Related papers: Prospects for laser cooling of polyatomic molecule…
We propose a coherent optical population transfer of weakly bound field-linked (FL) tetratomic molecules (tetramers) to deeper FL bound states using stimulated Raman adiabatic passage. We consider static-electric-field shielded polar…
The development of the magneto-optical trap revolutionized the fields of atomic and quantum physics by providing a simple method for the rapid production of ultracold, trapped atoms. A similar technique for producing a diverse set of dense,…
Doppler cooling is a widely used technique to laser cool atoms and nanoparticles exploiting the Doppler shift involved in translational transformations. The rotational Doppler effect arising from rotational coordinate transformations should…
We find that transparent conducting oxides (TCOs) exhibit oscillatory (sign-reversing) dynamics on a few optical cycle timescale under extreme electron temperatures. We demonstrate a mechanism for such transient dynamics and present an…
Hybrid structures formed between organic molecules and inorganic quantum dots can accomplish unique photophysical transformations by taking advantage of their disparate properties. The electronic coupling between these materials is…
The interaction of strong laser fields with matter intrinsically provides powerful tools to image transient dynamics with an extremely high spatiotemporal resolution. Here, we study strong-field ionisation of laser-aligned molecules and…
Functionalized adamantane molecular cluster materials show highly transient nonlinear optical properties of currently unclear structural origin. Several interaction mechanisms in compounds comprising molecular clusters, their inter- and…
For laser cooling considerations, we have theoretically investigated the electronic, rovibrational and hypefine structures of BaF molecule. The highly diagonal Franck-Condon factors and the branching ratios for all possible transitions…
In weakly bound diatomic molecules, energy levels are closely spaced and thus more susceptible to mixing by magnetic fields than in the constituent atoms. We use this effect to control the strengths of forbidden optical transitions in…
Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…
We propose to introduce additional control in levitated optomechanics by trapping a meta-atom, i.e. a subwavelength and high-permittivity dielectric particle supporting Mie resonances. In particular, we theoretically demonstrate that…
We study optical cycling in the polar free radical calcium monohydroxide (CaOH) and establish an experimental path towards scattering $\sim$$10^4$ photons. We report rovibronic branching ratio measurements with precision at the…
We demonstrate the possibility of three-dimensional cooling of neutral atoms by illuminating them with two counterpropagating laser beams of mutually orthogonal linear polarization, where one of the lasers is a speckle field, i.e. a highly…
Optomechanics is a prime example of light matter interaction, where photons directly couple to phonons, allowing to precisely control and measure the state of a mechanical object. This makes it a very appealing platform for testing…
We present a laser cooling scheme for trapped ions and atoms using a combination of laser couplings and a magnetic gradient field. In a Schrieffer-Wolff transformed picture, this setup cancels the carrier and blue sideband terms completely…
Most ions lack the fast, cycling transitions that are necessary for direct laser cooling. In most cases, they can still be cooled sympathetically through their Coulomb interaction with a second, coolable ion species confined in the same…
Beams of polar molecules can be focused using an array of electrostatic lenses in alternating gradient (AG) configuration. They can also be accelerated or decelerated by applying an appropriate high voltage switching sequence to the lenses.…
We show that the vibrations of an ion Coulomb crystal can be cooled to the zero-point motion through the optomechanical coupling with a high-finesse cavity. Cooling results from the interplay between coherent scattering of cavity photons by…
Optical cycling refers to repeated excitation and spontaneous emission on an electronic transition in an atom or molecule. Optical cycling in molecules can enable a wide range of quantum control and readout techniques, but unfortunately it…
The atom-by-atom characterization of quantum gases requires the development of novel measurement techniques. One particularly promising new technique demonstrated in recent experiments uses strong fluorescent laser scattering from neutral…