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Finding an accurate ab initio approach for calculating the electronic properties of transition metal oxides has been a problem for several decades. In this paper, we investigate the electronic structure of the transition metal monoxides…

Strongly Correlated Electrons · Physics 2015-06-23 Suvadip Das , John E. Coulter , Efstratios Manousakis

A new implementation of the GW approximation (GWA) based on the all-electron Projector-Augmented-Wave method (PAW) is presented, where the screened Coulomb interaction is computed within the Random Phase Approximation (RPA) instead of the…

Materials Science · Physics 2009-11-10 S. Lebègue , B. Arnaud , M. Alouani , P. E. Bloechl

In this work, we perform steady-state continuous wave (cw) photoluminescence (PL) measurements on a MAPbI$_3$ thin film in the temperature range of 10-160 K, using excitation densities spanning over almost seven orders of magnitude, in…

Chu et al. recently reported extensive results of local density approximation (LDA) and of four (4) different Green function and dressed Coulomb (GW) approximation calculations of electronic properties of several semiconductors and…

Materials Science · Physics 2016-10-18 Diola Bagayoko , Yacouba Issa Diakite , Lashounda Franklin

We introduce an alternative route to quasiparticle self-consistent $GW$ calculations ($\mathrm{qs}GW$) on the basis of a Joint Approximate Diagonalization of the one-body $GW$ Green's functions $G(\varepsilon_n^{QP})$ taken at the input…

Materials Science · Physics 2024-12-05 Ivan Duchemin , Xavier Blase

The physics of electronic energy level alignment at interfaces formed between molecules and metals can in general be accurately captured by the \emph{ab initio} $GW$ approach. However, the computational cost of such $GW$ calculations for…

Materials Science · Physics 2019-06-27 Zhen-Fei Liu , Felipe H. da Jornada , Steven G. Louie , Jeffrey B. Neaton

Accurate and efficient predictions of the quasiparticle properties of complex materials remain a major challenge due to the convergence issue and the unfavorable scaling of the computational cost with respect to the system size.…

Materials Science · Physics 2020-07-14 Weiyi Xia , Weiwei Gao , Gabriel Lopez-Candales , Yabei Wu , Wei Ren , Wenqing Zhang , Peihong Zhang

We introduce a method that allows for the calculation of quasi-particle spectra in the GW approximation, yet avoiding any explicit reference to empty one-electron states. This is achieved by expressing the irreducible polarizability…

Materials Science · Physics 2015-05-14 P. Umari , G. Stenuit , S. Baroni

A GW approximation (GWA) method named U+GWA is proposed, where we can start GWA with more localized wave functions obtained by the local spin-density approximation (LSDA)+U method. Then GWA and U+GWA are applied to MnO, NiO, and V$_2$O$_3$…

Strongly Correlated Electrons · Physics 2008-10-18 S. Kobayashi , Y. Nohara , S. Yamamoto , T. Fujiwara

In many-body perturbation theory (MBPT) the self-energy \Sigma=iGW\Gamma plays the key role since it contains all the many body effects of the system. The exact self-energy is not known; as first approximation one can set the vertex…

Strongly Correlated Electrons · Physics 2012-04-23 Pina Romaniello , Friedhelm Bechstedt , Lucia Reining

Methods exhibiting linear scaling with respect to the size of the system, so called O(N) methods, are an essential tool for the calculation of the electronic structure of large systems containing many atoms. They are based on algorithms…

Condensed Matter · Physics 2007-05-23 Stefan Goedecker

We use hybrid functionals and restricted self-consistent GW, state-of-the-art theoretical approaches for quasiparticle band structures, to study the electronic states of delafossite Cu(Al,In)O$_2$, the first p-type and bipolar transparent…

Materials Science · Physics 2010-07-30 Julien Vidal , Fabio Trani , Fabien Bruneval , Miguel A. L. Marques , Silvana Botti

We describe a version of an algorithm for evolving self-gravitating collections of particles that should be nearly ideal for parallel architectures. Our method is derived from the ``self-consistent field'' (SCF) approach suggested…

Astrophysics · Physics 2016-08-30 Lars Hernquist , Steinn Sigurdsson , Greg L. Bryan

We present quasiparticle (QP) energies from fully self-consistent $GW$ (sc$GW$) calculations for a set of prototypical semiconductors and insulators within the framework of the projector-augmented wave methodology. To obtain converged…

Materials Science · Physics 2018-10-31 Manuel Grumet , Peitao Liu , Merzuk Kaltak , Jiří Klimeš , Georg Kresse

We present a simple implementation of the dynamical mean-field theory approach to the electronic structure of strongly correlated materials. This implementation achieves full self-consistency over the charge density, taking into account…

Strongly Correlated Electrons · Physics 2009-11-13 L. V. Pourovskii , B. Amadon , S. Biermann , A. Georges

We describe an implementation of Hedin's GW approximation for molecules and clusters, the complexity of which scales as O(N^3) with the number of atoms. Our method is guided by two strategies: i) to respect the locality of the underlying…

Other Condensed Matter · Physics 2015-05-27 Dietrich Foerster , Peter Koval , Daniel Sánchez-Portal

The GW approximation for the electronic self-energy is an important tool for the quantitative prediction of excited states in solids, but its mathematical exploration is hampered by the fact that it must, in general, be evaluated…

Materials Science · Physics 2013-02-27 Arno Schindlmayr

We describe the following new features which significantly enhance the power of the recently developed real-space imaginary-time GW scheme (Rieger et al., Comp. Phys. Commun. 117, 211 (1999)) for the calculation of self-energies and related…

Condensed Matter · Physics 2009-10-31 L. Steinbeck , A. Rubio , L. Reining , M. Torrent , I. D. White , R. W. Godby

We propose a novel approach to quasiparticle GW calculations which does not require the computation of unoccupied electronic states. In our approach the screened Coulomb interaction is evaluated by solving self-consistent linear-response…

Materials Science · Physics 2015-05-14 Feliciano Giustino , Marvin L. Cohen , Steven G. Louie

We describe an algorithm to generate temperature and polarization maps of the cosmic microwave background radiation containing non-Gaussianity of arbitrary local type. We apply an optimized quadrature scheme that allows us to predict and…

Cosmology and Nongalactic Astrophysics · Physics 2024-06-04 Franz Elsner , Benjamin D. Wandelt
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