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We consider a mechanism to generate controllable qudit-qudit interactions in a charge-position paradigm for a quantum computer, through the use of auxiliary states. By controlling the tunneling rates onto these auxiliaries from the qudits…

Quantum Physics · Physics 2007-05-23 S. G. Schirmer , A. D. Greentree , D. K. L. Oi

Electronic defects in semiconductors form the basis for many emerging quantum technologies. Understanding defect spin and charge dynamics in solid state platforms is crucial to developing these building blocks, but many defect centers are…

Quantum computers promise to revolutionise electronic simulations by overcoming the exponential scaling of many-electron problems. While electronic wave functions can be represented using a product of fermionic unitary operators, shallow…

Quantum Physics · Physics 2022-07-04 Hugh G. A. Burton , Daniel Marti-Dafcik , David P. Tew , David J. Wales

Despite an apparent progress in implementing individual solid-state qubits, there have been no experimental reports so far on multi-bit gates required for building a real quantum computer. Here we report a new circuit comprising two coupled…

Mesoscale and Nanoscale Physics · Physics 2010-04-20 Yu. A. Pashkin , T. Yamamoto , O. Astafiev , Y. Nakamura , D. V. Averin , J. S. Tsai

Creating a quantum-coherent architecture at the atomic scale has long been an ambition in quantum science and nanotechnology. This ultimate length scale requires the use of fundamental quantum properties of atoms, such as the spin of…

Quantum computers hold promise to improve the efficiency of quantum simulations of materials and to enable the investigation of systems and properties more complex than tractable at present on classical architectures. Here, we discuss…

Quantum Physics · Physics 2022-05-03 Christian Vorwerk , Nan Sheng , Marco Govoni , Benchen Huang , Giulia Galli

We show how a quantum computer can be employed to elucidate reaction mechanisms in complex chemical systems, using the open problem of biological nitrogen fixation in nitrogenase as an example. We discuss how quantum computers can augment…

Quantum Physics · Physics 2017-08-14 Markus Reiher , Nathan Wiebe , Krysta M Svore , Dave Wecker , Matthias Troyer

Quantum simulators, in which well controlled quantum systems are used to reproduce the dynamics of less understood ones, have the potential to explore physics that is inaccessible to modeling with classical computers. However, checking the…

Quantum Physics · Physics 2015-06-18 C. Senko , J. Smith , P. Richerme , A. Lee , W. C. Campbell , C. Monroe

We study a two-electron quantum dot molecule in a magnetic field by the direct diagonalization of the Hamiltonian matrix. The ground states of the molecule with the total spin S=0 and S=1 provide a possible realization for a qubit of a…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 A. Harju , S. Siljamäki , R. M. Nieminen

We study the low energy states of finite spin chains with isotropic (Heisenberg) and anisotropic (XY and Ising-like) exchange interaction with uniform and non-uniform coupling constants. We show that for an odd number of sites a spin…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Florian Meier , Jeremy Levy , Daniel Loss

We present a brief survey of methods that utilize computer simulations and quantum and statistical mechanics in the analysis of electrochemical systems. The methods, Molecular Dynamics and Monte Carlo simulations and quantum-mechanical…

Chemical Physics · Physics 2009-10-15 P. A. Rikvold , I. Abou Hamad , T. Juwono , D. T. Robb , M. A. Novotny

Constructing general programmable circuits to be able to run any given unitary operator efficiently on a quantum processor is of fundamental importance. We present a new quantum circuit design technique resulting two general programmable…

Quantum Physics · Physics 2012-07-24 Anmer Daskin , Ananth Grama , Giorgos Kollias , Sabre Kais

Quantum phase estimation is at the heart of most quantum algorithms with exponential speedup. In this letter we demonstrate how to utilize it to compute the dynamical response functions of many-body quantum systems. Specifically, we design…

Quantum Physics · Physics 2021-05-21 Dries Sels , Eugene Demler

Measurement of charge configurations in few-electron quantum dots is a vital technique for spin-based quantum information processing. While fast and high-fidelity measurement is possible by using proximal quantum dot charge sensors, their…

Mesoscale and Nanoscale Physics · Physics 2021-03-30 Takashi Nakajima , Yohei Kojima , Yoshihiro Uehara , Akito Noiri , Kenta Takeda , Takashi Kobayashi , Seigo Tarucha

Characterizing thermally activated transitions in high-dimensional rugged energy surfaces is a very challenging task for classical computers. Here, we develop a quantum annealing scheme to solve this problem. First, the task of finding the…

Quantum Physics · Physics 2021-01-18 Philipp Hauke , Giovanni Mattiotti , Pietro Faccioli

Optically connecting quantum bits can effectively reduce decoherence and facilitate long-distance communication. Optically addressable spin-bearing molecules have been demonstrated to have a good potential for quantum computing. In this…

Quantum Physics · Physics 2023-03-28 Jiawei Chang , Tianhong Huang , Lin Ma , Taoyu Zou , Hai Wang , Wei Wu

Shallow, CNOT-efficient quantum circuits are crucial for performing accurate computational chemistry simulations on current noisy quantum hardware. Here, we explore the usefulness of non-iterative energy corrections, based on the method of…

Chemical Physics · Physics 2023-05-03 Ilias Magoulas , Francesco A. Evangelista

Graph-based linear scaling electronic structure theory for quantum-mechanical molecular dynamics simulations is adapted to the most recent shadow potential formulations of extended Lagrangian Born-Oppenheimer molecular dynamics, including…

Chemical Physics · Physics 2023-03-08 Christian F. A. Negre , Michael E. Wall , Anders M. N. Niklasson

Given the effectiveness of semiconductor devices for classical computation one is naturally led to consider semiconductor systems for solid state quantum information processing. Semiconductors are particularly suitable where local control…

Materials Science · Physics 2009-11-11 A. M. Tyryshkin , J. J. L. Morton , S. C. Benjamin , A. Ardavan , G. A. D. Briggs , J. W. Ager , S. A. Lyon

We use the spin-polarized excitons in a single quantum dot to design optical controls for basic operations in quantum computing. We examine the ultrafast nonlinear optical processes required and use the coherent nonlinear optical responses…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Pochung Chen , C. Piermarocchi , L. J. Sham