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The pyrochlore metal Cd2Re2O7 has been recently investigated by second-harmonic generation (SHG) reflectivity. In this paper, we develop a general formalism that allows for the identification of the relevant tensor components of the SHG…

Strongly Correlated Electrons · Physics 2017-10-04 S. Di Matteo , M. R. Norman

Single crystal X-ray diffraction measurements have been carried out on Cd_2Re_2O_7 near and below the phase transition it exhibits at Tc' ~195 K. Cd_2Re_2O_7 was recently discovered as the first, and to date only, superconductor with the…

Strongly Correlated Electrons · Physics 2009-11-07 J. P. Castellan , B. D. Gaulin , J. van Duijn , M. J. Lewis , M. D. Lumsden , R. Jin , J. He , S. E. Nagler , D. Mandrus

Evidence for another phase transition at 120 K in the metallic pyrochlore oxide Cd2Re2O7, following the structural transition at 200 K and followed by the superconducting transition at 1.0 K, is given through resistivity, magnetoresistance,…

Strongly Correlated Electrons · Physics 2009-11-07 Zenji Hiroi , Jun-Ichi Yamaura , Yuji Muraoka , Masafumi Hanawa

It is shown that both structural phase transitions in Cd2Re2O7, which occur at T_{s1}=200 K and T_{s2}=120 K, are due to an instability of the Re tetrahedral network with respect to the same doubly degenerate long-wavelength phonon mode.…

Superconductivity · Physics 2009-11-10 I. A. Sergienko , S. H. Curnoe

The 5d-transition metal pyrochlore oxide Cd2Re2O7, which was recently suggested to be a prototype of the spin-orbit-coupled metal [Phys. Rev. Lett. 115, 026401 (2015)], exhibits an inversion-symmetry breaking (ISB) transition at 200 K and a…

Strongly Correlated Electrons · Physics 2017-01-13 Jun-ichi Yamaura , Keiki Takeda , Yoichi Ikeda , Naohisa Hirao , Yasuo Ohishi , Tatsuo C. Kobayashi , Zenji. Hiroi

A chain of singly-charged particles, confined by a harmonic potential, exhibits a sudden transition to a zigzag configuration when the radial potential reaches a critical value, depending on the particle number. This structural change is a…

Statistical Mechanics · Physics 2009-11-13 Shmuel Fishman , Gabriele De Chiara , Tommaso Calarco , Giovanna Morigi

The superconducting pyrochlore oxide Cd2Re2O7 (Tc = 1 K), which is now considered as a candidate of the spin-orbit-coupled metal, shows an inversion-symmetry-breaking structural transition at Ts1 = 200 K. Ts1 decreases with increasing…

Strongly Correlated Electrons · Physics 2018-04-30 Yasuhito Matsubayashi , Takumi Hasegawa , Norio Ogita , Jun-ichi Yamaura , Zenji Hiroi

The structural, electronic, and optical properties of pyrochlore-type Pb$_{2}$Ir$_{2}$O$_{6}$O'$_{0.55}$, which is a metal without spatial inversion symmetry at room temperature, were investigated. Structural analysis revealed that the…

The unusual 2-stage spin flop transition in BaCu2Si2O7 is studied by single-crystal neutron diffraction. The magnetic structures of the various spin-flop phases are determined. The results appear to be inconsistent with the previously…

Strongly Correlated Electrons · Physics 2009-11-07 A. Zheludev , E. Ressouche , I. Tsukada , T. MasudaK. Uchinokura

Ferroelectric materials contain a switchable spontaneous polarization that persists even in the absence of an external electric field. The coexistence of ferroelectricity and metallicity in a material appears to be illusive, since…

We report the X-ray study for the pyrochlore oxide Cd2Re2O7. Two symmetry-lowering structural transitions were observed at Ts1=200K and Ts2=120K. The former is of the second order from the ideal cubic pyrochlore structure with space group…

Strongly Correlated Electrons · Physics 2009-11-07 Jun-Ichi Yamaura , Zenji Hiroi

Understanding the mechanisms and spatial correlations of crystallographic symmetry breaking in ferroelectric materials is essential to tuning their functional properties. While optical second harmonic generation (SHG) has long been utilized…

Materials Science · Physics 2022-08-10 Wei Li , Yunpeng Ma , Tianyi Feng , Sergei V. Kalinin , Jing-Feng Li , Qian Li

RuO$_2$ was considered for a long time to be a paramagnetic metal with an ideal rutile-type structure down to low temperatures, but recent studies on single-crystals claimed evidence for antiferromagnetic order and some symmetry breaking in…

The notion of spontaneous symmetry breaking has been used to describe phase transitions in a variety of physical systems. In crystalline solids, the breaking of certain symmetries, such as mirror symmetry, is difficult to detect…

Materials Science · Physics 2020-07-01 Bryan T. Fichera , Anshul Kogar , Linda Ye , Bilal Gökce , Alfred Zong , Joseph G. Checkelsky , Nuh Gedik

We describe the low temperature behaviour of the magnetic susceptibility of Cd2Re2O7 in terms of a Landau theory of structural phase transitions. We calculate the zero temperature Pauli susceptibility using a tight-binding approach to…

Superconductivity · Physics 2007-05-23 I. A. Sergienko , S. H. Curnoe

The bandstructure was calculated by the full-potential linearized augmented plane wave method. The result reveals two important insights to the novel second harmonic generation (SHG) of alpha-phase lithium iodate ($\alpha-LiIO_{3}$)…

Optics · Physics 2007-05-23 Yung-mau Nie

We report a structural phase transition found at Ts = 200 K in a pyrochlore oxide Cd2Re2O7 which shows superconductivity at Tc = 1.0 K. X-ray diffractionexperiments indicate that the phase transition is of the second order, from a…

Superconductivity · Physics 2009-11-07 M. Hanawa , J. Yamaura , Y. Muraoka , F. Sakai , Z. Hiroi

A Landau theory is presented for the structural transition of electrically stabilized colloidal crystals under shear. The model suggests that a structural transition from an ordered layered colloidal crystal into a disordered structure…

Materials Science · Physics 2013-12-31 Joachim Kaldasch , Bernhard Senge , Jos Laven

The controlled assembly of twisted 2D structures requires precise determination of the crystal orientation of their component layers. In the established procedure, the second-harmonic generation (SHG) intensity of a noncentrosymmetric layer…

Inversion symmetry breaking is critical for many quantum effects and fundamental for spin-orbit torque, which is crucial for next-generation spintronics. Recently, a novel type of gigantic intrinsic spin-orbit torque has been established in…

Materials Science · Physics 2025-01-09 Kai-Xuan Zhang , Hwiin Ju , Hyuncheol Kim , Jingyuan Cui , Jihoon Keum , Je-Geun Park , Jong Seok Lee
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