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Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

We present an experimental study of the quantum spin ice candidate pyrochlore coumpound \przr\ by means of magnetization measurements, specific heat and neutron scattering up to 12 T and down to 60 mK. When the field is applied along the…

Within the past 20 years or so, there has occurred an explosion of interest in the magnetic behavior of pyrochlore oxides of the type $A_{2}^{3+}$$B_{2}^{4+}$O$_{7}$ where $A$ is a rare-earth ion and $B$ is usually a transition metal. Both…

Disordered Systems and Neural Networks · Physics 2010-01-26 Jason S. Gardner , Michel J. P. Gingras , John E. Greedan

While the spin liquid state in the frustrated pyrochlore Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ has been studied both experimentally and theoretically for more than two decades, no definite description of this unconventional state has been achieved.…

The intrinsic noncollinear spin patterns in rare-earth pyrochlore are physically interesting, hosting many emergent properties, e.g. spin ice and monopole-type excitation. Recently, the magnetic monopole excitation of spin ice systems was…

Materials Science · Physics 2015-12-18 Lin Lin , Y. L. Xie , J. -J. Wen , Shuai Dong , Z. B. Yan , J. -M. Liu

Geometrical frustration is a central challenge in contemporary condensed matter physics, a crucible favourable to the emergence of novel physics. The pyrochlore magnets, with rare earth magnetic moments localized at the vertices of…

Strongly Correlated Electrons · Physics 2015-05-30 Sylvain Petit , Pierre Bonville , Isabelle Mirebeau , Hannu Mutka , Julien Robert

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

Statistical Mechanics · Physics 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

Geometric frustration usually arises in systems that comprise magnetic moments (spins) which reside on the sites of a lattice made up of elementary triangular or tetrahedral units and which interact via antiferromagnetic nearest-neighbor…

Statistical Mechanics · Physics 2009-03-17 Michel J. P. Gingras

Frustration in magnetic systems is fertile ground for complex behaviour, including unconventional ground states with emergent symmetries, topological properties, and exotic excitations. A canonical example is the emergence of…

Strongly Correlated Electrons · Physics 2022-03-02 M. J. Pearce , K. Götze , A. Szabó , T. S. Sikkenk , M. R. Lees , A. T. Boothroyd , D. Prabhakaran , C. Castelnovo , P. A. Goddard

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

Magnetic skyrmions, vortex-like swirling spin textures characterized by a quantized topological invariant, realized in chiral-lattice magnets are currently attracting intense research interest. In particular, their dynamics under external…

Strongly Correlated Electrons · Physics 2016-01-20 Masahito Mochizuki , Shinichiro Seki

Recent excitement in the quantum spin ice community has come from the experimental discovery of pseudospin-$1/2$ breathing pyrochlores, including Ba$_3$Yb$_2$Zn$_5$O$_{11}$, in which inversion symmetry is broken by the `up' and `down'…

Strongly Correlated Electrons · Physics 2024-05-14 Alaric Sanders , Claudio Castelnovo

The magnetic pyrochlore oxide materials of general chemical formula R2Ti2O7 and R2Sn2O7 (R = rare earth) display a host of interesting physical behaviours depending on the flavour of rare earth ion. These properties depend on the value of…

Statistical Mechanics · Physics 2015-06-24 Adrian G. Del Maestro , Michel J. P. Gingras

Quantum spin liquids (QSL) have generated considerable excitement as phases of matter with emergent gauge structures and fractionalized excitations. In this context, phase transitions out of QSLs have been widely discussed as Higgs…

Strongly Correlated Electrons · Physics 2021-09-15 Hyeok-Jun Yang , Nic Shannon , SungBin Lee

While there is compelling evidence for the existence of magnetic monopoles in spin ice, the direct observation of a point-like source of magnetic field in these systems remains an open challenge. One promising approach is electron…

Strongly Correlated Electrons · Physics 2021-12-20 Ankur Dhar , Ludovic D. C. Jaubert , Cathal Cassidy , Tsumoru Shintake , Nic Shannon

We investigate the emergence of quantum spin liquid phases in pyrochlore oxides with non-Kramers ions, in which structural randomness effectively acts as a transverse field, introducing quantum fluctuations on top of the spin ice manifold.…

Strongly Correlated Electrons · Physics 2026-01-09 Marcus V. Marinho , Eric C. Andrade

We combine two aspects of magnetic frustration, multiferroicity and emergent quasi-particles in spin liquids, by studying magneto-electric monopoles. Spin ice offers to couple these emergent topological defects to external fields, and to…

Strongly Correlated Electrons · Physics 2015-06-24 Ludovic D. C. Jaubert , R. Moessner

We present a comprehensive study of the magnetoelastic properties of the Ising pyrochlore oxide Ho$_{2}$Ti$_{2}$O$_{7}$, known as spin ice, by means of high-field magnetostriction measurements and numerical calculations. When a magnetic…