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Corrections to the atomic orbital sum rule for circular magnetic x-ray dichroism in solids are derived using orthonormal LMTOs as a single-particle basis for electron band states.

Materials Science · Physics 2009-10-31 R. Benoist , P. Carra , O. K. Andersen

X-ray magnetic circular dichroism (XMCD) and X-ray magnetic linear dichroism (XMLD) are powerful spectroscopic techniques for probing magnetic properties in solids. In this study, we revisit the XMCD and XMLD sum rules within a complete…

Materials Science · Physics 2025-07-03 Y. Yamasaki , Y. Ishii , N. Sasabe

We describe a new experimental setup for the detection of magnetic circular dichroism with fast electrons (EMCD). As compared to earlier findings the signal is an order of magnitude higher, while the probed area could be significantly…

Measuring magnetic moments in ferromagnetic materials with atomic column resolution is theoretically possible using the electron magnetic circular dichroism (EMCD) technique in a (scanning) transmission electron microscope ((S)TEM).…

It is known that the longitudinal and transverse excitation modes can exist in the vicinity of a quantum critical point in the ordered phase of quantum magnetic systems. The total moment sum rule for such systems is derived on the basis of…

Strongly Correlated Electrons · Physics 2020-12-04 Masashige Matsumoto

In the highly non-equilibrium conditions of laser induced spin dynamics magnetic moments can only be obtained from the spectral information, most commonly from the spectroscopy of semi-core states using the so-called x-ray magnetic circular…

Materials Science · Physics 2021-04-05 S. Shallcross , J. K. Dewhurst , P. Elliott , S. Eisebitt , C. von Korff Schmising , S. Sharma

The orbital and spin magnetic moments, and the X-ray-magnetic circular-dichroism (XMCD) spectra at the $M_{4,5}$ edges of the U atoms in a UAs/Co multilayer and in an $\alpha$-U film are calculated within the framework of the…

Strongly Correlated Electrons · Physics 2009-11-10 Matej Komelj , Natasa Stojic

A complete set of QCD sum rules for the magnetic moments of decuplet baryons are derived using the external field method. They are analyzed thoroughly using a Monte-Carlo based procedure. Valid sum rules are identified under the criteria of…

High Energy Physics - Phenomenology · Physics 2009-10-30 Frank X. Lee

Magnetic Circular Dichroism (MCD) is a standard technique for the study of magnetic properties of materials in synchrotron beamlines. We present here a new scattering geometry in the Transmission Electron Microscope through which MCD can be…

A 3-fold symmetric kagome lattice that has negative spin chirality can give a non-zero x-ray magnetic circular dichroism (XMCD) signal, despite that the total spin moment amounts to zero. This is explained by a hitherto unnoticed rule for…

Materials Science · Physics 2021-11-16 Gerrit van der Laan

Energy-loss magnetic chiral dichroism (EMCD) is a versatile method for studying magnetic properties on the nanoscale. However, the classical EMCD technique is notorious for its low signal to noise ratio (SNR). Here, we study the theoretical…

Instrumentation and Detectors · Physics 2019-03-12 Stefan Löffler , Walid Hetaba

In this work we present an alternative way to look at electron diffraction in a transmission electron microscope. In stead of writing the scattering amplitude in Fourier space as a set of plane waves, we use the cylindrical Fourier…

Instrumentation and Detectors · Physics 2015-11-13 Roeland Juchtmans , Jo Verbeeck

Rashba-split surface band is characterized by a one-to-one correspondence between the electron's momentum k and its spin orientation. Here we show that a similar correspondence between momentum and orbital angular momentum (OAM) must exist…

Electron vortex beams carry well-defined orbital angular momentum (OAM) about the propagation axis. Such beams are thus characterised by chirality features which make them potentially useful as probes of magnetic and other chiral materials.…

Quantum Physics · Physics 2015-06-15 J. Yuan , S. M. Lloyd , M. Babiker

A detailed theoretical study on the electronic structure and magnetic properties of half-metallic ferromagnet CrO$_2$ was carried out by means of relativistic full-potential linear muffin-tin orbital method within the generalized gradient…

Materials Science · Physics 2009-11-11 V. Kanchana , G. Vaitheeswaran , M. Alouani

Contrary to the optical spin angular momentum (SAM), the role played by the orbital angular momentum (OAM) of light in magneto-optics remains largely unexplored. However, the SAM and OAM are known to be coupled when light interacts with…

We present the classical electromagnetic theory framework of reflection of a light beam carrying Orbital Angular Momentum (OAM) by an in-plane magnetic structure with generic symmetry. Depending on the magnetization symmetry, we find a…

The inherent spin-orbit interaction of electrons inevitably couples spin to the orbital angular momentum (OAM), posing a fundamental challenge to spin-free orbital transport. Here, we propose a novel strategy to achieve spin-decoupled OAM…

Materials Science · Physics 2026-05-21 Dongjin Oh , Sungsoo Hahn , Chiara Pacella , Junseo Yoo , Angel Rubio , Domenico Di Sante , Changyoung Kim

In an earlier letter [Ducharme \textit{et al.} Phys. Rev. Lett. \textbf{126}, 134803 (2021)], a solution to the Dirac equation for a relativistic Gaussian electron beam showed that for a diverging beam the spin of each electron is the sum…

Quantum Physics · Physics 2026-04-24 Robert Ducharme , Irismar G. da Paz

The need to acquire multiple angle-resolved electron energy loss spectra (EELS) is one of the several critical challenges associated with electron magnetic circular dichroism (EMCD) experiments. If the experiments are performed by scanning…