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We propose a new scheme to control the shape of the Autler-Townes (AT) doublet in the photoelectron spectrum from atomic resonance-enhanced multiphoton ionization (REMPI). The scheme is based on the interference of two AT doublets created…

Atomic Physics · Physics 2025-07-01 T. Bayer , K. Eickhoff , D. Köhnke , M. Wollenhaupt

We study non-classical pathways and quantum interference in enhanced ionisation of diatomic molecules in strong laser fields using machine learning techniques. Quantum interference provides a bridge, which facilitates intramolecular…

We use orthogonally polarized two-colour (OTC) laser pulses to separate quantum paths in multiphoton ionization of Ar atoms. Our OTC pulses consist of 400~nm and 800~nm light at a relative intensity ratio of 10:1. We find a hitherto…

We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…

We use a Wigner distribution-like function based on the strong field approximation theory to obtain the time-energy distributions and the ionization time distributions of electrons ionized by an XUV pulse alone and in the presence of an…

Atomic Physics · Physics 2021-09-01 L. Guo , Y. Jia , M. Q. Liu , X. Y. Jia , S. L. Hu , R. H. Lu , S. S. Han , J. Chen

The dynamics of atomic levels resonantly coupled by a coherent and intense short high-frequency laser pulse is discussed and it is advocated that this dynamics is sensitively probed by measuring the spectra of the particles emitted. It is…

Atomic and Molecular Clusters · Physics 2013-01-11 Philipp V. Demekhin , Lorenz S. Cederbaum

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…

Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…

Chemical Physics · Physics 2019-09-11 R. Chamakhi , M. Telmini , O. Atabek , E. Charron

We investigate electron momentum distributions from single ionization of Ar by two orthogonally polarized laser pulses of different color. The two-color scheme is used to experimentally control the interference between electron wave packets…

We study ionization of atoms in strong orthogonal two-color ($\omega,2\omega$) (OTC) laser fields numerically and analytically. The calculated photoelectron momentum distribution shows two typical structures: a rectangular-like structure…

Atomic Physics · Physics 2023-06-21 J. N. Wu , J. Y. Che , F. B. Zhang , C. Chen , W. Y. Li , G. G. Xin , Y. J. Chen

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

Atomic Physics · Physics 2016-03-30 Jhih-An You , Nina Rohringer , Jan Marcus Dahlström

The coherent control of light with matter, enabling storage and manipulation of optical signals, was revolutionized by electromagnetically induced transparency (EIT), which is a quantum interference effect. For strong electromagnetic fields…

How fast can a laser pulse ionize an atom? We address this question by considering pulses that carry a fixed time-integrated energy per-area, and finding those that achieve the double requirement of maximizing the ionization that they…

Atomic Physics · Physics 2017-06-07 David Kammerlander , Alberto Castro , Miguel A. L. Marques

Controllable arrays of ions and ultra-cold atoms can simulate complex many-body phenomena and may provide insights into unsolved problems in modern science. To this end, experimentally feasible protocols for quantifying the buildup of…

Femtosecond light pulses carrying optical angular momentums (OAMs), possessing intriguing properties of helical phase fronts and ultrafast temporal profiles, enable many applications in nonlinear optics, strong-field physics and laser…

Recent experimental techniques in multicolor waveform synthesis allow the temporal shaping of strong femtosecond laser pulses with applications in the control of quantum mechanical processes in atoms, molecules, and nanostructures.…

Atomic Physics · Physics 2017-10-11 Janne Solanpää , Marcelo F. Ciappina , Esa Räsänen

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

We analyze the two-dimensional momentum distribution of electrons ionized by few-cycle laser pulses in the transition regime from multiphoton absorption to tunneling by solving the time-dependent Schr\"odinger equation and by a…

Quantum Physics · Physics 2007-05-23 D. G. Arbó , S. Yoshida , E. Persson , K. I. Dimitriou , J. Burgdörfer

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

We consider pump-probe spectroscopy of a single ion with a highly metastable (probe) clock transition which is monitored by using the quantum jump technique. For a weak clock laser we obtain the well known Autler-Townes splitting. For…

Quantum Physics · Physics 2015-01-15 J. von Zanthier , C. Skornia , G. S. Agarwal , H. Walther
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