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We report phase-coherent Doppler detection of optical dipole forces using large ion crystals in a Penning trap. The technique is based on laser Doppler velocimetry using a cycling transition in $^{9}$Be$^{+}$ near 313 nm and the…

Quantum Physics · Physics 2015-05-27 M. J. Biercuk , H. Uys , J. W. Britton , A. P. VanDevender , J. J. Bollinger

We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…

Quantum Physics · Physics 2021-06-23 Zhedong Zhang , Tao Peng , Xiaoyu Nie , Girish S. Agarwal , Marlan O. Scully

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

Raman scattering spectroscopy is widely used as an analytical technique in various fields, but its measurement process tends to be slow due to the low scattering cross-section. In the last decade, various broadband coherent Raman scattering…

Optics · Physics 2025-05-06 Takuma Nakamura , Kazuki Hashimoto , Takuro Ideguchi

We demonstrate a novel technique of coherent Raman spectroscopy with a femtosecond laser. We apply to a molecular sample a sequence of pairs of ultrashort excitation and probe pulses, with a linearly increasing time delay between the two…

Raman spectroscopy uses light scattering to extract information on low-energy excitations of solids. The Raman process is described by diagrams which are fourth order in the light-matter interaction, and in particular the resonant…

Strongly Correlated Electrons · Physics 2024-01-30 Philipp Werner , Martin Eckstein , Naoto Tsuji

An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…

Atomic Physics · Physics 2016-12-21 David A. Long , Adam J. Fleisher , David F. Plusquellic , Joseph T. Hodges

We present a novel approach to achieve hyper spectral resolution, high sensitive detection, and high speed data acquisition Stimulated Raman Spectroscopy by employing amplified offset-phase controlled fs-pulse bursts. In this approach, the…

Measuring the phase of light is fundamental to optical imaging, sensing, and signal processing applications. Conventional optical phase measurements rely on multipath configurations, bulky interferometric setups, and computationally…

Nonlinear frequency conversion provides an elegant method to detect photons in a spectral range which differs from the pump wavelength, making it highly attractive for photons with inherently low energy. Aside from the intensity of the…

Optics · Physics 2022-02-10 Tobias Pfeiffer , Jens Klier , Georg von Freymann , Daniel Molter

We consider theoretically light scattering by a resonant layer that periodically moves in real space. At small frequencies of motion the scattered light spectrum reveals the frequency shift that is governed by the Doppler effect. At higher…

Optics · Physics 2020-12-02 A. V. Poshakinskiy , A. N. Poddubny , N. A. Gippius

Conventional optical coherent receivers capture the full electrical field, including amplitude and phase, of a signal waveform by measuring its interference against a stable continuous-wave local oscillator (LO). In optical coherent…

Signal Processing · Electrical Eng. & Systems 2020-06-24 Haoshuo Chen , Nicolas K. Fontaine , Joan M. Gene , Roland Ryf , David T. Neilson , Gregory Raybon

High-gain resonant nonlinear Raman scattering on trapped cold atoms within a high-fineness ring optical cavity is simply explained under a nonlinear opto-mechanical mechanism, and a proposal using it to detect frequency of micro-trap on…

Atomic Physics · Physics 2014-03-24 Lin Zhang

Measuring the spectral phase of a pulse is key for performing wavelength resolved ultrafast measurements in the few femtosecond regime. However, accurate measurements in real experimental conditions can be challenging. We show that the…

Enhanced Raman scattering can be obtained by injecting a seeded light field which is correlated with the initially prepared collective atomic excitation. This Raman amplification process can be used to realize atom-light hybrid…

Quantum Physics · Physics 2016-08-24 Zhao-Dan Chen , Chun-Hua Yuan , Hong-Mei Ma , Dong Li , L. Q. Chen , Z. Y. Ou , Weiping Zhang

Stimulated Raman spectroscopy has become a powerful tool to study the spatiodynamics of molecular bonds with high sensitivity, resolution and speed. However, sensitivity and speed of state-of-the-art stimulated Raman spectroscopy are…

Optical parametric amplification/oscillation provide a powerful tool for coherent light generation in spectral regions inaccessible to lasers. Parametric gain is based on a frequency {\it down-conversion} process, and thus it can not be…

Optics · Physics 2016-05-04 Stefano Longhi

We extend the technique of multiplex coherent Raman spectroscopy with two femtosecond mode-locked lasers to oscillators of a pulse repetition frequency of 1 GHz. We demonstrate spectra of liquids, which span 1100 cm$^{-1}$ of Raman shifts.…

Dispersive Fourier transformation is a powerful technique in which spectral information is mapped into the time domain using chromatic dispersion. It replaces a spectrometer with an electronic digitizer, and enables real-time spectroscopy.…

Optics · Physics 2009-11-13 J. Chou , D. R. Solli , B. Jalali

The Doppler spectrum estimation of a weather radar signal in a classic way can be made by two methods, temporal one based in the autocorrelation of the successful signals, whereas the other one uses the estimation of the power spectral…

Numerical Analysis · Mathematics 2025-10-20 Mohand Lagha , Messaoud Bensebti