Related papers: Theory of EELS in atomically thin metallic films
Since holography yields exact results, even in situations where perturbation theory is not applicable, it is an ideal framework for modeling strongly correlated systems. We extend previous holographic methods to take the dynamical charge…
A mathematical model is developed to analyze the growth/decay rate of surface perturbations of an ultrathin metal film on an amorphous substrate (SiO_{2}). The formulation combines the approach of Mullins [J. Appl. Phys. v30, 77, 1959] for…
Electron beam imaging is a common technique used for characterizing the morphology of plasmonic nanostructures. During the imaging process, the electron beam interacts with traces of organic material in the chamber and produces a well-know…
In plasmonics, nonlocal effects arise when the material response to optical excitations is strongly dependent on the spatial correlations of the excitation. It is well known that a classical free electron gas system supports local Drude…
The implementation of ultrasoft pseudopotentials into time-dependent density-functional perturbation theory is detailed for both the Sternheimer approach and the Liouville-Lanczos (LL) method, and equations are presented in the scalar…
The structural evolution of laser-excited systems of gold has previously been measured through ultrafast MeV electron diffraction. However, there has been a long-standing inability of atomistic simulations to provide a consistent picture of…
A theory for the collective plasma excitations in a linear periodic array of spherical two-dimensional electron gases (S2DEGs) is presented. This is a simple model for an ultra thin and narrow microribbon of fullerenes or metallic shells.…
We report the observation of plasma oscillations in an ultracold neutral plasma. With this collective mode we probe the electron density distribution and study the expansion of the plasma as a function of time. For classical plasma…
We have used symmetric normal metal-insulator-superconductor (NIS) tunnel junction pairs, known as SINIS structures, for ultrasensitive thermometry in the temperature range 50 - 700 mK. By Joule heating the electron gas and measuring the…
We use momentum-dependent electron energy-loss spectroscopy in transmission to study collective charge excitations in the layer metal Sr$_2$RuO$_4$. This metal has a transition from a perfect Fermi liquid below $T\approx30\,$K into a…
The theory of surface electromagnetic waves (SEMWs) propagating at optical frequencies along the interface of an isotropic noble metal [e.g., gold (Au)] and a uniaxial crystal [e.g., Rutile (TiO$_2$)] is revisited with the Drude-Lorentz…
Electron energy-loss spectroscopy (EELS) is a powerful tool for imaging chemical variations at the nanoscale. Here, we investigate a polymer/organic small molecule-blend used as absorber layer in an organic solar cell and employ EELS for…
The recent surface plasmon entanglement experiment [E. Altewischer et al., Nature (London) 418, 304 (2002)] is theoretically analyzed. The entanglement preservation upon transmission in the non-focused case is found to provide information…
It has been argued in a recent paper by R. Joynt (R. Joynt, Science 284, p 777 (1999)) that in the case of poorly conducting solids the photoemission spectrum close to the Fermi Energy may be strongly influenced by extrinsic loss processes…
In three dimensional (3D) disordered metals, the electron-phonon (\emph{e}-ph) scattering is the sole significant inelastic process. Thus the theoretical predication concerning the electron-electron (\emph{e}-\emph{e}) scattering rate…
We present a derivation of the dispersion relation for electrostatic oscillations (ESOs) in a zero temperature quantum plasma. In the latter, degenerate electrons are governed by the Wigner equation, while non-degenerate ions follow the…
We present a new theory for partitioning simulations of periodic and solid-state systems into physically sound atomic contributions at the level of Kohn-Sham density functional theory. Our theory is based on spatially localized linear…
Simulation results are presented to demonstrate electron temperature and electrical potential development in dilute and cold plasma development. The simulation method is a hybrid method which adopted fluid model for electrons due to their…
We observe using ab initio methods that localized surface plasmon resonances in icosahedral silver nanoparticles enter the asymptotic region already between diameters of 1 and 2 nm, converging close to the classical quasistatic limit around…
An interaction of electromagnetic S-wave with thin flat metallic film is numerically studied for the quantum degenerate electron plasma. One considers the reflectance, transmittance and absorptance power coefficients. A contribution of…