English
Related papers

Related papers: Strong-field molecular alignment mediated by nonad…

200 papers

We theoretically consider the phenomenon of field-free long-lasting orientation of symmetric-top molecules ionized by two-color laser pulses. The anisotropic ionization produces a significant long-lasting orientation of the surviving…

Chemical Physics · Physics 2023-03-08 Long Xu , Ilia Tutunnikov , Yehiam Prior , Ilya Sh. Averbukh

The interaction of a trapped ion with a laser beam in the strong excitation regime is analyzed. In this regime, a variety of non--classical states of motion can be prepared either by using laser pulses of well defined area, or by an…

Quantum Physics · Physics 2009-10-28 J. F. Poyatos , J. I. Cirac , R. Blatt , P. Zoller

The transition between two distinct mechanisms for the laser-induced field-free orientation of CO molecules is observed via measurements of orientation revival times and subsequent comparison to theoretical calculations. In the first…

A moderately intense $450$ fs laser pulse is used to create rotational wave packets in gas phase $\rm{I_2}$ molecules. The ensuing time-dependent alignment, measured by Coulomb explosion imaging with a delayed probe pulse, exhibits the…

We present a theoretical study of the time-dependent laser alignment of molecules taking into account the hyperfine coupling due to nuclear-quadrupole interactions. The coupling of nuclear spins to the overall angular momentum of molecules…

Chemical Physics · Physics 2020-06-18 Linda V. Thesing , Andrey Yachmenev , Rosario González-Férez , Jochen Küpper

We consider a system of two linear and linearly coupled oscillators with ideal impact constraints. Primary resonant energy exchange is investigated by analysis of the slow-flow using the action-angle (AA) formalism. Exact inversion of the…

Chaotic Dynamics · Physics 2018-08-15 Nathan Perchikov , O. V. Gendelman

The interaction of an intense laser pulse with a solid target produces energetic proton and ion beams through the Target Normal Sheath Acceleration (TNSA) mechanism. Such beams are under active investigation for applications in proton beam…

Plasma Physics · Physics 2025-12-25 Vasiliki E. Alexopoulou

Intense single-cycle THz pulses resonantly interacting with molecular rotations are shown to induce significant field-free orientation under ambient conditions. We calculate and measure the angular distribution associated with THz-driven…

Chemical Physics · Physics 2015-05-28 Sharly Fleischer , Yan Zhou , Robert W. Field , Keith A. Nelson

We present a detailed experimental and theoretical study on the relativistic non-dipole effects in strong-field atomic ionisation by near-infrared linearly-polarised few-cycle laser pulses in the intensity range 1014 -1015 W/cm2. We record…

The nondipole under-the-barrier dynamics of the electron during strong-field tunneling ionization is investigated, examining the role of the Coulomb field of the atomic core. The common analysis in the strong field approximation is…

Atomic Physics · Physics 2022-04-06 Pei-Lun He , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

In high energy heavy-ion collisions the magnetic field is very strong right after the nuclei penetrate each other and a non-equilibrium system of quarks and gluons builds up. Even though quarks might not be very abundant initially, their…

High Energy Physics - Phenomenology · Physics 2017-07-12 Moritz Greif , Carsten Greiner , Zhe Xu

Strong optical pulses at mid-infrared and terahertz frequencies have recently emerged as a powerful tool to manipulate and control the solid state and especially complex condensed matter systems with strongly correlated electrons. The…

Strongly Correlated Electrons · Physics 2016-08-22 Daniele Nicoletti , Andrea Cavalleri

Polaritons have gained significant attention for the tantalizing possibility of modifying chemical properties and dynamics by coupling molecules to resonant cavity modes to create hybrid light-matter quantum states. Herein, we implement the…

Chemical Physics · Physics 2025-06-24 Scott M. Garner , Xiaosong Li , Sharon Hammes-Schiffer

Microscopic control over polar molecules with tunable interactions would enable realization of novel quantum phenomena. Using an applied electric field gradient, we demonstrate layer-resolved state preparation and imaging of ultracold…

We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…

Quantum Physics · Physics 2022-11-21 Emil J. Zak

Ionization is one of the most fundamental processes in intense laser-matter interaction. It is extremely efficient for clusters in laser fields and often leads to surprisingly high charge states at moderate laser intensities. Here we reveal…

Plasma Physics · Physics 2023-09-26 Xiaohui Gao

A new perspective on how to manipulate molecules by means of very strong laser pulses is emerging with insights from the so-called light-induced potentials, which are the adiabatic potential energy surfaces of molecules severely distorted…

Chemical Physics · Physics 2016-03-03 Bo Y. Chang , Ignacio R. Sola , Seokmin Shin

We analyze, quantum mechanically, the dynamics of ionization with a strong, circularly polarized, laser field. We show that the main source for non-adiabatic effects is connected to an effective barrier lowering due to the laser frequency.…

Atomic Physics · Physics 2014-09-26 Francois Mauger , A. D. Bandrauk

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

Inducing and controlling the ultrafast molecular rotational dynamics using shaped laser fields is essential in numerous applications. Several approaches exist that allow following the coherent molecular motion in real-time, including…