Related papers: Strong-field molecular alignment mediated by nonad…
Anisotropy is a fundamental property of particle interactions. It occupies a central role in cold and ultra-cold molecular processes, where long range forces have been found to significantly depend on orientation in ultra-cold polar…
We analytically tackle opto-vibronic interactions in molecular systems driven by either classical or quantum light fields. In particular, we examine a simple model of molecules with two relevant electronic levels, characterized by potential…
We demonstrate that strong-field ionization of atoms driven by circularly polarized light becomes an adiabatic process when described in the frame rotating with the laser field. As a direct consequence, a conservation law emerges: in the…
We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…
Non-resonant light interacting with diatomics via the polarizability anisotropy couples different rotational states and may lead to strong hybridization of the motion. The modification of shape resonances and low-energy scattering states…
We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show…
We present an implementation of a time-dependent multiconfiguration self-consistent-field (TD-MCSCF) method [R. Anzaki et al., Phys. Chem. Chem. Phys. 19, 22008 (2017)] with the full configuration interaction expansion for coupled…
Twisted light (TL), a special kind of light carrying orbital angular momentum, provides a powerful tool for driving symmetry resolved transitions in quantum confined nanostructures. We study a realistic model where a TL pulse excites two…
The impulsive phase of a solar flare is known to generate strong turbulence and to transfer magnetic energy into accelerated electrons. Recognizing the importance of angular diffusion on the dynamics of the accelerated electrons, we extend…
Interaction of an ultrastrong short laser pulse with non-prepolarized near-critical density plasma is investigated in an ultrarelativistic regime, with an emphasis on the radiative spin polarization of ejected electrons. Our…
New emergent states of matter in quantum systems may be created under non-equilibrium conditions if - through many body interactions - its constituents order on a timescale which is shorter than the time required for the system to reach…
The creation of nanoscale lasers that operate above a coherent threshold is a challenging problem. We propose a way to circumvent this issue using systems in which a strong coupling regime is achieved between the light and the active…
Twisted coronal loops should be ubiquitous in the solar corona. Twisted magnetic fields contain excess magnetic energy, which can be released during magnetic reconnection, causing solar flares. The aim of this work is to investigate…
The present work explores quantitative limits to the Single-Active Electron (SAE) approximation, often used to deal with strong-field ionization and subsequent attosecond dynamics. Using a time-dependent multi\-configuration approach,…
We demonstrate strong laser-field-free orientation of absolute-ground-state carbonyl sulfide molecules. The molecules are oriented by the combination of a 485-ps-long non-resonant laser pulse and a weak static electric field. The edges of…
Two mechanisms of two-color (\omega + 2\omega) laser-induced field-free molecular orientation, based on the hyperpolarizability and ionization depletion, are explored and compared. The CO molecule is used as a computational example. While…
In this study, we utilize intense laser pulses and advanced quantum mechanical frameworks to investigate the behavior of high-velocity electrons within magnetized plasma environments. The focus of our research is placed within the context…
The present work reports on the generation of short-pulse coherent extreme ultraviolet radiation of controlled polarization. The proposed strategy is based on high-order harmonics generated in pre-aligned molecules. Field-free molecular…
We use an optical centrifuge to align asymmetric top $\mathrm{SO_2}$ molecules by adiabatically spinning their most polarizable O-O axis. The effective centrifugal potential in the rotating frame confines sulfur atoms to the plane of the…
On the basis of optimal control theory, we numerically study how to optimally manipulate molecular vibrational dynamics by using cycle-averaged polarizability interactions induced by mildly intense non-resonant laser (NR) pulses. As the…