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Strong Coulomb correlations together with multi-valley electronic bands in the presence of spin-orbit interaction and possible new optoelectronic applications are at the heart of studies of the rich physics of excitons in semiconductor…

Photophysics of single-wall carbon nanotubes (SWCNTs) is intensively studied due to their potential application in light harvesting and optoelectronics. Excited states of SWCNTs form strongly bound electron-hole pairs, excitons, of which…

Mesoscale and Nanoscale Physics · Physics 2021-01-28 J. Palotas , M. Negyedi , S. Kollarics , A. Bojtor , P. Rohringer , Th. Pichler , F. Simon

Optical properties in van der Waals heterostructures based on monolayer transition-metal dichalcogenides (TMDs), are often dominated by excitonic transitions. While intrinsic spin-orbit coupling (SOC) and an isotropic band structure are…

Mesoscale and Nanoscale Physics · Physics 2024-02-07 Jiayu David Cao , Gaofeng Xu , Benedikt Scharf , Konstantin Denisov , Igor Zutic

Over the past few decades, thin film optoelectronic devices based on transition metal dichalcogenides (TMDs) have made significant progress. However, the sensitivity of the exciton states to environmental change presents challenges for…

Optics · Physics 2024-03-13 Shuangping Han , Pengyu Zan , Yu Yan , Yaoxing Bian , Chengbing Qin , Liantuan Xiao

Monolayer transition metal dichalcogenides (TMDs) are direct gap semiconductors that hold great promise for advanced applications in photonics and optoelectronics. Understanding the interplay between their radiative and non-radiative…

Transition metal dichalcogenides (TMDs) constitute a versatile platform for atomically thin optoelectronics devices and spin-valley memory applications. In monolayers optical absorption is strong, but the transition energy is not tunable as…

Two-dimensional van der Waals (vdW) magnetic semiconductors CrSBr offer an ideal platform to achieve exciton-polaritons correlated with magnetic orders for developing solid-state quantum, spintronic, and photonic devices. However, for the…

Transition-metal dichalcogenide bilayers exhibit a rich exciton landscape including layer-hybridized excitons, i.e. excitons which are of partly intra- and interlayer nature. In this work, we study hybrid exciton-exciton interactions in…

Mesoscale and Nanoscale Physics · Physics 2023-06-28 Daniel Erkensten , Samuel Brem , Raul Perea-Causin , Joakim Hagel , Fedele Tagarelli , Edoardo Lopriore , Andras Kis , Ermin Malic

The degree of electronic coupling between individual layers in few-layer van der Waals heterostructures offers a route to engineer their magnetic, electronic, and optical functionalities. Using state-of-the-art first-principles…

Materials Science · Physics 2026-01-21 Sijia Ke , Yusuf Shaidu , Jeffrey B. Neaton

Semiconducting Transition Metal Dichalcogenides (TMDs) have significant nonlinear optical effects. In this work we have used second-harmonic generation (SHG) and the four-wave mixing (FWM) spectroscopy in resonance with the excitons in…

Excitons in monolayer transition-metal-dichalcogenides (TMDs) dominate their optical response and exhibit strong light-matter interactions with lifetime-limited emission. While various approaches have been applied to enhance light-exciton…

Transitions metal dichalcogenides (TMDs) are direct semiconductors in the atomic monolayer (ML) limit with fascinating optical and spin-valley properties. The strong optical absorption of up to 20 % for a single ML is governed by excitons,…

Mesoscale and Nanoscale Physics · Physics 2018-09-26 B. Han , C. Robert , E. Courtade , M. Manca , S. Shree , T. Amand , P. Renucci , T. Taniguchi , K. Watanabe , X. Marie , L. E. Golub , M. M. Glazov , B. Urbaszek

The nanoscale periodic potentials introduced by moir\'{e} patterns in semiconducting van der Waals (vdW) heterostructures provide a new platform for designing exciton superlattices. To realize these applications, a thorough understanding of…

Control of excitons in transition metal dichalcogenides (TMDCs) and their heterostructures is fundamentally interesting for tailoring light-matter interactions and exploring their potential applications in high-efficiency optoelectronic and…

Mesoscale and Nanoscale Physics · Physics 2023-06-13 Mahfujur Rahaman , Gwangwoo Kim , Kyung Yeol Ma , Seunguk Song , Hyeon Suk Shin , Deep Jariwala

Monolayer transition-metal dichalcogenide (TMD) semiconductors exhibit strong excitonic effects and hold promise for optical and optoelectronic applications. Yet, electron doping of TMDs leads to the conversion of neutral excitons into…

Excitons -- bound electron-hole pairs -- play a central role in light-matter interaction phenomena, and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing…

Mesoscale and Nanoscale Physics · Physics 2023-08-15 Jenny Hu , Etienne Lorchat , Xueqi Chen , Kenji Watanabe , Takashi Taniguchi , Tony F. Heinz , Puneet A. Murthy , Thibault Chervy

Control over the optical properties of atomically thin two-dimensional (2D) layers, including those of transition metal dichalcogenides (TMDs), is needed for future optoelectronic applications. Remarkable advances have been achieved through…

Heterostructures comprising different monolayer semiconductors provide a new system for fundamental science and device technologies, such as in the emerging field of valleytronics. Here, we realize valley-specific interlayer excitons in…

Mesoscale and Nanoscale Physics · Physics 2016-01-13 Pasqual Rivera , Kyle L. Seyler , Hongyi Yu , John R. Schaibley , Jiaqiang Yan , David G. Mandrus , Wang Yao , Xiaodong Xu

An anomalous magneto-optical spectrum is discovered for dipolar valley excitons in twisted double layer transition metal dichalcogenides (TMD), where in-plane magnetic field induces a sizable multiplet splitting of exciton states inside the…

Mesoscale and Nanoscale Physics · Physics 2022-07-22 Huiyuan Zheng , Dawei Zhai , Wang Yao

Two-dimensional transition metal dichalcogenides (2D TMDCs) are promising candidates for ultra-thin active nanophotonic elements due to the strong tunable excitonic resonances that dominate their optical response. Here we demonstrate…

Optics · Physics 2023-04-26 Melissa Li , Claudio U. Hail , Souvik Biswas , Harry A. Atwater