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The latest discovery of ferromagnetism in atomically thin films of semiconductors Cr$_2$Ge$_2$Te$_6$ and CrI$_3$ has unleashed numerous opportunities for fundamental physics of magnetism in two-dimensional (2D) limit and also for…

Mesoscale and Nanoscale Physics · Physics 2019-05-09 Vijay Kumar Gudelli , Guang-Yu Guo

After the discovery of magnetism in monolayer CrI3, the magnetic properties of different 2D materials from the chromium-trihalide family are intuitively assumed to be similar, yielding magnetic anisotropy from the spin-orbit coupling on…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 C. Bacaksiz , D. Šabani , R. M. Menezes , M. V. Milošević

The discovery of atomically thin two-dimensional (2D) magnetic semiconductors has triggered enormous research interest recently. In this work, we use first-principles many-body perturbation theory to study a prototypical 2D ferromagnetic…

Materials Science · Physics 2022-02-01 Meng Wu , Zhenglu Li , Steven G. Louie

A monolayer of CrI3 has an amazing ferromagnetic ground-state. In this work, we calculate band structures and magnetic moments of tensile-strained and bent zigzag CrI3 nanoribbons with density functional theory. The edge iodine atoms form…

Materials Science · Physics 2022-11-02 Hong Tang , Santosh Neupane , Qimin Yan , Adrienn Ruzsinszky

Chromium trihalides, CrX$_3$ (with X = Cl, Br, I), are a family of layered magnetic materials that can be easily exfoliated to provide ferromagnetic monolayers. When two layers are stacked together to form a bilayer the interlayer exchange…

Materials Science · Physics 2020-12-30 Marco Gibertini

We analyze magnetic properties of monolayers and bilayers of chromium trihalides, CrI$_3$, in two different stacking configurations: AA and rhombohedral ones. Our main focus is on the corresponding Curie temperatures, hysteresis curves,…

Mesoscale and Nanoscale Physics · Physics 2024-04-25 S. Stagraczynski , P. Balaz , M. Jafari , J. Barnas , A. Dyrdal

Bright excitons in ferromagnetic monolayers CrI$_3$ efficiently interact with lattice magnetization, which makes possible all-optical resonant magnetization control in this material. Using the combination of ab-initio simulations within…

Mesoscale and Nanoscale Physics · Physics 2023-05-23 A. Kudlis , M. Kazemi , Y. Zhumagulov , H. Schrautzer , P. F. Bessarab , I. V. Iorsh , I. A. Shelykh

We present a density functional theory (DFT) based study of a two-dimensional phase of chromium bismuthate (CrBi), previously unknown material with exceptional magnetic and magnetooptical characteristics. Monolayer CrBi is a ferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2021-06-29 A. Mogulkoc , M. Modarresi , A. N. Rudenko

Recent observation of intrinsic ferromagnetism in two-dimensional (2D) CrI$_3$ is associated with the large magnetic anisotropy due to strong spin-orbit coupling (SOC) of I. Magnetic anisotropy energy (MAE) defines the stability of…

Mesoscale and Nanoscale Physics · Physics 2018-10-10 Lucas Webster , Jia-An Yan

The discovery of ferromagnetic order in monolayer 2D crystals has opened a new venue in the field of two dimensional (2D) materials. 2D magnets are not only interesting on their own, but their integration in van der Waals heterostructures…

Mesoscale and Nanoscale Physics · Physics 2020-08-24 D. Soriano , M. I. Katsnelson , J. Fernández-Rossier

We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

Considerable research interest has been attracted to noncollinear magnetic structures for their intriguing physics and promising applications. In this work, based on relativistic density functional theory, we reveal the interesting magnetic…

Materials Science · Physics 2022-11-14 Na Wang , Jun Chen , Ning Ding , Huimin Zhang , Shuai Dong , Shan-Shan Wang

Chromium triiodide is an intrinsically magnetic van der Waals material down to the single-layer limit. Here, we provide a first-principles description of finite-temperature magnetic and spectral properties of monolayer (ML) CrI$_3$ based on…

Strongly Correlated Electrons · Physics 2022-05-24 Yaroslav O. Kvashnin , Alexander N. Rudenko , Patrik Thunström , Malte Rösner , Mikhail I. Katsnelson

We present a detailed study on the microscopic origin of magnetism in suspended and dielectrically embedded CrI$_3$ monolayer. To this end, we down-fold two distinct minimal generalized Hubbard models with different orbital basis sets from…

Strongly Correlated Electrons · Physics 2021-10-06 D. Soriano , A. N. Rudenko , M. I. Katsnelson , M. Rösner

We apply the density-functional theory to study various phases (including non-magnetic (NM), anti-ferromagnetic (AFM), and ferromagnetic (FM)) in monolayer magnetic chromium triiodide (CrI$_3$), a recently fabricated 2D magnetic material.…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Lucas Webster , Liangbo Liang , Jia-An Yan

The discovery of spontaneous magnetism in van der Waal (vdW) magnetic monolayers has opened up an unprecedented platform for investigating magnetism in purely two-dimensional systems. Recently, it has been shown that the magnetic properties…

Mesoscale and Nanoscale Physics · Physics 2022-01-19 Eliot Heinrich , Xin Li , Benedetta Flebus

Twisting in bilayers introduces structural chirality with two enantiomers, i.e., left- and right-hand bilayers, depending on the oriented twist angle. The interplay between this global chirality and additional degrees of freedom, such as…

Mesoscale and Nanoscale Physics · Physics 2022-11-14 Kunihiro Yananose , Paolo G. Radaelli , Mario Cuoco , Jaejun Yu , Alessandro Stroppa

We show that the regime of strong-light matter coupling with remarkable magnetic properties can be realized in systems based on monolayers of chromium triiodide (CrI3). This two-dimensional material combines the presence of ferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2024-05-14 Yaroslav V. Zhumagulov , Salvatore Chiavazzo , Ivan A. Shelykh , Oleksandr Kyriienko

Chromium trihalides (CrX$_3$, with $\rm{X=I,Br,Cl}$) are layered ferromagnetic materials with rich physics and possible applications. Their structure consists of magnetic Cr atoms positioned between two layers of halide atoms. The choice of…

Magnetic skyrmions are nano-scale spin structures that are promising for ultra-dense memory and logic devices. Recent progresses in two-dimensional magnets encourage the idea to realize skyrmionic states in freestanding monolayers. However,…

Materials Science · Physics 2020-02-19 Changsong Xu , Junsheng Feng , Hongjun Xiang , L. Bellaiche
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