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Excitons are composite bosons that can feature spin singlet and triplet states. In usual semiconductors, without an additional spin-flip mechanism, triplet excitons are extremely inefficient optical emitters. Transition metal…

Excitons in semiconductors, bound pairs of excited electrons and holes, can form the basis for new classes of quantum optoelectronic devices. A van der Waals heterostructure built from atomically thin semiconducting transition metal…

Excitons in monolayer semiconductors have large optical transition dipole for strong coupling with light field. Interlayer excitons in heterobilayers, with layer separation of electron and hole components, feature large electric dipole that…

Mesoscale and Nanoscale Physics · Physics 2019-03-07 Wei-Ting Hsu , Bo-Han Lin , Li-Syuan Lu , Ming-Hao Lee , Ming-Wen Chu , Lain-Jong Li , Wang Yao , Wen-Hao Chang , Chih-Kang Shih

Long-lived interlayer excitons with distinct spin-valley physics in van der Waals heterostructures based on transition metal dichalcogenides make them promising for information processing in next-generation devices. While the emission…

Mesoscale and Nanoscale Physics · Physics 2021-10-18 Alberto Ciarrocchi , Dmitrii Unuchek , Ahmet Avsar , Kenji Watanabe , Takashi Taniguchi , Andras Kis

Excitons are key to the optoelectronic applications of van der Waals semiconductors with the potential for versatile on-demand tuning of properties. Yet, their electrical manipulation is complicated by their inherent charge neutrality and…

Mesoscale and Nanoscale Physics · Physics 2024-04-16 Sarthak Das , Ding Huang , Ivan Verzhbitskiy , Zi-En Ooi , Chit Siong Lau , Rainer Lee , Calvin Pei Yu Wong , Kuan Eng Johnson Goh

We investigate the optical properties of spin-triplet interlayer excitons in heterobilayer transition metal dichalcogenides in comparison with the spin-singlet ones. Surprisingly, the optical transition dipole of the spin-triplet exciton is…

Mesoscale and Nanoscale Physics · Physics 2018-05-15 Hongyi Yu , Gui-Bin Liu , Wang Yao

The optical properties of monolayer and bilayer transition metal dichalcogenide semiconductors are governed by excitons in different spin and valley configurations, providing versatile aspects for van der Waals heterostructures and devices.…

Mesoscale and Nanoscale Physics · Physics 2020-10-28 J. Förste , N. V. Tepliakov , S. Yu. Kruchinin , J. Lindlau , V. Funk , M. Förg , K. Watanabe , T. Taniguchi , A. S. Baimuratov , A. Högele

Monolayers of transition metal dichalcogenides (TMDCs) feature exceptional optical properties that are dominated by excitons, tightly bound electron-hole pairs. Forming van der Waals heterostructures by deterministically stacking individual…

Excitons in transition metal dichalcogenides (TMDs) have emerged as a promising platform for novel applications ranging from optoelectronic devices to quantum optics and solid state quantum simulators. While much progress has been made…

Controlling interlayer excitons in van der Waals heterostructures holds promise for exploring Bose-Einstein condensates and developing novel optoelectronic applications, such as excitonic integrated circuits. Despite intensive studies,…

Mesoscale and Nanoscale Physics · Physics 2024-04-09 Lifu Zhang , Ruihao Ni , Liuxin Gu , Ming Xie , Suji Park , Houk Jang , Takashi Taniguchi , Kenji Watanabe , You Zhou

Integrating two-dimensional van der Waals materials with optical cavities has revealed a fascinating platform to study exciton-polariton physics. Manipulating exciton polaritons often requires external control over the electrical and…

Optics · Physics 2023-11-08 Zhi Wang , Li He , Bumho Kim , Bo Zhen

Transition metal dichalcogenide (TMD) monolayers are two-dimensional semiconductors with two valleys in their band structure that can be selectively addressed using circularly polarized light. Their photoluminescence spectrum is…

Mesoscale and Nanoscale Physics · Physics 2020-10-26 Joris J. Carmiggelt , Michael Borst , Toeno van der Sar

The ultrathin transition metal dichalcogenides (TMDs) have emerged as promising materials for various applications using two dimensional (2D) semiconductors. They have attracted increasing attention due to their unique optical properties…

Mesoscale and Nanoscale Physics · Physics 2016-09-20 Aïda Hichri , Imen Ben Amara , Sabrine Ayari , Sihem Jaziri

Strongly bound excitons and many-body interactions between them determine light-matter interactions in van der Waals (vdW) heterostructures of 2D semiconductors. Unlike fundamental particles, quasiparticles in condensed matter, such as…

Mesoscale and Nanoscale Physics · Physics 2022-08-12 Weijie Li , Zach Hadjri , Jin Zhang , Luka M. Devenica , Song Liu , James Hone , Kenji Watanabe , Takashi Taniguchi , Angel Rubio , Ajit Srivastava

Emerging photo-induced excitonic processes in transition metal dichalcogenide (TMD) heterobilayers, e.g., coupling, dephasing, and energy transfer of intra- and inter-layer excitons, allow new opportunities for ultrathin photonic devices.…

Spin triplet exciton formation sets limits on technologies using organic semiconductors that are confined to singlet-triplet photophysics. In contrast, excitations in the spin doublet manifold in organic radical semiconductors can show…

Chemical Physics · Physics 2023-12-19 Qinying Gu , Sebastian Gorgon , Alexander S. Romanov , Feng Li , Richard H. Frienda , Emrys Evansd

Twisted atomically thin semiconductors are characterized by moir\'{e} excitons. Their optical signatures and selection rules are well understood. However, their hybridization with photons in the strong coupling regime for heterostructures…

Mesoscale and Nanoscale Physics · Physics 2022-06-22 Jamie M. Fitzgerald , Joshua J. P. Thompson , Ermin Malic

Throughout the years, strongly correlated coherent states of excitons have been the subject of intense theoretical and experimental studies. This topic has recently boomed due to new emerging quantum materials such as van der Waals (vdW)…

Mesoscale and Nanoscale Physics · Physics 2021-12-30 Igor V. Bondarev , Oleg L. Berman , Roman Ya. Kezerashvili , Yurii E. Lozovik

Van der Waals materials and heterostructures manifesting strongly bound room temperature exciton states exhibit emergent physical phenomena and are of a great promise for optoelectronic applications. Here, we demonstrate that nanostructured…

Because of the reduced dielectric screening and enhanced Coulomb interactions, two-dimensional (2D) materials like phosphorene and transition metal dichalcogenides (TMDs) exhibit strong excitonic effects, resulting in fascinating…

Materials Science · Physics 2019-11-04 Xiaoyang Zheng , Xian Zhang
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