Related papers: Interpreting fluorescence detected 2D electronic s…
Recent interest in the role of quantum mechanics in the primary events of photosynthetic energy transfer has led to a convergence of nonlinear optical spectroscopy and quantum optics on the topic of energy-transfer dynamics in…
Two-dimensional (2D) fluorescence-excitation (2D-FLEX) spectroscopy is a recently proposed nonlinear femtosecond technique for the detection of photoinduced dynamics. The method records a time-resolved fluorescence signal in its excitation-…
We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…
Identifying signatures of quantum coherent behaviour in photoactive systems that are maintained in stationary states away from thermal equilibrium is an open problem of wide interest in a variety of physical scenarios, including single…
Vibrational coherences in ultrafast pump-probe (PP) and 2D electronic spectroscopy (2DES) provide insight into the excited state dynamics of molecules. Femtosecond coherence spectra (FCS) and 2D beat maps yield information about…
Experimental conclusions from air shower observations on cosmic-ray photons above 10^19 eV are based on the comparison to detailed shower simulations. For the calculations, the photonuclear cross-section needs to be extrapolated over…
We analyze the operation of a quantum tunneling detector coupled to a coherent conductor. We demonstrate that in a certain energy range the output of the detector is determined by two-photon processes, two-electron processes and the…
While calculations and measurements of single-particle spectral properties often offer the most direct route to study correlated electron systems, the underlying physics may remain quite elusive, if information at higher particle levels is…
It has recently been proposed, with the help of numerical investigations, that fluorescence correlation spectroscopy at variable observation area can reveal the existence of a meshgrid of semi-permeable barriers hindering the…
The brief review of modern theoretical models describing the process of the photon absorption by nucleons at superhigh energies of real photons is given. The main aim of the work is an estimation of the theoretical uncertainty of the cross…
We present a widefield two-dimensional electronic spectroscopy microscope (2DESM) that integrates multidimensional coherent spectroscopy with optical imaging, enabling femtosecond temporal and micrometer spatial resolution. The broadband…
Important analyses at a future linear collider, including top-quark and W-boson mass measurements will depend upon the precise determination of the luminosity spectrum. This can be done, in principle,in the planned detectors. We review the…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
Resonance fluorescence of a two-level emitter displays persistently anti-bunching irrespective of the excitation intensity, but inherits the driving laser's linewidth under weak monochromatic excitation. These properties are commonly…
Hyperspectroscopy is a new method of surface image taking, providing simultaneously high position and spectral resolutions which allow one to make some conclusions about chemical compositions of the surfaces. We are now studying…
I sketch some pressing questions in several active areas of particle physics and outline the challenges they present for the design and operation of detectors.
We study a system of two interacting, non-indentical quantum emitters driven by a coherent field. We focus on the particular condition of two-photon resonance and obtain analytical expressions for the stationary density matrix of the system…
In this paper the coherence and crossing symmetry of the electromagnetic interaction of photons involved in the spontaneous parametric down conversion (SPDC) phenomena in nonlinear crystals, are investigated. On this basis a new…
We investigate light scattering under nanofocusing in the context of coherent spectroscopy. We discuss the different mechanisms that may enhance the signal in extinction and how these depend on nanofocusing as well as on the probed system.…
Double-quantum two-dimensional coherent spectroscopy (MDCS) is a powerful optical method that is used to study optical properties of atomic and complex molecular systems and semiconductor materials. Double-quantum 2D spectra and…