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During the processes of nucleation and growth of a precipitate cluster from a supersaturated solution, the diffusion flux between the cluster and the solution changes the solute concentration near the cluster-solution interface from its…

Chemical Physics · Physics 2016-06-08 Alexander Borisenko

We investigate the early part of the crystal nucleation process in the hard sphere fluid using data produced by computer simulation. We find that hexagonal order manifests continuously in the overcompressed liquid, beginning approximately…

Soft Condensed Matter · Physics 2016-06-29 Joshua T. Berryman , Muhammad Anwar , Sven Dorosz , Tanja Schilling

Using molecular dynamics simulation, we investigate the slow dynamics of a supercooled binary mixture of soft particles interacting with a generalized Hertzian potential. At low density, it displays typical slow dynamics near its glass…

Soft Condensed Matter · Physics 2016-10-18 Ryoji Miyazaki , Takeshi Kawasaki , Kunimasa Miyazaki

Surface icing affects the safety and performance of numerous processes in technology. Previous studies mostly investigated freezing of individual droplets. The interaction among multiple droplets during freezing is investigated less,…

Soft Condensed Matter · Physics 2019-01-23 Gustav Graeber , Valentin Dolder , Thomas M. Schutzius , Dimos Poulikakos

An analytical description of nucleation stage in a supersaturated vapor with instantly created supersaturation is given with taking into account the vapor concentration inhomogeneities arising as a result of depletion due to non-stationary…

Chemical Physics · Physics 2014-04-25 Anatoly Kuchma , Maxim Markov , Alexander Shchekin

We report a molecular dynamics simulation of a supercooled simple monatomic glass-forming liquid. It is found that the onset of the supercooled regime results in formation of distinct domains of slow diffusion which are confined to the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Mikhail Dzugutov , Sergei I. Simdyankin , Fredrik H. M. Zetterling

When moist air meets a cold surface, it creates a breath figure characterized by numerous small droplets. The central question is how the vapor flux is distributed between the growth of previously condensed drops and the nucleation of new…

Fluid Dynamics · Physics 2025-08-27 Ambre Bouillant , Christopher Henkel , Uwe Thiele , Bruno Andreotti , Jacco H. Snoeijer

We study the nucleation of crystalline cluster phases in the generalized exponential model with exponent n=4. Due to the finite value of this pair potential for zero separation, at high densities the system forms cluster crystals with…

Soft Condensed Matter · Physics 2016-09-01 Christian Leitold , Christoph Dellago

We study the dynamics of quasi-two-dimensional concentrated suspensions of colloidal particles in active gels by computer simulations. Remarkably, we find that activity induces a dynamic clustering of colloids even in the absence of any…

Soft Condensed Matter · Physics 2019-10-11 G. Foffano , J. S. Lintuvuori , K. Stratford , M. E. Cates , D. Marenduzzo

We investigate the behavior of a mixture of asymmetric colloidal dumbbells and emulsion droplets by means of kinetic Monte Carlo simulations. The evaporation of the droplets and the competition between droplet-colloid attraction and…

Soft Condensed Matter · Physics 2016-05-24 Hai Pham Van , Andrea Fortini , Matthias Schmidt

We report observations of the self-assembly of coated droplets into regular clusters at the sudden expansion of a microfluidic channel. A double emulsion consisting of a regular train of coated microdroplets was created upstream of the…

Soft Condensed Matter · Physics 2020-10-19 Kerstin Schirrmann , Gabriel Cáceres-Aravena , Anne Juel

One of the most ubiquitous and technologically important phenomena in nature is the nucleation of homogeneous flowing systems. The microscopic effects of shear on a nucleating system are still imperfectly understood, although in recent…

Soft Condensed Matter · Physics 2021-08-11 Amrita Goswami , Jayant K. Singh

We report computer simulation results on the cluster formation of dipolar colloidal particles driven by a rotating external field in a quasi-two-dimensional setup. We focus on the interplay between permanent dipolar and hydrodynamic…

Soft Condensed Matter · Physics 2015-06-12 Sebastian Jäger , Holger Stark , Sabine H. L. Klapp

We investigate the collective dynamics of self-propelled droplets, confined in a one dimensional micro-fluidic channel. On one hand, neighboring droplets align and form large trains of droplets moving in the same direction. On the other…

Soft Condensed Matter · Physics 2020-05-14 Pierre Illien , Charlotte de Blois , Yang Liu , Marjolein N. van der Linden , Olivier Dauchot

Recent theories predict that when a supercooled liquid approaches the glass transition, particle clusters with a special "amorphous order" nucleate within the liquid, which lead to static correlations dictating the dramatic slowdown of…

Soft Condensed Matter · Physics 2016-03-04 Bo Zhang , Xiang Cheng

Using state-of-the-art rare-event sampling simulations, we precisely characterize the nucleation of liquid droplets from a supersaturated Lennard-Jones gas and uncover a key physical feature: critical clusters nucleate with a density that…

Chemical Physics · Physics 2026-01-07 Yijian Wu , Thomas Philippe , Aymane Graini , Julien Lam

Droplets are essential for spatially controlling biomolecules in cells. To work properly, cells need to control the emergence and morphology of droplets. On the one hand, driven chemical reactions can affect droplets profoundly. For…

Soft Condensed Matter · Physics 2024-03-14 Noah Ziethen , David Zwicker

We survey our research on modeling the mechanisms of control of uniformity in growth of nanosize and colloid particles. The former are produced as nanocrystals, by burst-nucleation from solution. The latter, colloid-size particles, are…

Soft Condensed Matter · Physics 2010-10-12 Vladimir Privman

Crystal growth and crystal coalescence processes in supercooled systems strongly depend on the concentration of crystallization centers. We perform atomistic dynamics simulations of the crystallization process in the ultrathin metallic film…

Materials Science · Physics 2019-09-04 Bulat N. Galimzyanov , Vladimir I. Ladyanov , Anatolii V. Mokshin

A mixture of hard-sphere particles and model emulsion droplets is studied with a Brownian dynamics simulation. We find that the addition of nonwetting emulsion droplets to a suspension of pure hard spheres can lead to both gas-liquid and…

Soft Condensed Matter · Physics 2015-03-13 Andrea Fortini