Related papers: Bell correlations between light and vibration at a…
Plasmon-enhanced Raman scattering can push single-molecule vibrational spectroscopy beyond a regime addressable by classical electrodynamics. We employ a quantum electrodynamics (QED) description of the coherent interaction of plasmons and…
We have theoretically investigated the possibility of using any of several continuous-variable Bell-type inequalities - for which the dichotomic measurements are achieved with coarse-grained quadrature (homodyne) measurements - in a…
We image with cameras entangled photon light transmitted through a random medium. Near-field and far-field spatial quantum correlations show that entangled photon pairs (bi-photons) generated by spontaneous optical parametric…
Recent advances in non-Hermitian physical systems have led to numerous novel optical phenomena and applications. However, most realizations are limited to classical systems and quantum fluctuations of light is unexplored. For the first…
The pure quantum correlations totally independent of the classical coherence of light have been experimentally demonstrated. By measuring the visibility of the interference fringes and the correlation variances of amplitude and phase…
Low-frequency Raman and inelastic neutron scattering of amorphous bis-phenol A polycarbonate is measured at low temperature, and compared. The vibrational density of states and light-vibration coupling coefficient are determined. The…
We investigate the feasibility of correlating an optical cavity field and a vibrational phonon mode. A laser pumped quantum dot fixed on a nano-mechanical resonator beam interact as a whole with the optical resonator mode. When the quantum…
The conventional explanation of plasmon-enhanced Raman scattering attributes the enhancement to the antenna effect focusing the electromagnetic field into sub-wavelength volumes. Here we introduce a new model that additionally accounts for…
There is a growing consensus that the exceptional optoelectronic properties of metal halide perovskites (MHPs) are largely due to the peculiar interplay between the inorganic cage lattice, composed of a labile network of corner-sharing…
Frequency-resolved photon correlations have proven to be a useful resource to unveil nonlinearities hidden in standard observables such as the spectrum or the standard (color-blind) photon correlations. In this manuscript, we analyze the…
Interplay between the effects of coherent radiation and localization of light is analysed. A system of two-level atoms is placed in a medium interacting with electromagnetic field. The matter-light interaction can result in the appearance…
The light-harvesting efficiency of a photoactive molecular complex is largely determined by the properties of its electronic quantum states. Those, in turn, are influenced by molecular vibrational states of the nuclear degrees of freedom.…
We explore quantum correlations, in particular, quantum entanglement, among vibrational phonon modes as well as between electronic and vibrational degrees of freedom in molecular systems, described by Jahn-Teller mechanism. Specifically, to…
A theoretical model describing the Raman scattering process in atomic vapors is constructed. The treatment investigates the low-excitation regime suitable for modern experimental applications. Despite the incorporated decoherence effects…
Nonlocal entanglement between pair-correlated particles is a highly counter-intuitive aspect of quantum mechanics, where measurement on one particle can instantly affect the other, regardless of distance. While the rigorous Bell's…
Resonant coupling of a vibration to a cavity mode has been reported to dramatically modify spontaneous Raman scattering, but subsequent studies have produced conflicting results. In this Letter, we develop a microscopic quantum framework…
Ultrafast spectroscopies can access the dynamics of electrons and nuclei at short timescales, shedding light on nonequilibrium phenomena in materials. However, development of accurate calculations to interpret these experiments has lagged…
Vibrational polaritons are formed by strong coupling of molecular vibrations and photon modes in an optical cavity. Experiments have demonstrated that vibrational strong coupling can change molecular properties and even affect chemical…
Raman spectroscopy uses light scattering to extract information on low-energy excitations of solids. The Raman process is described by diagrams which are fourth order in the light-matter interaction, and in particular the resonant…
Photons of a laser beam driving the upper motional sideband of an optomechanical cavity can decay into photon-phonon pairs by means of an optomechanical parametric process. The phononic state can subsequently be mapped to a photonic state…