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State of the art quantum sensing experiments targeting frequency measurements or frequency addressing of nuclear spins require to drive the probe system at the targeted frequency. In addition, there is a substantial advantage to perform…

Quantum Physics · Physics 2019-04-02 Nati Aharon , Ilai Schwartz , Alex Retzker

Zero-field nuclear magnetic resonance (NMR) provides complementary analysis modalities to those of high-field NMR and allows for ultra-high-resolution spectroscopy and measurement of untruncated spin-spin interactions. Unlike for the…

Quantum Physics · Physics 2022-03-01 Min Jiang , Teng Wu , John W. Blanchard , Guanru Feng , Xinhua Peng , Dmitry Budker

Experiments in coherent spectroscopy correspond to control of quantum mechanical ensembles guiding them from initial to final target states. The control inputs (pulse sequences) that accomplish these transformations should be designed to…

Quantum Physics · Physics 2009-11-07 Navin Khaneja , Timo Reiss , Burkhard Luy , Steffen J. Glaser

In nanoscale metrology applications, measurements are commonly limited by the performance of the sensor. Here we show that in nuclear magnetic resonance (NMR) spectroscopy measurements using single nitrogen-vacancy (NV) centers in diamond,…

Magnetic resonance spectroscopy is universally regarded as one of the most important tools in chemical and bio-medical research. However, sensitivity limitations typically restrict imaging resolution to length scales greater than 10 \mu m.…

Achieving atomic resolution is the ultimate limit of magnetic resonance imaging (MRI), and attaining this capability offers enormous technological and scientific opportunities, from drug development to understanding the dynamics in…

The limits of frequency resolution in nano-NMR experiments have been discussed extensively in recent years. It is believed that there is a crucial difference between the ability to resolve a few frequencies and the precision of estimating a…

Quantum sensors hold considerable promise for precision measurement, yet their capabilities are inherently constrained by environmental noise. A fundamental task in quantum sensing is determining the precision limit of noisy sensor devices.…

Quantum Physics · Physics 2026-04-14 Dayou Yang , Moulik Ketkar , Koenraad Audenaert , Susana F. Huelga , Martin B. Plenio

We present the architecture of the versatile NMR spectrometer with software-defined radio (SDR) technology and its application to the dynamically controlled pulsed magnetic fields. The pulse-field technology is the only solution to access…

Strongly Correlated Electrons · Physics 2021-11-24 Yoshihiko Ihara , Kaoru Hayashi , Tomoki Kanda , Kazuki Matsui , Koichi Kindo , Yoshimitsu Kohama

Precise timekeeping is critical to metrology, forming the basis by which standards of time, length and fundamental constants are determined. Stable clocks are particularly valuable in spectroscopy as they define the ultimate frequency…

The manipulation and metrology of light beams are pivotal for optical science and applications. In particular, achieving ultra-high precision in the measurement of light beam rotations has been a long-standing challenge. Instead of…

Quantum Physics · Physics 2025-10-13 Binke Xia , Jingzheng Huang , Hongjing Li , Zhongyuan Luo , Guihua Zeng

In this paper, we study the design of pulse sequences for NMR spectroscopy as a problem of time optimal control of the unitary propagator. Radio frequency pulses are used in coherent spectroscopy to implement a unitary transfer of state.…

Quantum Physics · Physics 2009-11-06 Navin Khaneja , Roger Brockett , Steffen Glaser

Quantum sensors have recently achieved to detect the magnetic moment of few or single nuclear spins and measure their magnetic resonance (NMR) signal. However, the spectral resolution, a key feature of NMR, has been limited by relaxation of…

We address metrological protocols for the estimation of the intensity and the orientation of a magnetic field, and show that quantum-enhanced precision may be achieved by probing the field with an arbitrary spin at thermal equilibrium. We…

Quantum Physics · Physics 2018-07-04 Filippo Troiani , Matteo G. A. Paris

Nonlinear spectroscopy is widely used for studying physical systems. Conventional nonlinear optical spectroscopy and magnetic resonance spectroscopy, which use classical probes such as electromagnetic waves, can only access certain types of…

Quantum metrology experiments in atomic physics and quantum optics have demonstrated measurement accuracy beyond the shot-noise limit via multi-particle entanglement. At the same time, electron microscopy, an essential tool for…

Quantum control plays a crucial role in enhancing precision scaling for quantum sensing. However, most existing protocols require perfect control, even though real-world devices inevitably have control imperfections. Here, we consider a…

Quantum Physics · Physics 2025-12-09 Zi-Shen Li , Xinyue Long , Xiaodong Yang , Dawei Lu , Yuxiang Yang

Nano-mechanical resonators have a large potential as sensors of very small adsorbed masses, down to the atomic level and beyond. Here I establish the fundamental lower bound on the mass that can be measured with a nano-mechanical oscillator…

Quantum Physics · Physics 2012-07-23 Daniel Braun

Nuclear magnetic resonance offers an appealing prospect for implementation of quantum computers, because of the long coherence times associated with nuclear spins, and extensive laboratory experience in manipulating the spins with radio…

Quantum Physics · Physics 2007-05-23 Leonard J. Schulman , Umesh Vazirani

The shot-noise detection limit in current high-precision atomic magnetometry is a manifestation of quantum fluctuations that scale as the square root of N in an ensemble of N particles. However, there is a general expectation that the…

Quantum Physics · Physics 2007-05-23 JM Geremia , John K. Stockton , Andrew C. Doherty , Hideo Mabuchi
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