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We calculate the crystal-field splitting, ground-state Kramers doublet and intersite exchange interactions within the ground-state doublet manifold using an ab initio Hubbard-I based approach for a representative set of Ce and Yb…

Strongly Correlated Electrons · Physics 2026-02-06 Leonid V. Pourovskii , Rafael D. Soares , Alexander Wietek

The spiral spin liquid (SSL) is a highly degenerate state characterized by a continuous contour or surface in reciprocal space spanned by a spiral propagation vector. Although the SSL state has been predicted in a number of various…

Quantum spin liquid (QSL) state in rare-earth triangular lattice has attracted much attention recently due to its potential application in quantum computing and communication. Here we report the single-crystal growth synthesis, crystal…

Strongly Correlated Electrons · Physics 2021-11-16 Jie Xing , Liurukara D. Sanjeewa , Andrew F. May , Athena S. Sefat

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

Strongly Correlated Electrons · Physics 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa

A quantum spin liquid (QSL) is a state of matter where unpaired electrons' spins in a solid are quantum entangled, but do not show magnetic order in the zero-temperature limit. Because such a state may be important to the microscopic origin…

Ytterbium-based delafossites with effective S=1/2 moments are investigated intensively as candidates for quantum spin-liquid ground states. While the synthesis of related cerium compounds has also been reported,many important details…

Strongly Correlated Electrons · Physics 2020-12-25 M. S. Eldeeb , T. Petersen , L. Hozoi , V. Yushankhai , U. K. Rossler

Quantum spin liquids (QSLs) represent a novel state of matter in which quantum fluctuations prevent conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many…

Strongly Correlated Electrons · Physics 2018-10-11 Zhen Ma , Kejing Ran , Jinghui Wang , Song Bao , Zhengwei Cai , Shichao Li , Jinsheng Wen

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

A quantum spin liquid (QSL) is an exotic quantum state of matter characterized by fluctuating spins which may exhibit long-range entanglement. Among the possible host candidates for a QSL ground state, the $S$=1/2 kagome lattice…

We study the ground-state properties of the quantum spin liquid (QSL) phases of the spin-$1/2$ antiferromagnetic Heisenberg model on the triangular lattice with nearest- ($J_1$), next-nearest- ($J_2$), and third-neighbor ($J_3$)…

Strongly Correlated Electrons · Physics 2023-05-10 Yi-Fan Jiang , Hong-Chen Jiang

The existence of a quantum spin liquid (QSL) in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its…

We report discovery of a new iridate family K$_x$Ir$_y$O$_2$ with depleted triangular lattice planes made up of edge sharing IrO$_6$ octahedra separated by K planes. Such a material interpolates between the triangular and honeycomb lattices…

Strongly Correlated Electrons · Physics 2019-08-23 Kavita Mehlawat , Yogesh Singh

The three-dimensional $S = {\frac{1}{2}}$ system Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$ consists of two inequivalent Cu$^{2+}$ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility $\chi(T)$, specific heat $C_p(T)$,…

We report a comprehensive investigation of the magnetism of the $S$ = 3/2 triangular-lattice antiferromagnet, $\alpha$-CrOOH(D) (delafossites green-grey powder). The nearly Heisenberg antiferromagnetic Hamiltonian ($J_1$ $\sim$ 23.5 K) with…

Strongly Correlated Electrons · Physics 2021-05-04 Jiabin Liu , Benqiong Liu , Long Yuan , Boqiang Li , Lei Xie , Xiping Chen , Hongxia Zhang , Daye Xu , Wei Tong , Jinchen Wang , Yuesheng Li

A layered triangular lattice with spin-1/2 ions is an ideal platform to explore highly entangled exotic states like quantum spin liquid (QSL). Here, we report a systematic in-field neutron scattering study on a perfect two-dimensional…

Strongly Correlated Electrons · Physics 2024-07-18 Tao Xie , Jie Xing , S. E. Nikitin , S. Nishimoto , M. Brando , P. Khanenko , J. Sichelschmidt , L. D. Sanjeewa , Athena S. Sefat , A. Podlesnyak

Quantum spin liquid (QSL) is a novel state of matter with exotic excitations and was theoretically predicted to be realized most possibly in an S=1/2 kagome antiferromagnet. Experimentally searching for the candidate materials is a big…

Strongly Correlated Electrons · Physics 2014-09-15 Yuesheng Li , Bingying Pan , Shiyan Li , Wei Tong , Langsheng Ling , Zhaorong Yang , Junfeng Wang , Zhongjun Chen , Zhonghua Wu , Qingming Zhang

Based on experimental data and our theoretical analysis, we provide a strategy for unambiguous establishing of gapless quantum spin liquid state (QSL) in herbertsmithite and other materials. To clarify the nature of QSL, we recommend…

One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…

Strongly Correlated Electrons · Physics 2023-01-10 Chengpeng Tu , Dongzhe Dai , Xu Zhang , Chengcheng Zhao , Xiaobo Jin , Bin Gao , Tong Chen , Pengcheng Dai , Shiyan Li

A spinel related oxide, Na4Ir3O8, was found to have a three dimensional network of corner shared Ir4+ (t2g^5) triangles. This gives rise to an antiferromagnetically coupled S = 1/2 spin system formed on a geometrically frustrated…

Strongly Correlated Electrons · Physics 2009-11-13 Yoshihiko Okamoto , Minoru Nohara , Hiroko Aruga-Katori , Hidenori Takagi

Quantum spin liquids (QSLs) represent highly entangled states of matter in which frustration-induced quantum fluctuations suppress any symmetry-breaking phase transition down to absolute zero, giving rise to fractionalized excitations and…