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The experimental investigations of the magnetic interactions in an atomically thin magnetic layer are essential to understand the physics of low-dimensional magnets. The full spectrum of collective magnetic excitations (magnons) would…

Strongly Correlated Electrons · Physics 2024-05-17 Khalil Zakeri , Albrecht von Faber , Arthur Ernst

We investigate the magnetocrystalline anisotropy, critical behavior, and magnetocaloric effect in ferromagnetic-layered Cr$_2$Te$_3$. We have studied the critical behavior around the Curie temperature ($T_C$) using various techniques,…

Materials Science · Physics 2024-07-26 Shubham Purwar , Tushar Kanti Bhowmik , Soumya Ghorai , Setti Thirupathaiah

Following the recent isolation of monolayer CrI3, there has been a surge of new two-dimensional van der Waals magnetic materials, whose incorporation in van der Waals heterostructures offers a new platform for spintronics, proximity…

We use a first-principles calculations approach to reveal the electronic and magnetic properties of chromium diiodide (CrI$_2$) bilayers and establish a hierarchy of magnetic interactions across stable registries. The monolayer presents a…

Materials Science · Physics 2025-12-23 B. Valdés-Toro , I. Ferreira-Araya , R. A. Gallardo , J. W. González

Neutron spectroscopy measurements have been performed on single crystals of the antiferromagnetic van der Waals compound NiPS$_3$. Linear spin wave theory using a Heisenberg Hamiltonian with single-ion anisotropies has been applied to…

Strongly Correlated Electrons · Physics 2022-12-19 A. R. Wildes , J. R. Stewart , M. D. Le , R. A. Ewings , K. C. Rule , G. Deng , K. Anand

We analyze magnetic properties of monolayers and bilayers of chromium trihalides, CrI$_3$, in two different stacking configurations: AA and rhombohedral ones. Our main focus is on the corresponding Curie temperatures, hysteresis curves,…

Mesoscale and Nanoscale Physics · Physics 2024-04-25 S. Stagraczynski , P. Balaz , M. Jafari , J. Barnas , A. Dyrdal

We investigate the far-from-equilibrium nature of magnetic anisotropy and exchange interactions between molecular magnets embedded in a tunnel junction. By mapping to an effective spin model, these magnetic interactions can be divided into…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 Jonas Fransson , Jie Ren , Jian-Xin Zhu

Using density functional theory combined with a Hubbard model (DFT+U ), the electronic band structure of CrI3 multilayers, both free-standing and enclosed between graphene contacts, is calculated. We show that the DFT+U approach, together…

Materials Science · Physics 2020-10-21 Soumyajit Sarkar , Peter Kratzer

In this report we review the method of explicit calculations of interatomic exchange interactions of magnetic materials. This involves exchange mechanisms normally referred to as Heisenberg exchange, Dzyaloshinskii-Moriya interaction and…

Comprehensive studies of magnetic properties of GdCr3(BO3)4 single crystal have been carried out. The integrals of intrachain and interchain exchange interactions in the chromium subsystem have been determined and the strength of Cr-Gd…

We investigate antiferromagnetic spin chains, which are coupled by a weak antiferromagnetic exchange interaction on a hexagonal lattice. We particulary study the role of the dipole-dipole interaction within the framework of a Heisenberg…

Statistical Mechanics · Physics 2009-10-31 M. Hummel , C. Pich , F. Schwabl

The development of room-temperature magnetic semiconductors is critical for advancing spintronic technologies, yet van der Waals magnets like CrI3 exhibit intrinsically low Curie temperatures (Tc = 45 K). This study employs first-principles…

Materials Science · Physics 2025-08-12 Qing-Han Yang , Jia-Wen Li , Xin-Wei Yi , Xiang Li , Jing-Yang You , Gang Su , Bo Gu

Magneto-optical effect refers to a rotation of polarization plane, which has been widely studied in traditional ferromagnetic metal and insulator films and scarcely in two-dimensional layered materials. Here we uncover a new nonreciprocal…

We present a detailed study on the microscopic origin of magnetism in suspended and dielectrically embedded CrI$_3$ monolayer. To this end, we down-fold two distinct minimal generalized Hubbard models with different orbital basis sets from…

Strongly Correlated Electrons · Physics 2021-10-06 D. Soriano , A. N. Rudenko , M. I. Katsnelson , M. Rösner

The moir\'e engineering of two-dimensional magnets opens unprecedented opportunities to design novel magnetic states with promises for spintronic device applications. The possibility of stabilizing skyrmions in these materials without…

Materials Science · Physics 2022-08-03 Doried Ghader , Bilal Jabakhanji , Alessandro Stroppa

After the discovery of magnetism in monolayer CrI3, the magnetic properties of different 2D materials from the chromium-trihalide family are intuitively assumed to be similar, yielding magnetic anisotropy from the spin-orbit coupling on…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 C. Bacaksiz , D. Šabani , R. M. Menezes , M. V. Milošević

The scenario of a metal-insulator transition driven by the onset of antiferromagnetic order in NaOsO$_3$ calls for a trustworthy derivation of the underlying effective spin Hamiltonian. To determine the latter we rely on {\it ab initio}…

The latest discovery of ferromagnetism in atomically thin films of semiconductors Cr$_2$Ge$_2$Te$_6$ and CrI$_3$ has unleashed numerous opportunities for fundamental physics of magnetism in two-dimensional (2D) limit and also for…

Mesoscale and Nanoscale Physics · Physics 2019-05-09 Vijay Kumar Gudelli , Guang-Yu Guo

A recent theoretical study reported large effects of perpendicular electric fields on the atomic structure of a monolayer CrI3, which could be related to the microscopic origin of the technologically promising and experimentally observed…

Materials Science · Physics 2019-07-24 S. Ghosh , N. Stojic , N. Binggeli

We present a model of equal spin $s_1$ dimer single molecule magnets. The spins within each dimer interact via the Heisenberg and the most general set of four quadratic anisotropic spin interactions with respective strengths $J$ and…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Dmitri V. Efremov , Richard A. Klemm