

Chemical Physics · Physics 2009-08-17 Jr-Shin Li , Justin Ruths , Dionisis Stefanatos

Conventional approaches for controlling open quantum systems use coherent control which affects the system's evolution through the Hamiltonian part of the dynamics. Such control, although being extremely efficient for a large variety of…

Quantum Physics · Physics 2009-05-04 Alexander Pechen , Herschel Rabitz

For the model Hamiltonian describing the electron-nuclear dynamics of a quantum dot, we obtained an exact expression for the limiting nuclear polarization as a function of the number of groups of equivalent nuclei. It is shown that the…

Mesoscale and Nanoscale Physics · Physics 2008-01-10 G. G. Kozlov

Optimal quantum control of continuous variable systems poses a formidable computational challenge because of the high-dimensional character of the system dynamics. The framework of quantum invariants can significantly reduce the complexity…

A New theoretical formalism for the optimal quantum control has been presented. The approach stems from the consideration of describing the time-dependent quantum system in terms of the real physical observables, viz., the probability…

Chemical Physics · Physics 2015-06-26 Bijoy K. Dey

The angular momentum of molecules, or, equivalently, their rotation in three-dimensional space, is ideally suited for quantum control. Molecular angular momentum is naturally quantized, time evolution is governed by a well-known Hamiltonian…

Quantum Physics · Physics 2019-10-23 Christiane P. Koch , Mikhail Lemeshko , Dominique Sugny

Previous studies have used numerical methods to optimize the hyperpolarizability of a one-dimensional quantum system. These studies were used to suggest properties of one-dimensional organic molecules, such as the degree of modulation of…

Optics · Physics 2015-05-18 Urszula B. Szafruga , Mark G. Kuzyk , David S. Watkins

A precise time-dependent control of a quantum system relies on an accurate account of the quantum interference among the system, the control and the environment. A diagrammatic technique has been recently developed to precisely calculate…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Ching-Kit Chan , L. J. Sham

This article provides a review of recent developments in the formulation and execution of optimal control strategies for the dynamics of quantum systems. A brief introduction to the concept of optimal control, the dynamics of of open…

Quantum Physics · Physics 2009-10-06 Robert Roloff , Markus Wenin , Walter Pötz

We study quantum information processing by means of optimal control theory. To this end, we analyze the damped Jaynes-Cummings model, and derive optimal control protocols that minimize the heating or energy dispersion rates, and controls…

Quantum Physics · Physics 2014-07-14 Sebastian Deffner

Quantum computation is based on implementing selected unitary transformations which represent algorithms. A generalized optimal control theory is used to find the driving field that generates a prespecified unitary transformation. The…

Quantum Physics · Physics 2009-11-07 Jose P. Palao , Ronnie Kosloff

We present an efficient strategy for controlling a vast range of non-integrable quantum many body one-dimensional systems that can be merged with state-of-the-art tensor network simulation methods like the density Matrix Renormalization…

Quantum Physics · Physics 2015-03-13 Patrick Doria , Tommaso Calarco , Simone Montangero

Classical polarizable approaches have become the gold standard for simulating complex systems and processes in the condensed phase. These methods describe intrinsically dissipative polarizable media, requiring a formal definition within the…

In this dissertation I analyze Hamiltonian control of $d$-dimensional quantum systems as realized in alkali atomic spins. Alkali atoms provide an ideal platform for studies of quantum control due to the extreme precision with which the…

Quantum Physics · Physics 2009-06-29 Seth Merkel

A critical engineering challenge in quantum technology is the accurate control of quantum dynamics. Model-based methods for optimal control have been shown to be highly effective when theory and experiment closely match. Consequently,…

Quantum Physics · Physics 2022-10-19 Andy J. Goldschmidt , Jonathan L. DuBois , Steven L. Brunton , J. Nathan Kutz

The dynamics of a quantum system driven by an external field is well described by a unitary transformation generated by a time dependent Hamiltonian. The inverse problem of finding the field that generates a specific unitary transformation…

Quantum Physics · Physics 2009-11-10 Jose P. Palao , R. Kosloff

Achieving high-fidelity control of quantum systems is of fundamental importance in physics, chemistry and quantum information sciences. However, the successful implementation of a high-fidelity quantum control scheme also requires…

Quantum Physics · Physics 2018-06-05 Yu Guo , Daoyi Dong , Chuan-Cun Shu

We present a general method to efficiently design optimal control sequences for non-Markovian open quantum systems, and illustrate it by optimizing the shape of a laser pulse to prepare a quantum dot in a specific state. The optimization of…

Quantum Physics · Physics 2023-07-11 Gerald E. Fux , Eoin P. Butler , Paul R. Eastham , Brendon W. Lovett , Jonathan Keeling

Quantum discrimination and estimation are pivotal for many quantum technologies, and their performance depends on the optimal choice of probe state and measurement. Here we show that their performance can be further improved by suitably…

Quantum Physics · Physics 2020-09-14 Daniel Basilewitsch , Haidong Yuan , Christiane P. Koch

We investigate optimal control strategies for state to state transitions in a model of a quantum dot molecule containing two active strongly interacting electrons. The Schrodinger equation is solved nonperturbatively in conjunction with…

Quantum Physics · Physics 2016-08-14 R. Nepstad , L. Sælen , I. Degani , J. P. Hansen