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Traditional thermoelectric materials rely on low thermal conductivity to enhance their efficiency but suffer from inherently limited power factors. Novel pathways to optimize electronic transport are thus crucial. Here, we achieve ultrahigh…

We have revisited the electronic structure of infinite-layer RNiO$_2$ (R= La, Nd) in light of the recent discovery of superconductivity in Sr-doped NdNiO$_2$. From a comparison to their cuprate counterpart CaCuO$_2$, we derive essential…

Superconductivity · Physics 2020-02-05 Antia S. Botana , Michael R. Norman

We investigate the structural and electronic conditions conducive to superconductivity in layered nickelates using density functional theory with Hubbard corrections (DFT+$U$). For both the bilayer and 1-3 polymorphs of La$_3$Ni$_2$O$_7$,…

Superconductivity · Physics 2025-06-16 Bipasa Samanta , Alexandru B. Georgescu

The relationship between the long-range antiferromagnetic order in cuprates and the high-temperature superconductivity in these compounds represents unresolved, nearly four-decades long scientific problem. Because recently discovered…

Superconductivity · Physics 2023-09-21 E. F. Talantsev

For layered materials, the interlayer stacking is a critical degree of freedom tuning electronic properties, while its microscopic characterization faces great challenges. The transition-metal dichalcogenide 1T-TaS$_2$ represents a novel…

Materials Science · Physics 2025-08-01 Li Cheng , Linpeng Nie , Xuanyu Long , Li Liang , Dan Zhao , Jian Li , Zheng Liu , Tao Wu , Xianhui Chen , Xiaolong Zou

The recent discovery of ambient-pressure superconductivity in thin-film bilayer nickelates opens new possibilities for investigating electronic structures in this new class of high-transition temperature $T_C$ superconductors. Here, we…

We report the synthesis of infinite-layer LaNiO2 thin films by metal organic decomposition. Our work is aimed to synthesize perovskite-like oxides with 3d9 electronic configuration, which is common to high-Tc copper oxides. The 3d9…

Superconductivity · Physics 2015-05-13 D. Kaneko , K. Yamagishi , A. Tsukada , T. Manabe , M. Naito

Effective models are constructed for a newly discovered superconductor (Nd,Sr)NiO2, which has been considered as a possible nickelate analogue of the cuprates owing to the d9 electron configuration. Estimation of the effective interaction,…

Superconductivity · Physics 2020-08-14 Hirofumi Sakakibara , Hidetomo Usui , Katsuhiro Suzuki , Takao Kotani , Hideo Aoki , Kazuhiko Kuroki

Recent discovery of superconductivity in the doped infinite-layer nickelates has renewed interest in understanding the nature of high-temperature superconductivity more generally. The low-energy electronic structure of the parent compound…

We study the normal state electronic structure of the recently discovered infinite-layer nickelate superconductor, Nd$_{1-x}$Sr$_x$NiO$_2$. Using SrNiO$_2$ as a reference, we find that Nd$_{1-x}$Sr$_x$NiO$_2$ is a multi-orbital electronic…

Strongly Correlated Electrons · Physics 2020-11-04 Y. Wang , C. -J. Kang , H. Miao , G. Kotliar

The intensive search for alternative non-cuprate high-transition-temperature ($T_c$) superconductors has taken a positive turn recently with the discovery of superconductivity in infinite layer nickelates. This discovery is expected to be…

The correlated electronic structure of the infinite-layer compounds NdNiO$_2$ and SrCuO$_2$ at stoichiometry and with finite hole doping is compared. Key differences are elucidated from an advanced first-principles many-body perspective.…

Strongly Correlated Electrons · Physics 2020-03-06 Frank Lechermann

The recently discovered infinite-layer nickelates show great promise in helping to disentangle the various cooperative mechanisms responsible for high-temperature superconductivity. However, lack of antiferromagnetic order in the pristine…

Strongly Correlated Electrons · Physics 2022-08-18 Christopher Lane , Ruiqi Zhang , Bernardo Barbiellini , Robert S. Markiewicz , Arun Bansil , Jianwei Sun , Jian-Xin Zhu

We report a determinant quantum Monte Carlo study of a two-band model, inspired by infinite-layer nickelates, focusing on the influence of interlayer hybridization between $3d_{x^2-y^2}$ orbitals derived from Ni (or Ni and O) in one layer…

Strongly Correlated Electrons · Physics 2024-06-10 Fangze Liu , Cheng Peng , Edwin W. Huang , Brian Moritz , Chunjing Jia , Thomas P. Devereaux

Following the successful prediction of the superconducting phase diagram for infinite-layer nickelates, here we calculate the superconducting $T_{\mathrm{c}}$ vs. the number of layers $n$ for finite-layer nickelates using the dynamical…

Strongly Correlated Electrons · Physics 2025-07-23 Andreas Hausoel , Simone Di Cataldo , Motoharu Kitatani , Oleg Janson , Karsten Held

Motivated by the recent discovery of superconductivity in the pentalayer nickelate Nd$_6$Ni$_5$O$_{12}$ [Nature Materials 10.1038], we calculate its electronic structure and superconducting critical temperature. We find that electronic…

Superconductivity · Physics 2022-09-08 Paul Worm , Liang Si , Motoharu Kitatani , Ryotaro Arita , Jan M. Tomczak , Karsten Held

We provide a set of computational experiments based on \textit{ab initio} calculations to elucidate whether a cuprate-like antiferromagnetic insulating state can be present in the phase diagram of the low-valence layered nickelate family…

Superconductivity · Physics 2022-03-04 Myung-Chul Jung , Harrison LaBollita , Victor Pardo , Antia S. Botana

Conflicting theoretical scenarios for infinite-layer nickelate superconductors have been hotly debated, particularly regarding whether {only} a single Ni-3$d_{x^2-y^2}$ band is relevant at low energies besides electron pockets or whether…

The status of nickelate superconductors in relation to cuprate high temperature superconductors is one of the concepts being discussed in high temperature superconductivity in correlated transition metal oxides. New additions to the class…

Strongly Correlated Electrons · Physics 2022-04-14 Hyo-Sun Jin , W. E. Pickett , K. -W. Lee

Superconducting nickelates are a new family of strongly correlated electron materials with a phase diagram closely resembling that of superconducting cuprates. While analogy with the cuprates is natural, very little is known about the…

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