Related papers: Optically Driven Magnetic Phase Transition of Mono…
The parallel or antiparallel arrangement of electron spins plays a pivotal role in determining the properties of a physical system. To meet the demands for innovative technological solutions, extensive efforts have been dedicated to…
Leveraging coherent light-matter interaction in solids is a promising new direction towards control and functionalization of quantum materials, to potentially realize regimes inaccessible in equilibrium and stabilize new or useful states of…
Controlling the optical properties of rare-earth ions in wide-bandgap semiconductors remains a major challenge in the development of next-generation photonic materials. Here, we show that external hydrostatic pressure modulates the…
$\alpha$-RuCl$_3$ is a promising candidate material to realize the so far elusive quantum spin liquid ground state. However, at low temperatures, the coexistence of different exchange interactions couple the effective pseudospins into an…
Based on nonlinear optics, we develop a band theory to elucidate how light could manipulate magnetization, which is rooted by the quantum geometric structure and topological nature of electronic wavefunctions. Their existence are determined…
Resistivity measurements are widely exploited to uncover electronic excitations and phase transitions in metallic solids. While single crystals are preferably studied to explore crystalline anisotropies, these usually cancel out in…
In this article, we review recent theoretical research on photocontrol of magnetism in several spin-charge coupled systems. The control of magnetism with light has been a central issue in condensed-matter physics, attracting enormous…
Controlling magnetism and spin structures in strongly correlated systems by using electric field is of fundamental importance but challenging. Here, a high-spin ruthenate phase is achieved via a solid ionic chemical junction at…
Magnetization and high-resolution x-ray diffraction measurements of the Kitaev-Heisenberg material alpha-RuCl3 reveal a pressure-induced crystallographic and magnetic phase transition at a hydrostatic pressure of p=0.2 GPa. This structural…
The majority of research on $\alpha$-RuCl$_3$ has focused on applying in-plane magnetic fields to suppress antiferromagnetic order and induce a quantum spin liquid (QSL). However, this effort has been complicated by the materials…
Ultrathin bismuth exhibits rich physics including strong spin-orbit coupling, ferroelectricity, nontrivial topology, and light-induced structural dynamics. We use \textit{ab initio} calculations to show that light can induce structural…
Long before the recent fascination with two-dimensional materials, the critical behaviour and universality scaling of phase transitions in low-dimensional systems has been a topic of great interest. Particularly intriguing is the case of…
Efficient control of a magnetization without an application of the external magnetic fields is the ultimate goal of spintronics. We demonstrate, that in monolayers of $\text{CrI}_3$, magnetization can be switched all optically, by…
The realization of long-range magnetic ordering in two-dimensional (2D) systems can potentially revolutionize next-generation information technology. Here, we report the successful fabrication of crystalline Cr3Te4 monolayers with room…
Material research has been a major driving force in the development of modern nano-electronic devices. In particular, research in magnetic thin films has revolutionized the development of spintronic devices; identifying new magnetic…
At optical frequencies, interactions of the electric field component of light with matter are dominating, whereas magnetic dipole transitions are inherently weak and challenging to access independently from electric dipole transitions.…
Single wall carbon nanotubes grown entirely from 13-C form an ideal system to study the effect of electron interaction on nuclear magnetism in one dimension. If the electrons are in the metallic, Luttinger liquid regime, we show that even a…
Motivated by the possibility of an intermediate U(1) quantum spin liquid phase in out-of-plane magnetic fields and enhanced magnetic fluctuations in exfoliated {\alpha}-RuCl3 flakes, we study magneto-Raman spectra of exfoliated multilayer…
Two-dimensional (2D) materials enable new types of magnetic and electronic phases mediated by their reduced dimensionality like magic-angle induced phase transitions, 2D Ising antiferromagnets and ferromagnetism in 2D atomic layers and…
We report high-resolution dilatometry on high-quality single crystals of NiTiO3 grown by means of the optical floating-zone technique. The anisotropic magnetic phase diagram is constructed from thermal expansion and magnetostriction studies…