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We formulate a general three-dimensional semiclassical model for the study of correlated multielectron escape during fragmentation of molecules driven by intense infrared laser pulses, while fully accounting for the magnetic field of the…

Atomic Physics · Physics 2023-11-30 Georgios Petros Katsoulis , Matthew Benjamin Peters , Agapi Emmanouilidou

At intensities below-the-recollision threshold, we show that re-collision-induced excitation with one electron escaping fast after re-collision and the other electron escaping with a time delay via a Coulomb slingshot motion is one of the…

Atomic Physics · Physics 2020-02-12 G. P. Katsoulis , A. Hadjipittas , B. Bergues , M. F. Kling , A. Emmanouilidou

We have investigated the energy correlation of the two electrons from nonsequential double ionization of helium atom in 800 nm laser fields at intensities below the recollision threshold by quantum calculations. The circular arcs structure…

Optics · Physics 2011-10-07 Qing Liao , Peixiang Lu

We demonstrate the control of electron-electron correlation in frustrated double ionization (FDI) of the two-electron triatomic molecule D$_{3}^{+}$ when driven by two orthogonally polarized two-color laser fields. We employ a…

Atomic Physics · Physics 2017-09-13 A. Chen , M. F. Kling , A. Emmanouilidou

When intense laser pulses release correlated electrons, the time delay between the ionizations may last more than one laser cycle. We show that this "Recollision-Excitation with Subsequent Ionization" pathway originates from the inner…

Atomic Physics · Physics 2012-02-09 Francois Mauger , Adam Kamor , Cristel Chandre , Turgay Uzer

We investigate the dynamics of the photodissociation of the hydrohelium cation HeH$^+$ by XUV radiation with the aim to establish a detailed comparison with a recent experimental work carried out at the FLASH free electron laser using both…

Atomic Physics · Physics 2015-05-28 J. Loreau , J. Lecointre , X. Urbain , N. Vaeck

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · Physics 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

We study double ionization of He driven by a near-single-cycle laser pulse at low intensities at 400 nm. Using a three-dimensional semiclassical model, we identify the pathways that prevail non-sequential double ionization (NSDI). We focus…

Atomic Physics · Physics 2020-02-12 Georgios Petros Katsoulis , Agapi Emmanouilidou

As opposed to purely molecular systems where electron dynamics proceed only through intramolecular processes, weakly bound complexes such as He droplets offer an environment where local excitations can interact with neighbouring embedded…

Atomic and Molecular Clusters · Physics 2021-04-15 A. C. LaForge , M. Shcherbinin , F. Stienkemeier , R. Richter , R. Moshammer , T. Pfeifer , M. Mudrich

We numerically investigate the dynamics of multiply charged hydrogenic ions in near-optical linearly polarized laser fields with intensities of order 10^16 to 10^17 W/cm^2. Depending on the charge state Z of the ion the relation of strength…

Quantum Physics · Physics 2009-11-06 S. X. Hu , C. H. Keitel

Double photoelectron emission from He atoms by intense laser pulses with a wave length of $394.5\,nm$ is computed for intensities $3.5 - 9.2\times 10^{14}W/cm^2$. Joint momentum distributions confirm the characteristics seen in classical…

Atomic Physics · Physics 2020-07-01 Jinzhen Zhu , Armin Scrinzi

In the recent work of Herath et al. [Phys. Rev. Lett. 109, 043004 (2012)] the first experimental observation of a dependence of strong-field ionization rate on the sign of the magnetic quantum number m (of the initial bound state (n,l.m))…

Atomic Physics · Physics 2015-06-23 J. H. Bauer , Francisca Mota-Furtado , Patrick F. O'Mahony , Bernard Piraux , K. Warda

We study theoretically the fragmentation of the helium dimer, $^4$He$_2$, into singly charged ions in collisions with relativistic highly-charged projectiles. We discuss the main mechanisms driving this process with the focus on the…

Atomic Physics · Physics 2022-06-22 B. Najjari , S. F. Zhang , X. Ma , A. B. Voitkiv

The ionization of H2 in intense laser pulses is studied by numerical integration of the time-dependent Schr\"odinger equation for a single-active-electron model including the vibrational motion. The electron kinetic-energy spectra in…

Atomic Physics · Physics 2009-11-13 Stefan Pieper , Manfred Lein

In this brief review we discuss the transient processes in solids under irradiation with femtosecond X-ray free-electron-laser (FEL) pulses and swift-heavy ions (SHI). Both kinds of irradiation produce highly excited electrons in a target…

Materials Science · Physics 2017-03-06 N. Medvedev , A. E. Volkov , B. Ziaja

Ionization, excitation, and de-excitation to the ground state is studied theoretically for the first excited singlet state B $^1\Sigma_u^+$ of H$_2$ exposed to intense laser fields with photon energies in between about 3 eV and 13 eV. A…

Atomic Physics · Physics 2015-05-18 Manohar Awasthi , Alejandro Saenz

High-order harmonic generation (HHG) from molecular ion HeH$^{2+}$ in two initial states of $1s\sigma$ (ground state) and $2p\sigma$ (first excited state) is investigated theoretically, in homogeneous and plasmonic-enhanced laser fields.…

Atomic Physics · Physics 2018-07-04 Nehzat Safaei

The ionization of two-active-electron systems by intense laser fields is investigated theoretically. In comparison with time-dependent Hartree-Fock and exact two electron simulation, we show that the ionization rate is overestimated in SAE…

Atomic Physics · Physics 2015-06-18 Zengxiu Zhao , Jianmin Yuan

The electron dynamics of rare gas clusters in laser fields is investigated quantum mechanically by means of time-dependent density functional theory. The mechanism of early inner and outer ionization is revealed. The formation of an…

Atomic Physics · Physics 2009-11-10 D. Bauer , A. Macchi

We demonstrate kinematically complete measurements on frustrated double ionization of argon atoms in strong laser fields with a reaction microscope. We found that the electron trapping probability after strong field double ionization is…

Atomic Physics · Physics 2020-01-15 Seyedreza Larimian , Sonia Erattupuzha , Andrius Baltuška , Markus Kitzler , Xinhua Xie