Related papers: Ultrafast Intercavity Nonlinear Couplings between …
Modulational instabilities play a key role in a wide range of nonlinear optical phenomena, leading e.g. to the formation of spatial and temporal solitons, rogue waves and chaotic dynamics. Here we experimentally demonstrate the existence of…
Controlling matter-light interactions with cavities is of fundamental importance in modern science and technology. It is exemplified in the strong-coupling regime, where matter-light hybrid modes form, with properties controllable via the…
Sub-wavelength electromagnetic field localization has been central in photonic research in the last decade, allowing to enhance sensing capabilities as well as increasing the coupling between photons and material excitations. The…
The strong coupling of an IR-active molecular transition with an optical mode of the cavity results in vibrational polaritons, which opens a new way to control chemical reactivity via confined electromagnetic fields of the cavity. In this…
We analytically tackle opto-vibronic interactions in molecular systems driven by either classical or quantum light fields. In particular, we examine a simple model of molecules with two relevant electronic levels, characterized by potential…
Realizing strong interactions between individual photons is a cornerstone for advancing photonic quantum computing and quantum nonlinear optics. Here, we experimentally demonstrate strong interactions between counter-propagating photons…
Semiconductor microcavities operating in the polaritonic regime are highly non-linear, high speed systems due to the unique half-light, half-matter nature of polaritons. Here, we report for the first time the observation of propagating…
Ultrafast atomic vibrations mediate heat transport, serve as fingerprints for chemical bonds and drive phase transitions in condensed matter systems. Light pulses shorter than the atomic oscillation period can not only probe, but even…
Optomechanical systems provide a unique platform for observing quantum behavior of macroscopic objects. However, efforts towards realizing nonlinear behavior at the single photon level have been inhibited by the small size of the radiation…
Cavity-polaritons in semiconductor photonic structures have emerged as a test bed for exploring non-equilibrium dynamics of quantum fluids in an integrated solid-state device setting. Several recent experiments demonstrated the potential of…
Strong inter-particle interactions between polaritons have traditionally stemmed from their exciton component. In this work, we impart a strong photonic nonlinearity to a polaritonic mode by embedding a nonlinear polymethine dye within a…
A theoretical framework is presented for the computation of rovibrational polaritonic states of a molecule in a lossless infrared (IR) microcavity. In the proposed approach the quantum treatment of the rotational and vibrational motion of…
The achievement of large values of the light-matter coupling in nanoengineered photonic structures can lead to multiple photonic resonances contributing to the final properties of the same hybrid polariton mode. We develop a general theory…
An outstanding goal in quantum optics is the realization of fast optical non-linearities at the single-photon level. Such non-linearities would allow for the realization of optical devices with new functionalities such as a single-photon…
Phonon polaritons are hybrid states of light and matter that are typically realised when optically active phonons couple strongly to photons. We suggest a new approach to realising phonon polaritons, by employing a transverse-pumping Raman…
Conventional approaches to probing ultrafast molecular dynamics rely on the use of synchronized laser pulses with a well-defined time delay. Typically, a pump pulse excites a wavepacket in the molecule. A subsequent probe pulse can then…
Large exciton-polariton optical nonlinearities present a key mechanism for photonics-based communication, ultimately in the quantum regime. Enhanced nonlinear response from various materials hosting excitons and allowing for their strong…
We investigate Jahn-Teller (JT) polaritons, which emerge from the interaction of the two normal-incidence electromagnetic modes with perpendicular polarizations in a Fabry-Perot cavity resonator with JT active systems. These JT polaritons…
We provide a systemic theory to entangle excitons with microcavity photons. This is realized by adopting an exciton-optomechanics system and introducing a nonlinear dispersive interaction with a mechanical oscillator. We show that when…
The strong coupling between an intersubband excitation in a quantum cascade structure and a photonic mode of a planar microcavity has been detected by angle-resolved photovoltaic measurements. A typical anticrossing behavior, with a…