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Hot carriers produced from the decay of localized surface plasmons in metallic nanoparticles are intensely studied because of their optoelectronic, photovoltaic and photocatalytic applications. From a classical perspective, plasmons are…

Mesoscale and Nanoscale Physics · Physics 2019-04-09 Lara Román Castellanos , Ortwin Hess , Johannes Lischner

Harvesting non-equilibrium hot carriers from photo-excited metal nanoparticles has enabled plasmon-driven photochemical transformations and tunable photodetection with resonant nanoantennas. Despite numerous studies on the ultrafast…

Exploring nonequilibrium hot carriers from plasmonic metal nanostructures is a dynamic field in optoelectronics, driving photochemical reactions such as solar fuel generation. The hot carrier injection mechanism and the reaction rate are…

Photoinduced ultrafast phenomena in materials exhibiting nonequilibrium behavior can lead to the emergence of exotic phases beyond the limits of thermodynamics, presenting opportunities for femtosecond photoexcitation. Despite extensive…

Localized plasmons formed in ultrathin metallic nanogaps can lead to robust absorption of incident light. Plasmonic metasurfaces based on this effect can efficiently generate energetic charge carriers, also known as hot electrons, owing to…

Optics · Physics 2022-09-28 Larousse Khosravi Khorashad , Christos Argyropoulos

We propose a model accounting for plasmons within a two temperature description, to investigate the role of surface plasmon polaritons (SPP) in the energy redistribution between laser excited electrons and the lattice, leading to surface…

Mesoscale and Nanoscale Physics · Physics 2021-11-10 Othmane Benhayoun , P. N. Terekhin , Dmitry Ivanov , Bärbel Rethfeld , Martin Garcia

Nanoscale localization of electromagnetic fields near metallic nanostructures underpins the fundamentals and applications of plasmonics. The unavoidable energy loss from plasmon decay, initially seen as a detriment, has now expanded the…

Heterogeneous catalysis of adsorbates on metallic surfaces mediated by plasmon has potential high photoelectric conversion efficiency and controllable reaction selectivity. Theoretical modeling of dynamical reaction processes provides…

Chemical Physics · Physics 2023-06-05 Xiaoyan Wu , Tammo van der Heide , Thomas Frauenheim , Sergei Tretiak , ChiYung Yam , Yu Zhang

Hot electrons generated from the decay of localized surface plasmons in metallic nanostructures have the potential to transform photocatalysis, photodetection and other optoelectronic applications. However, the understanding of hot-carrier…

Harnessing hot electrons and holes resulting from the decay of localized surface plasmons in nanomaterials has recently led to new devices for photovoltaics, photocatalysis and optoelectronics. Properties of hot carriers are highly tunable…

Materials Science · Physics 2018-02-15 Stefano Dal Forno , Luigi Ranno , Johannes Lischner

Electron-electron scattering is one of the most important hot carrier relaxation pathways in plasmonic nanoparticles. Understanding the dynamics of this scattering process and the effects of this on excited state dephasing and relaxation is…

Chemical Physics · Physics 2026-03-09 Yanze Wu , George C. Schatz

When plasmonic nanoparticles are coupled with semiconductors, highly energetic hot carriers can be extracted from the metal-semiconductor interface for various applications in light energy conversion. Hot charge-carrier extraction upon…

Hot carrier spatial and momentum distributions in nanoplasmonic systems depend sensitively on the optical excitation parameters and nanoscale geometry, which therefore determine the efficiency and functionality of plasmon-enhanced…

Mesoscale and Nanoscale Physics · Physics 2021-02-03 Jacob Pettine , Sean M. Meyer , Fabio Medeghini , Catherine J. Murphy , David J. Nesbitt

Surface plasmon enhanced processes and hot-carrier dynamics in plasmonic nanostructures are of great fundamental interest to reveal light-matter interactions at the nanoscale. Using plasmonic tunnel junctions as a platform supporting both…

We theoretically investigate equilibrium behaviors and photothermal effects of a flexible plasmonic metamaterial composed of aramid nanofibers and gold nanoparticles. The fiber matrix is considered as an external field to reconfigure a…

Mesoscale and Nanoscale Physics · Physics 2020-11-12 Anh D. Phan , Vu D. Lam , Katsunori Wakabayashi

In the present paper, the collective near-field effects in a two-graphene sheets plasmonic waveguide loaded with an array of Ag$_2$Se quantum dots excited by external radiation are theoretically studied. This research aims to develop a…

Mesoscale and Nanoscale Physics · Physics 2021-10-07 M. Yu. Gubin , A. V. Prokhorov , V. S. Volkov , A. B. Evlyukhin

The generation of the localized surface plasmon resonance (LSPR) on the surface of plasmonic structures in the nanoscale has paved the way for advanced biosensing, surpassing the conventional detection limits. The electric field enhancement…

Optics · Physics 2023-12-12 Siddhartha Banerjee , Jolly Xavier

Using ultrafast pump-probe reflectivity with 3.1 eV pump and coherent white light probe (1.1 to 2.6 eV), we show that graphene on gold nanostructures exhibits a strong coupling to the plasmonic resonances of the ordered lattice hole array,…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Gyan Prakash , Rajesh Kumar Srivastava , Satyendra Nath Gupta , A. K. Sood

Understanding the interplay between illumination and the electron distribution in metallic nanostructures is a crucial step towards developing applications such as plasmonic photo-catalysis for green fuels, nano-scale photo-detection and…

Optics · Physics 2019-07-23 Yonatan Dubi , Yonatan Sivan

Collective excitations in topologically non-trivial systems have attracted considerable attention in recent years. Here we study plasmons in the Su-Schrieffer-Heeger model whose low-energy electronic band is only partially filled, such that…

Materials Science · Physics 2021-07-28 Zhihao Jiang , Henning Schlömer , Stephan Haas