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The antiferromagnetic compound Ba(TiO)Cu$_4$(PO$_4$)$_4$ contains square cupola of corner-sharing CuO$_4$ plaquettes, which were proposed to form effective quadrupolar order. To identify the magnetic structure, we have performed spherical…

Strongly Correlated Electrons · Physics 2018-01-03 P. Babkevich , L. Testa , K. Kimura , T. Kimura , G. S. Tucker , B. Roessli , H. M. Rønnow

The structural and magnetic properties of the square-cupola antiferromagnet Sr(TiO)Cu$_{4}$(PO$_{4}$)$_{4}$ are investigated via x-ray diffraction, magnetization, heat capacity, and $^{31}$P nuclear magnetic resonance experiments on…

Materials Science · Physics 2018-07-04 S. S. Islam , K. M. Ranjith , M. Baenitz , Y. Skourski , A. A. Tsirlin , R. Nath

We report a comprehensive NMR study of the chiral square-cupola antiferromagnet Pb(TiO)Cu$_4$(PO$_4$)$_4$ and compare its microscopic hyperfine and local-field parameters with the Ba/Sr analogues in the $A$(TiO)Cu$_4$(PO$_4$)$_4$ family.…

Strongly Correlated Electrons · Physics 2026-05-11 Riho Rästa , Ivo Heinmaa , Joosep Link , Yusuke Kousaka , Tsuyoshi Kimura , Yoshihiko Ihara , Kenta Kimura , Raivo Stern

The square cupola antiferromagnet Pb(TiO)Cu$_4$(PO$_4$)$_4$ exhibits the intriguing magnetoelectric responses arising from the consecutive change in the magnetic quadrupolar-type configuration of magnetic moments under external magnetic…

Strongly Correlated Electrons · Physics 2025-08-19 Y. Ihara , T. Kanda , Y. Kato , Y. Motome , K. Matsui , K. Kindo , Y. Kohama , T. Kimura , K. Kimura

We report our combined experimental and theoretical study of magnetoelectric properties of an antiferromagnet Sr(TiO)Cu$_4$(PO$_4$)$_4$, in comparison with the isostructurals Ba(TiO)Cu$_4$(PO$_4$)$_4$ and Pb(TiO)Cu$_4$(PO$_4$)$_4$. The…

We perform a combined experimental and theoretical study of a magnetic-field ($B$) induced evolution of magnetic and ferroelectric properties in an antiferromagnetic material Pb(TiO)Cu$_4$(PO$_4$)$_4$, whose structure is characterized by a…

We present the synthesis and a detailed investigation of structural and magnetic properties of polycrystalline Ba(TiO)Cu$_{4}$(PO$_{4}$)$_{4}$ (BTCPO) via x-ray diffraction, magnetic susceptibility, heat capacity, and $^{31}$P Nuclear…

Strongly Correlated Electrons · Physics 2019-09-17 Vinod Kumar , Aga Shahee , S. Kundu , M. Baenitz , A. V. Mahajan

We report high-resolution single-crystal inelastic neutron scattering measurements on the spin-1/2 antiferromagnet Ba(TiO)Cu$_4$(PO$_4$)$_4$. This material is formed from layers of four-site \cupola" structures, oriented alternately upwards…

The chain-like system Ba_{3}Cu_{3}Sc_4O_{12} has potentially interesting magnetic properties due to the presence of Cu^{2+} and a structure-suggested low-dimensionality. We present magnetization M versus magnetic field H and temperature T,…

Strongly Correlated Electrons · Physics 2012-11-16 B. Koteswararao , A. V. Mahajan , F. Bert , P. Mendels , J. Chakraborty , V. Singh , I. Dasgupta , S. Rayaprol , V. Siruguri , A. Hoser , S. D. Kaushik

Depending on the crystal growth conditions, an orthorhombic (O-type) or a tetragonal (T-type) structure can be found in the solid solution Cs2CuCl4-xBrx (0 < x < 4). Here we present measurements of the temperature-dependent magnetic…

We report results of 14N-NMR experiments on NH4CuCl3 at the magnetic field of 7 T, where the 1/4-magnetization plateau is observed at low temperatures. The quadrupole splitting parameter $\nu_{z}$ splits below 70 K, indicating a structural…

Strongly Correlated Electrons · Physics 2015-06-24 Katsuaki Kodama , Masashi Takigawa , Yoshiyuki Shimaoka , Hidekazu Tanaka

The magnetic, dielectric and structural properties of type-I multiferroic KNiPO$_4$ have been investigated by neutron powder diffraction, magnetization, dielectric and high temperature synchrotron-XRD measurements. Below the N\'{e}el…

Strongly Correlated Electrons · Physics 2022-07-15 Alexandre Pages , Jian-Rui Soh , Marjaneh Jafari Fesharaki , Henrik M. Ronnow , Hossein Ahmadvand

A detailed investigation of Ba$_2$MnGe$_2$O$_7$ was performed in its low-temperature magnetoelectric state combining neutron diffraction with magnetization measurements on single crystals. In the paramagnetic state at 10 K, polarized…

Strongly Correlated Electrons · Physics 2023-03-07 A. Sazonov , H. Thoma , R. Dutta , M. Meven , A. Gukasov , R. Fittipaldi , V. Granata , T. Masuda , B. Náfrádi , V. Hutanu

We report a detailed study of the ground state helical magnetic structure in monophosphide FeP by means of ${}^{31}$P NMR spectroscopy. We show that the zero-field NMR spectrum of the polycrystalline sample provides strong evidence of an…

The magnetic structure of (La${}_{1.8}$Eu${}_{0.2}$)CuO${}_4$ has been studied by magnetization measurements of single crystals, which show antiferromagnetic long-range order below $T_N$ = 265 K and a structural phase transition at $T_s$ =…

Superconductivity · Physics 2009-11-07 I. Tsukada , X. F. Sun , Seiki Komiya , A. N. Lavrov , Yoichi Ando

We report the single-crystal X-ray analysis and magnetic properties of a new double-layered perovskite antiferromagnet, Cs$_3$Cu$_2$Cl$_4$Br$_3$. This structure is composed of Cu$_2$Cl$_4$Br$_3$ double layers with elongated CuCl$_4$Br$_2$…

Strongly Correlated Electrons · Physics 2015-06-25 F. Yamada , T. Ono , H. Tanaka , J. Yamaura

We have carried out 63,65Cu NMR spectra measurements in magnetic field up to about 15.5 T on single crystal of a multiferroic triangular-lattice antiferromagnet CuCrO2. The measurements were performed for perpendicular and parallel…

Strongly Correlated Electrons · Physics 2014-12-30 Yu. A. Sakhratov , L. E. Svistov , P. L. Kuhns , H. D. Zhou , A. P. Reyes

Cubic spinel GeNi2O4 exhibits intriguing magnetic properties with two successive antiferromagnetic phase transitions (TN1 12.1 and TN2 11.4 K) with the absence of any structural transition. We have performed detailed heat capacity and…

Strongly Correlated Electrons · Physics 2020-12-02 T. Basu , T. Zou , Z. Dun , C. Q. Xu , C. R. Dela Cruz , Tao Hong , H. B. Cao , K. M. Taddei , H. D. Zhou , X. Ke

In vortex-like spin arrangements, multiple spins can combine into emergent multipole moments. Such multipole moments have broken space-inversion and time-reversal symmetries, and can therefore exhibit linear magnetoelectric (ME) activity.…

This paper presents results of a recent study of multiferroic \CCO\ by means of single crystal neutron diffraction. This system has two close magnetic phase transitions at $T\nsub{N1}=24.2$ K and $T\nsub{N2}=23.6$ K. The low temperature…

Materials Science · Physics 2015-05-30 M. Frontzek , G. Ehlers , A. Podlesnyak , H. Cao , M. Matsuda , O. Zaharko , N. Aliouane , S. Barilo , S. V. Shiryaev
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