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A combined experimental/theoretical study of the EPR in irradiated $\beta$-Ga$_2$O$_3$ is presented. Four EPR spectra, two $S=1/2$ and two $S=1$, are observed after high-energy proton or electron irradiation. One of the S=1/2 spectra (EPR1)…

A computational study of the electron paramagnetic resonance (EPR) $g$-tensors and hyperfine tensors in Mg and Zn doped $\beta$-Ga$_2$O$_3$ is presented. While Mg has been found previously to prefer the octahedral site, we find here that Zn…

Materials Science · Physics 2019-05-16 Dmitry Skachkov , Walter R. L. Lambrecht

Various defects in ZnO, focused on substitutional N$_O$ and N$_2$ in various sites, O-site, interstitial and Zn-site are studied using first-principles calculations with the goal of understanding the electron paramagnetic resonance (EPR)…

Materials Science · Physics 2022-11-02 Klichchupong Dabsamut , Adisak Boonchun , Walter R. L. Lambrecht

We present a state interaction spin-orbit coupling method to calculate electron paramagnetic resonance (EPR) $g$-tensors from density matrix renormalization group wavefunctions. We apply the technique to compute $g$-tensors for the…

Chemical Physics · Physics 2018-07-17 Elvira R. Sayfutyarova , Garnet K. -L. Chan

Multifrequency pulsed electron paramagnetic resonance (EPR) spectroscopy using S-, X-, Q- and W-Band frequencies (3.6, 9.7, 34, and 94 GHz, respectively) was employed to study paramagnetic coordination defects in undoped hydrogenated…

Materials Science · Physics 2011-09-20 M. Fehr , A. Schnegg , B. Rech , K. Lips , O. Asthakov , F. Finger , G. Pfanner , C. Freysoldt , J. Neugebauer , R. Bittl , C. Teutloff

Rare-earth spin ensembles are a promising platform for microwave quantum memory applications due to their hyperfine transitions, which can exhibit exceptionally long coherence times when using an operation point with zero first-order Zeeman…

Gallium oxide (b-Ga2O3) is a wide-bandgap compound semiconductor with a bandgap of ~ 4.9 eV that is currently considered promising for a wide range of applications ranging from transparent conducting electrodes to UV optoelectronic devices…

Materials Science · Physics 2020-01-08 Jan E. Stehr , Detlev M. Hofmann , Weimin M. Chen , Irina A. Buyanova

We present an electron paramagnetic resonance (EPR) study of ErSc2N@C80 fullerene in which there are two Er3+ sites corresponding to two different configurations of the ErSc2N cluster inside the C80 cage. For each configuration, the EPR…

Understanding (and controlling) hyperfine interactions in semiconductor nanostructures is important for fundamental studies of material properties as well as for quantum information processing with electron, hole, and nuclear-spin states.…

Mesoscale and Nanoscale Physics · Physics 2020-03-06 Pericles Philippopoulos , Stefano Chesi , W. A. Coish

Monolayer graphene grown by chemical vapor deposition and transferred to SiO_2 is used to introduce vacancies by Ar^+ ion bombardment at a kinetic energy of 50 eV. The density of defects visible in scanning tunneling microscopy (STM) is…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 S. Just , S. Zimmermann , V. Kataev , B. Buechner , M. Pratzer , M. Morgenstern

Electron paramagnetic resonance (EPR) is a valuable tool for physics, chemistry, biology and medicine, providing complementary spectroscopic information to NMR. It has long been known that EPR at high magnetic fields offers greater spectral…

The chemical, structural, mechanical, and dynamical stabilities of the $\alpha$- and $\beta$-Ga$_2$O$_3$ are confirmed from respective negative formation energies, negative cohesive energies, favorable elastic constants, and positive phonon…

Materials Science · Physics 2025-03-18 Yogendra Limbu , Hari Paudyal , Michael E. Flatté , Durga Paudyal

F+ center, an electron trapped at oxygen vacancy (VO), was investigated in the oxygen deficient Y3Al5O12 (YAG) crystals by EPR. The measurements were performed at temperatures 5-450 K and frequencies 9.4-350 GHz with using both the continue…

Materials Science · Physics 2020-01-22 V. Laguta , M. Buryi , S. Tkachenko , P. Arhipov , I. Gerasymov , O. Sidletskiy , O. Laguta , M. Nikl

We present general expressions for the magnetic transition rates in beam Electron Paramagnetic Resonance (EPR) experiments of anisotropic spin systems in the solid state. The expressions apply to general spin centers and arbitrary…

Mesoscale and Nanoscale Physics · Physics 2015-01-14 Joscha Nehrkorn , Alexander Schnegg , Karsten Holldack , Stefan Stoll

Proton irradiation of both n-type and semi-insulating bulk samples of \b{eta}-Ga2O3 leads to the formation of one paramagnetic defect with spin S=1/2, monoclinic point symmetry, a g-tensor with principal values of gb=2.0313, gc=2.0079, ga*=…

Electrically detected electron spin resonance (ESR) is used to study the hyperfine interaction of the two-dimensional electrons and the nuclei of the host lattice in a GaAs/AlGaAs heterostructure. Under the microwave and radio- frequency…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Chris Hillman , H. W. Jiang

Electron paramagnetic resonance (EPR) can provide unique insight into the chemical structure and magnetic properties of dopants in oxide and semiconducting materials that are of interest for applications in electronics, catalysis, and…

Metastable photoinduced Electron Paramagnetic Resonance (EPR) signal at low temperatures is reported in GaN alloyed with boron ($B_{x}Ga_{1-x}N$) epitaxial layers grown at temperatures ranging from 840 {\deg}C to 1090 {\deg}C. An isotropic…

We describe instrumentation for a high-frequency electron paramagnetic resonance (EPR) and pulsed electron-electron double resonance (PELDOR) spectroscopy. The instrumentation is operated in the frequency range of 107$-$120 GHz and…

Instrumentation and Detectors · Physics 2015-06-19 Franklin H. Cho , Viktor Stepanov , Susumu Takahashi

We report results of a multi-frequency (0.8-60 GHz) electron spin resonance study of the spin dynamics in the quasi-2D square lattice antiferromagnet Ba$_2$MnGe$_2$O$_7$ both in antiferromagnetically ordered and paramagnetic phases. We…

Strongly Correlated Electrons · Physics 2024-01-02 V. N. Glazkov , Yu. V. Krasnikova , I. K. Rodygina , H. -A. Krug von Nidda , T. Masuda
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