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Quantum systems of indistinguishable particles are commonly described using the formalism of second quantisation, which relies on the assumption that any admissible quantum state must be either symmetric or anti-symmetric under particle…

Quantum Physics · Physics 2023-07-13 Benjamin Yadin , Benjamin Morris , Kay Brandner

We introduce the time-dependent restricted active space Configuration Interaction method to solve the time-dependent Schr\"odinger equation for many-electron atoms, and particularly apply it to the treatment of photoionization processes in…

Atomic Physics · Physics 2013-05-30 David Hochstuhl , Michael Bonitz

In two previous papers (Price & Monaghan 2004a,b) (papers I,II) we have described an algorithm for solving the equations of Magnetohydrodynamics (MHD) using the Smoothed Particle Hydrodynamics (SPH) method. The algorithm uses dissipative…

Astrophysics · Physics 2009-11-13 D. J. Price , J. J. Monaghan

This paper presents the first implementation of a coupling between advanced wave function theories and molecular density functional theory (MDFT). This method enables the modeling of solvent effect into quantum mechanical (QM) calculations…

Chemical Physics · Physics 2024-04-12 Maxime Labat , Emmanuel Giner , Guillaume Jeanmairet

Solving non-Hermitian quantum many-body systems on a quantum computer by minimizing the variational energy is challenging as the energy can be complex. Here, based on energy variance, we propose a variational method for solving the…

Quantum Physics · Physics 2024-02-21 Xu-Dan Xie , Zheng-Yuan Xue , Dan-Bo Zhang

A system of $N$ particles in a chemical medium in $\mathbb{R}^{d}$ is studied in a discrete time setting. Underlying interacting particle system in continuous time can be expressed as \begin{eqnarray} dX_{i}(t) &=&[-(I-A)X_{i}(t) +…

Probability · Mathematics 2017-01-10 Abhishek Pal Majumder

We present a systematic method for dealing with time dependent quantum dynamics, based on the quantum brachistochrone and matrix mechanics. We derive the explicit time dependence of the Hamiltonian operator for a number of constrained…

Quantum Physics · Physics 2012-10-29 Peter G. Morrison

We propose a simple quantum algorithm for simulating highly oscillatory quantum dynamics, which does not require complicated quantum control logic for handling time-ordering operators. To our knowledge, this is the first quantum algorithm…

Quantum Physics · Physics 2022-04-20 Dong An , Di Fang , Lin Lin

The molecular dynamics following the electronic $B\ ^3\Pi_u\left(0^+\right) \longleftarrow X\ ^1\Sigma_g^+$ photoexcitation of the iodine molecule embedded in solid krypton are studied quantum mechanically using the Gaussian variant of the…

Chemical Physics · Physics 2019-03-27 David Picconi , Jeffrey A. Cina , Irene Burghardt

We present unrestricted Hartree Fock method coupled with configuration interaction (CI) method (URHF-CI) suitable for the calculation of ground and excited states of large number of electrons localized by complex gate potentials in…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Ramin M. Abolfath , Pawel Hawrylak

{Many-body quantum states at thermal equilibrium are ubiquitous in nature. Investigating their dynamical properties is a formidable task due to the complexity of the Hilbert space they live in. Quantum computers may have the potential to…

Quantum Physics · Physics 2024-07-25 Mirko Consiglio , Tony J. G. Apollaro

Simulating and predicting dynamics of quantum many-body systems is extremely challenging, even for state-of-the-art computational methods, due to the spread of entanglement across the system. However, in the long-wavelength limit, quantum…

Hamiltonian and Schrodinger evolution equations on finite-dimensional projective space are analyzed in detail. Hartree-Fock (HF) manifold is introduced as a submanifold of many electron projective space of states. Evolution equations, exact…

Chemical Physics · Physics 2011-11-10 A. I. Panin

A dynamical formulation of coupled cluster theory is derived using a variational principle. By allowing time-dependent single-particle functions, a high degree of adaptivity is introduced, allowing complex systems to be simulated with high…

Quantum Physics · Physics 2014-11-25 Simen Kvaal

We present a formulation and numerical algorithm to extend the scheme for grey radiation magneto-hydrodynamics (MHD) developed by Jiang (2021) to include the frequency dependence via the multi-group approach. The entire frequency space can…

Instrumentation and Methods for Astrophysics · Physics 2022-09-15 Yan-Fei Jiang

In quantum physics the free particle and the harmonically trapped particle are arguably the most important systems a physicist needs to know about. It is little known that, mathematically, they are one and the same. This knowledge helps us…

Quantum Physics · Physics 2014-06-18 Ole Steuernagel

We present the AM$^3$ ("Astrophysical Multi-Messenger Modeling") software. AM$^3$ is a documented open source software that efficiently solves the coupled integro-differential equations describing the temporal evolution of the spectral…

Recent progress in the realm of noisy, intermediate scale quantum (NISQ) devices represents an exciting opportunity for many-body physics, by introducing new laboratory platforms with unprecedented control and measurement capabilities. We…

Disordered Systems and Neural Networks · Physics 2021-09-24 Matteo Ippoliti , Kostyantyn Kechedzhi , Roderich Moessner , S. L. Sondhi , Vedika Khemani

We consider a general class of discrete unitary dynamical models on the lattice. We show that generically such models give rise to a wavefunction satisfying a Schroedinger equation in the continuum limit, in any number of dimensions. There…

Quantum Physics · Physics 2008-02-03 Bruce M. Boghosian , Washington Taylor

We consider within a finite element approach the usage of different adaptively refined meshes for different variables in systems of nonlinear, time-depended PDEs. To resolve different solution behaviours of these variables, the meshes can…

Numerical Analysis · Mathematics 2010-05-27 Thomas Witkowski , Axel Voigt