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The spectral and spatiotemporal dynamics of photoluminescence in monolayers of transition metal dichalcogenide WSe$_2$ obtained by mechanical exfoliation on a Si/SiO$_2$ substrate is studied over a wide range of temperatures and excitation…

Mesoscale and Nanoscale Physics · Physics 2021-02-03 M. A. Akmaev , M. V. Kochiev , A. I. Duleba , M. V. Pugachev , A. Yu. Kuntsevich , V. V. Belykh

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

Materials Science · Physics 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

We present optical spectroscopy (photoluminescence and reflectance) studies of thin layers of the transition metal dichalcogenide WSe2, with thickness ranging from mono- to tetra-layer and in the bulk limit. The investigated spectra show…

Mesoscale and Nanoscale Physics · Physics 2015-03-06 Ashish Arora , Maciej Koperski , Karol Nogajewski , Jacques Marcus , Clement Faugeras , Marek Potemski

Monolayers of transition metal dichalcogenide materials emerged as a new material class to study excitonic effects in solid state, since they benefit from enormous coulomb correlations between electrons and holes. Especially in WSe2, sharp…

Monolayers of transition-metal dichalcogenides such as WSe2 have become increasingly attractive due to their potential in electrical and optical applications. Because the properties of these 2D systems are known to be affected by their…

MoSe2-WSe2 heterostructures host strongly bound interlayer excitons (IXs) which exhibit bright photoluminescence (PL) when the twist-angle is near 0{\deg} or 60{\deg}. Over the past several years, there have been numerous reports on the…

Observations of polariton condensation in semiconductor microcavities suggest that polaritons can be exploited as a novel type of laser with low input-power requirements. The low-excitation regime is approximately equivalent to thermal…

Mesoscale and Nanoscale Physics · Physics 2013-07-16 Tomoyuki Horikiri , Yasuhiro Matsuo , Yutaka Shikano , Andreas Loeffler , Sven Hoefling , Alfred Forchel , Yoshihisa Yamamoto

We present a detailed investigation of the exciton and trion dynamics in naturally doped MoSe2 and WSe2 single atomic layers as a function of temperature in the range 10-300K under above band-gap laser excitation. By combining…

We report an efficient method to observe single photon emissions in monolayer WSe2 by applying hydrostatic pressure. The photoluminescence peaks of typical two-dimensional (2D) excitons show a nearly identical pressure-induced blue-shift,…

Materials Science · Physics 2017-07-05 Yanxia Ye , Xiuming Dou , Kun Ding , Yu Chen , Desheng Jiang , Fuhua Yang , Baoquan Sun

We study the optical properties of thin flakes of InSe encapsulated in hBN. More specifically, we investigate the photoluminescence (PL) emission and its dependence on sample thickness and temperature. Through the analysis of the PL…

Monolayer 2D semiconductors, such as WS2, exhibit uniquely strong light-matter interactions due to exciton resonances that enable atomically-thin optical elements. Similar to geometry-dependent plasmon and Mie resonances, these intrinsic…

In recent years, much research has been undertaken to investigate the suitability of two-dimensional materials to act as single-photon sources with high optical and quantum optical quality. Amongst them, transition-metal dichalcogenides,…

The band structure of MoS$_2$ strongly depends on the number of layers, and a transition from indirect to direct-gap semiconductor has been observed recently for a single layer of MoS$_2$. Single-layer MoS$_2$ therefore becomes an efficient…

Materials Science · Physics 2011-09-13 T. Korn , S. Heydrich , M. Hirmer , J. Schmutzler , C. Schüller

We studied multi-exciton dynamics in monolayer WSe2 using nonlinear photoluminescence (PL) spectroscopy and Monte Carlo simulations. We observed strong nonlinear saturation behavior of exciton PL with increasing excitation power density,…

Mesoscale and Nanoscale Physics · Physics 2014-11-05 Shinichiro Mouri , Yuhei Miyauchi , Minglin Toh , Weijie Zhao , Goki Eda , Kazunari Matsuda

Optical orientation of localized/bound excitons is shown to be effectively enhanced by the application of magnetic fields as low as 20 mT in monolayer WS$_2$. At low temperatures, the evolution of the polarization degree of different…

We study the excitonic recombination dynamics in an ensemble of (9,4) semiconducting single-wall carbon nanotubes by high sensitivity time-resolved photo-luminescence experiments. Measurements from cryogenic to room temperature allow us to…

Other Condensed Matter · Physics 2015-06-25 S. Berger , C. Voisin , G. Cassabois , C. Delalande , Philippe Roussignol , X. Marie

In heterostructures consisting of different transition-metal dichalcogenide monolayers, a staggered band alignment can occur, leading to rapid charge separation of optically generated electron-hole pairs into opposite monolayers. These…

We investigate the photoluminescence of interlayer excitons in heterostructures consisting of monolayer MoSe2 and WSe2 at low temperatures. Surprisingly, we find a doublet structure for such interlayer excitons. Both peaks exhibit long…

The optically dark states play an important role in the electronic and optical properties of monolayers (MLs) of semiconducting transition metal dichalcogenides. The effect of temperature on the in-plane-field activation of the neutral and…

Single-layer WS$_2$ is a direct-gap semiconductor showing strong excitonic photoluminescence features in the visible spectral range. Here, we present temperature-dependent photoluminescence measurements on mechanically exfoliated…

Mesoscale and Nanoscale Physics · Physics 2015-09-08 Gerd Plechinger , Philipp Nagler , Julia Kraus , Nicola Paradiso , Christoph Strunk , Christian Schüller , Tobias Korn
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